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Advanced separations technology is key to closing the nuclear fuel cycle and relieving future generations from the burden of radioactive waste produced by the nuclear power industry. Nuclear fuel reprocessing techniques not only allow for recycling of useful fuel components for further power generation, but by also separating out the actinides, lanthanides and other fission products produced by the nuclear reaction, the residual radioactive waste can be minimised. Indeed, the future of the industry relies on the advancement of separation and transmutation technology to ensure environmental protection, criticality-safety and non-proliferation (i.e., security) of radioactive materials by reducing their long-term radiological hazard.Advanced separation techniques for nuclear fuel reprocessing and radioactive waste treatment provides a comprehensive and timely reference on nuclear fuel reprocessing and radioactive waste treatment. Part one covers the fundamental chemistry, engineering and safety of radioactive materials separations processes in the nuclear fuel cycle, including coverage of advanced aqueous separations engineering, as well as on-line monitoring for process control and safeguards technology. Part two critically reviews the development and application of separation and extraction processes for nuclear fuel reprocessing and radioactive waste treatment. The section includes discussions of advanced PUREX processes, the UREX+ concept, fission product separations, and combined systems for simultaneous radionuclide extraction. Part three details emerging and innovative treatment techniques, initially reviewing pyrochemical processes and engineering, highly selective compounds for solvent extraction, and developments in partitioning and transmutation processes that aim to close the nuclear fuel cycle. The book concludes with other advanced techniques such as solid phase extraction, supercritical fluid and ionic liquid extraction, and biological treatment processes.With its distinguished international team of contributors, Advanced separation techniques for nuclear fuel reprocessing and radioactive waste treatment is a standard reference for all nuclear waste management and nuclear safety professionals, radiochemists, academics and researchers in this field. - A comprehensive and timely reference on nuclear fuel reprocessing and radioactive waste treatment - Details emerging and innovative treatment techniques, reviewing pyrochemical processes and engineering, as well as highly selective compounds for solvent extraction - Discusses the development and application of separation and extraction processes for nuclear fuel reprocessing and radioactive waste treatment
This book provides a readable and thought-provoking analysis of the issues surrounding nuclear fuel reprocessing and fast-neutron reactors, including discussion of resources, economics, radiological risk and resistance to nuclear proliferation. It describes the history and science behind reprocessing, and gives an overview of the status of reprocessing programmes around the world. It concludes that such programs should be discontinued. While nuclear power is seen by many as the only realistic solution to the carbon emission problem, some national nuclear establishments have been pursuing development and deployment of sodium-cooled plutonium breeder reactors, and plutonium recycling. Its proponents argue that this system would offer significant advantages relative to current light water reactor technology in terms of greater uranium utilization efficiency, and that separating out the long-lived plutonium and other transuranics from spent fuel and fissioning them in fast reactors would greatly reduce the duration of the toxicity of radioactive waste. However, the history of efforts to deploy this system commercially in a number of countries over the last six decades has been one of economic and technical failure and, in some cases, was used to mask clandestine nuclear weapon development programs. Covering topics of significant public interest including nuclear safety, fuel storage, environmental impact and the spectre of nuclear terrorism, this book presents a comprehensive analysis of the issue for nuclear engineers, policy analysts, government officials and the general public. "Frank von Hippel, Jungmin Kang, and Masafumi Takubo, three internationally renowned nuclear experts, have done a valuable service to the global community in putting together this book, which both historically and comprehensively covers the “plutonium age” as we know it today. They articulate in a succinct and clear manner their views on the dangers of a plutonium economy and advocate a ban on the separation of plutonium for use in the civilian fuel cycle in view of the high proliferation and nuclear-security risks and lack of economic justification." (Mohamed ElBaradei, Director General, International Atomic Energy Agency (1997-2009), Nobel Peace Prize (2005)) "The 1960s dream of a ‘plutonium economy’ has not delivered abundant low-cost energy, but instead has left the world a radioactive legacy of nuclear weapons proliferation and the real potential for nuclear terrorism. Kang, Takubo, and von Hippel explain with power and clarity what can be done to reduce these dangers. The governments of the remaining countries whose nuclear research and development establishments are still pursuing the plutonium dream should pay attention.” (Senator Edward Markey, a leader in the US nuclear-disarmament movement as a member of Congress since 1976) "The authors have done an invaluable service by putting together in one place the most coherent analysis of the risks associated with plutonium, and the most compelling argument for ending the practice of separating plutonium from spent fuel for any purpose. They have given us an easily accessible history of the evolution of thinking about the nuclear fuel cycle, the current realities of nuclear power around the world and, arguably most important, a clear alternative path to deal with the spent fuel arising from nuclear reactors for decades to centuries to come." (Robert Gallucci, Chief US negotiator with North Korea (1994); Dean, Georgetown University School of Foreign Service (1996-2009); President, MacArthur Foundation (2009-2014))
Drawing on the authors' extensive experience in the processing and disposal of waste, An Introduction to Nuclear Waste Immobilisation, Second Edition examines the gamut of nuclear waste issues from the natural level of radionuclides in the environment to geological disposal of waste-forms and their long-term behavior. It covers all-important aspects of processing and immobilization, including nuclear decay, regulations, new technologies and methods. Significant focus is given to the analysis of the various matrices used, especially cement and glass, with further discussion of other matrices such as bitumen. The final chapter concentrates on the performance assessment of immobilizing materials and safety of disposal, providing a full range of the resources needed to understand and correctly immobilize nuclear waste.
This book lays a comprehensive foundation for addressing the issue of safety in the lifecycle of nuclear waste. With the focus on the fundamental principles, the book covers key technical approaches to safety in the management of spent nuclear fuel, reprocessed high-level waste, low-level waste, and decommissioning wastes. Behaviors of nuclear waste in natural and engineered systems in relation to safety assessment are also described through the explanation of fundamental processes. For any country involved with the use of nuclear power, nuclear waste management is a topic of grave importance. Although many countries have heavily invested in nuclear waste management, having a successful national program still remains a major challenge. This book offers substantial guidance for those seeking solutions to these problems. As the problem of nuclear waste management is heavily influenced by social factors, the connection between technical and social issues in nuclear waste management is also discussed. The book is a core text for advanced students in nuclear and environmental engineering, and a valuable reference for those working in nuclear engineering and related areas.
Reprocessing and Recycling of Spent Nuclear Fuel presents an authoritative overview of spent fuel reprocessing, considering future prospects for advanced closed fuel cycles. Part One introduces the recycling and reprocessing of spent nuclear fuel, reviewing past and current technologies, the possible implications of Generation IV nuclear reactors, and associated safely and security issues. Parts Two and Three focus on aqueous-based reprocessing methods and pyrochemical methods, while final chapters consider the cross-cutting aspects of engineering and process chemistry and the potential for implementation of advanced closed fuel cycles in different parts of the world. - Expert introduction to the recycling and reprocessing of spent nuclear fuel - Detailed overview of past and current technologies, the possible implications of Generation IV nuclear reactors, and associated safely and security issues - A lucid exploration of aqueous-based reprocessing methods and pyrochemical methods
Nuclear power has been questioned almost since its early stages and one of the major issues in relation to its social acceptability around the world is nuclear waste management. An important and inevitable by-product of nuclear energy production is the spent nuclear fuel that needs to be managed and handled in a safe, responsible and effective way. Thus, reprocessing and recycling of spent nuclear fuel (SNF) could be one of the key points to advance the social acceptability of nuclear energy. Hence, it is very significant to know the technologies available for SNF management, their advantages and disadvantages, the technologies that are currently under research and the future R&D tendencies, as well as which alternative suits better the needs for each country and its particular context. Furthermore, the interactions among legal, economic, and technological issues are essential. This book covers the state of the art technologies on the recycling and reprocessing of spent nuclear fuel, reviewing past and current technologies, the possible implications of Fourth Generation nuclear reactors, and associated safely and security issues. It introduces both the conventional cycle along with new fuel cycle technologies and analyzes the benefits, economic considerations, and proliferation risks of spent nuclear fuel reprocessing. This book gives an overall view of the technologies available for SNF management, analyses the economic cost that the use of the different technologies could entail, as is key when selecting a strategy for SNF management, highlights the importance of the legislation and some intangible assets, such as social acceptability of the technology, which can have an influence so important that it may lead to the disappearance of that technology by making it economically unviable. This book will be of valued for Students, researchers as well as professionals working on the separation and recycling of spent nuclear fuel.
The implementation of advanced nuclear systems requires that new technologies associated with the back end of the fuel cycle are developed. The separation of minor actinides from other fuel components is one of the advanced concepts being studied to help close the nuclear fuel cycle and to improve the long-term effects on the performance of geological repositories. Separating spent fuel elements and subsequently converting them through transmutation into short-lived nuclides should considerably reduce the longterm risks associated with nuclear power generation.
Describes the rationale and vision for the peaceful use of nuclear energy. The publication identifies the basic principles that nuclear energy systems must satisfy to fulfil their promise of meeting growing global energy demands.