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This set of lectures provides an introduction to the structure, thermodynamics and dynamics of liquids, binary solutions and polymers at a level that will enable graduate students and non-specialist researchers to understand more specialized literature and to possibly start their own work in this field. Part I starts with the introduction of distribution functions, which describe the statistical arrangements of atoms or molecules in a simple liquid. The main concepts involve mean field theories like the Perkus-Yevick theory and the random phase approximation, which relate the forces to the distribution functions. In order to provide a concise, self-contained text, an understanding of the general statistical mechanics of an interacting many-body system is assumed. The fact that in a classic liquid the static and dynamic aspects of such a system can be discussed separately forms the basis of the two-fold structure of this approach. In order to allow polymer melts and solutions to be discussed, a short chapter acquaints readers with scaling concepts by discussing random walks and fractals. Part II of the lecture series is essentially devoted to the presentation of the dynamics of simple and complex liquids in terms of the generalized hydrodynamics concept, such as that introduced by Mori and Zwanzig. A special topic is a comprehensive introduction of the liquid-glass transition and its discussion in terms of a mode-coupling theory.
Of the three basic states of matter, liquid is perhaps the most complex. While its flow properties are described by fluid mechanics, its thermodynamic properties are often neglected, and for many years it was widely believed that a general theory of liquid thermodynamics was unattainable. In recent decades that view has been challenged, as new advances have finally enabled us to understand and describe the thermodynamic properties of liquids. This book explains the recent developments in theory, experiment and modelling that have enabled us to understand the behaviour of excitations in liquids and the impact of this behaviour on heat capacity and other basic properties. Presented in plain language with a focus on real liquids and their experimental properties, this book is a useful reference text for researchers and graduate students in condensed matter physics and chemistry as well as for advanced courses covering the theory of liquids.
This short primer offers non-specialist readers a concise, yet comprehensive introduction to the field of classical fluids – providing both fundamental information and a number of selected topics to bridge the gap between the basics and ongoing research. In particular, hard-sphere systems represent a favorite playground in statistical mechanics, both in and out of equilibrium, as they represent the simplest models of many-body systems of interacting particles, and at higher temperature and densities they have proven to be very useful as reference systems for real fluids. Moreover, their usefulness in the realm of soft condensed matter has become increasingly recognized – for instance, the effective interaction among (sterically stabilized) colloidal particles can be tuned to almost perfectly match the hard-sphere model. These lecture notes present a brief, self-contained overview of equilibrium statistical mechanics of classical fluids, with special applications to both the structural and thermodynamic properties of systems made of particles interacting via the hard-sphere potential or closely related model potentials. In particular it addresses the exact statistical-mechanical properties of one-dimensional systems, the issue of thermodynamic (in)consistency among different routes in the context of several approximate theories, and the construction of analytical or semi-analytical approximations for the structural properties. Written pedagogically at the graduate level, with many figures, tables, photographs, and guided end-of-chapter exercises, this introductory text benefits students and newcomers to the field alike.
Phases of Matter and their Transitions An all-in-one, comprehensive take on matter and its phase properties In Phases of Matter and their Transitions, accomplished materials scientist Dr. Gijsbertus de With delivers an accessible textbook for advanced students in the molecular sciences. It offers a balanced and self-contained treatment of the thermodynamic and structural aspects of phases and the transitions between them, covering solids, liquids, gases, and their interfaces. The book lays the groundwork to describe particles and their interactions from the perspective of classical and quantum mechanics and compares phenomenological and statistical thermodynamics. It also examines materials with special properties, like glasses, liquid crystals, and ferroelectrics. The author has included an extensive appendix with a guide to the mathematics and theoretical models employed in this resource. Readers will also find: Thorough introductions to classical and quantum mechanics, intermolecular interactions, and continuum mechanics Comprehensive explorations of thermodynamics, gases, liquids, and solids Practical discussions of surfaces, including their general aspects for solids and liquids Fulsome treatments of discontinuous and continuous transitions, including discussions of irreversibility and the return to equilibrium Perfect for advanced students in chemistry and physics, Phases of Matter and their Transitions will also earn a place in the libraries of students of materials science.
This pedagogical and self-contained text describes the modern mean field theory of simple structural glasses. The book begins with a thorough explanation of infinite-dimensional models in statistical physics, before reviewing the key elements of the thermodynamic theory of liquids and the dynamical properties of liquids and glasses. The central feature of the mean field theory of disordered systems, the existence of a large multiplicity of metastable states, is then introduced. The replica method is then covered, before the final chapters describe important, advanced topics such as Gardner transitions, complexity, packing spheres in large dimensions, the jamming transition, and the rheology of glass. Presenting the theory in a clear and pedagogical style, this is an excellent resource for researchers and graduate students working in condensed matter physics and statistical mechanics.
A self-contained, mathematical introduction to the driving ideas in equilibrium statistical mechanics, studying important models in detail.
An introductory book on the statistical mechanics of disordered systems, ideal for graduates and researchers.
''Intended mainly for physicists and mathematicians...its high quality will definitely attract a wider audience.'' ---Computational Mathematics and Mathematical Physics This work acquaints the physicist with the mathematical principles of algebraic topology, group theory, and differential geometry, as applicable to research in field theory and the theory of condensed matter. Emphasis is placed on the topological structure of monopole and instanton solution to the Yang-Mills equations, the description of phases in superfluid 3He, and the topology of singular solutions in 3He and liquid crystals.
This book describes significant tractable models used in solid mechanics - classical models used in modern mechanics as well as new ones. The models are selected to illustrate the main ideas which allow scientists to describe complicated effects in a simple manner and to clarify basic notations of solid mechanics. A model is considered to be tractable if it is based on clear physical assumptions which allow the selection of significant effects and relatively simple mathematical formulations. The first part of the book briefly reviews classical tractable models for a simple description of complex effects developed from the 18th to the 20th century and widely used in modern mechanics. The second part describes systematically the new tractable models used today for the treatment of increasingly complex mechanical objects – from systems with two degrees of freedom to three-dimensional continuous objects.