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Exciton dynamics in semiconductor nanostructures are dominated by the effects of many-body physics. The application of coherent spectroscopic tools, such as two-dimensional Fourier transform spectroscopy (2dFTS), to the study of these systems can reveal signatures of these effects, and in combination with sophisticated theoretical modeling, can lead to more complete understanding of the behaviour of these systems. 2dFTS has previously been applied to the study of GaAs quantum well samples. In this thesis, we outline a precis of the technique before describing our own experiments using 2dFTS in a partially collinear geometry. This geometry has previously been used to study chemical systems, but we believe these experiments to be the first such performed on semiconductor samples. We extend this technique to a reflection mode 2dFTS experiment, which we believe to be the first such measurement. In order to extend the techniques of coherent spectroscopy to structured systems, we construct an experimental apparatus that permits us to control the beam geometry used to perform four-wave mixing reflection measurements. To isolate extremely weak signals from intense background fields, we extend a conventional lock-in detection scheme to one that treats the optical fields exciting the sample on an unequal footing. To the best of our knowledge, these measurements represent a novel spectroscopic tool that has not previously been described.
The applications of nonlinear ultrafast spectroscopy are numerous and widespread and it is an established and indispensable technique for revealing ultrafast processes in modern material, chemical and biochemical research. Unfortunately it is also a topic that can be daunting to those meeting it for the first time. Assuming just an understanding of quantum mechanics and statistical mechanics and making use of many worked examples and accompanied by MATLAB codes for numerical simulations of spectra, this book delivers a practical and intuitive introduction to the subject for advanced students and researchers. It will also be useful for practitioners, who are already familiar with the subject, but who want to develop a more conceptual understanding. In this clear text, experienced practitioners present a simple and conceptually intuitive overview of ultrafast nonlinear spectroscopy using the formalism of quantum processes and wavepacket dynamics. Using this unified framework the authors provide the reader with simple analytical models, examples and concepts to understand the workings of nonlinear spectroscopy through a pedagogical and physically intuitive approach. The core of the book is the section on pump-probe spectroscopy as on understanding its mathematical description, more complex and multidimensional spectroscopies become easily understood derivatives. Readers, once familiar with the material in this text, will be fully equipped with the tools to devise and undertake well-reasoned spectroscopic experiments.
This volume is a collection of papers presented at the Ninth International Symposium on "Ultrafast Processes in Spectroscopy" (UPS '95) held at the International Centre for Theo retical Physics (ICTP), Trieste (Italy), October 30 -November 3, 1995. These meetings have become recognized as the major forum in Europe for discussion of new work in this rapidly moving field. The UPS'95 Conference in Trieste brought together a multidisciplinary group of researchers sharing common interests in the generation of ultrashort optical pulses and their application to studies of ultrafast phenomena in physics, chemistry, material science, electronics, and biology. It was attended by approximately 250 participants from 20 countries and the five-day program comprises more than 200 papers. The progress of both technology and applications in the field of ultrafast processes during these last years is truly remarkable. The advent of all solid state femtosecond lasers and the extension of laser wavelengths by frequency conversion techniques provide a large variety of high-performance light sources for ultrashort pulses. With these sources ultrafast phenomena in physical, chemical and biological systems and in electronic de vi(:es are now studied extensively. Ultrafast technology is becoming one of the basic and common tools presently entering a wide variety of scientific fields not only for basic re search but also for promoting new applications in various areas. We feel that these pro ceedings vividly reflect the present status of the field.
A stretched exponential function, I(t)= A*exp[-(t/?) beta], can be used to describe these systems, where beta
The phenomenon of spin-crossover has a large impact on the physical properties of a solid material, including its colour, magnetic moment, and electrical resistance. Some materials also show a structural phase change during the transition. Several practical applications of spin-crossover materials have been demonstrated including display and memory devices, electrical and electroluminescent devices, and MRI contrast agents. Switchable liquid crystals, nanoparticles, and thin films of spin-crossover materials have also been achieved. Spin-Crossover Materials: Properties and Applications presents a comprehensivesurvey of recent developments in spin-crossover research, highlighting the multidisciplinary nature of this rapidly expanding field. Following an introductory chapter which describes the spin-crossover phenomenon and historical development of the field, the book goes on to cover a wide range of topics including Spin-crossover in mononuclear, polynuclear and polymeric complexes Structure: function relationships in molecular spin-crossover materials Charge-transfer-induced spin-transitions Reversible spin-pairing in crystalline organic radicals Spin-state switching in solution Spin-crossover compounds in multifunctional switchable materials and nanotechnology Physical and theoretical methods for studying spin-crossover materials Spin-Crossover Materials: Properties and Applications is a valuable resource for academic researchers working in the field of spin-crossover materials and topics related to crystal engineering, solid state chemistry and physics, and molecular materials. Postgraduate students will also find this book useful as a comprehensive introduction to the field.
This volume is a collection of papers presented at the Fifteenth International Conference on Ultrafast Phenomena held at the Asilomar Conference Grounds, Pacifc Grove, CA, USA, from July 31 – August 4, 2006. The Ultrafast P- nomena conferences are held every two years and provide a forum for disc- sion of the latest results in ultrafast optics and their applications in science and engineering. These meetings bring together researchers spanning several felds of science and engineering to discuss and debate the latest advances in ult- fast science. This unique forum provides a conduit for the greater dissemi- tion of the latest advances using ultrashort coherent pulses of light. More than 280 papers were presented. Signifcant progress in creating ever shorter pulses of light was reported in the attosecond range, with new applications in high harmonic generation and frequency comb metrology. Multidimensional sp- troscopy is rapidly evolving to provide new insights into quantum coherence and interactions in complex systems. Improvements in time resolved electron and x-ray diffraction provide better atomic scale perspectives on structural dynamics. These examples are but a small subset of the collected works ga- ered in this volume, which provides a valuable synopsis of the recent advances and impact of ultrafast technology in illuminating fundamental processes in physics, chemistry, and biology. There were 323 attendees at the meeting, more than one third of which were graduate and postdoctoral students. Increased s- dent attendance energized the proceedings.
Since its inception in 1966, the series of numbered volumes known as Semiconductors and Semimetals has distinguished itself through the careful selection of well-known authors, editors, and contributors. The Willardson and Beer series, as it is widely known, has succeeded in producing numerous landmark volumes and chapters. Not only did many of these volumes make an impact at the time of their publication, but they continue to be well-cited years after their original release. Recently, Professor Eicke R. Weber of the University of California at Berkeley joined as a co-editor of the series. Professor Weber, a well-known expert in the field of semiconductor materials, will further contribute to continuing the series' tradition of publishing timely, highly relevant, and long-impacting volumes. Some of the recent volumes, such as Hydrogen in Semiconductors, Imperfections in III/V Materials, Epitaxial Microstructures, High-Speed Heterostructure Devices, Oxygen in Silicon, and others promise that this tradition will be maintained and even expanded.Reflecting the truly interdisciplinary nature of the field that the series covers, the volumes in Semiconductors and Semimetals have been and will continue to be of great interest to physicists, chemists, materials scientists, and device engineers in modern industry.
Biophysics is a rapidly-evolving interdisciplinary science that applies theories and methods of the physical sciences to questions of biology. Biophysics encompasses many disciplines, including physics, chemistry, mathematics, biology, biochemistry, medicine, pharmacology, physiology, and neuroscience, and it is essential that scientists working in these varied fields are able to understand each other's research. Comprehensive Biophysics, Nine Volume Set will help bridge that communication gap. Written by a team of researchers at the forefront of their respective fields, under the guidance of Chief Editor Edward Egelman, Comprehensive Biophysics, Nine Volume Set provides definitive introductions to a broad array of topics, uniting different areas of biophysics research - from the physical techniques for studying macromolecular structure to protein folding, muscle and molecular motors, cell biophysics, bioenergetics and more. The result is this comprehensive scientific resource - a valuable tool both for helping researchers come to grips quickly with material from related biophysics fields outside their areas of expertise, and for reinforcing their existing knowledge. Biophysical research today encompasses many areas of biology. These studies do not necessarily share a unique identifying factor. This work unites the different areas of research and allows users, regardless of their background, to navigate through the most essential concepts with ease, saving them time and vastly improving their understanding The field of biophysics counts several journals that are directly and indirectly concerned with the field. There is no reference work that encompasses the entire field and unites the different areas of research through deep foundational reviews. Comprehensive Biophysics fills this vacuum, being a definitive work on biophysics. It will help users apply context to the diverse journal literature offering, and aid them in identifying areas for further research Chief Editor Edward Egelman (E-I-C, Biophysical Journal) has assembled an impressive, world-class team of Volume Editors and Contributing Authors. Each chapter has been painstakingly reviewed and checked for consistent high quality. The result is an authoritative overview which ties the literature together and provides the user with a reliable background information and citation resource
The advent of laser-based sources of ultrafast infrared pulses has extended the study of very fast molecular dynamics to the observation of processes manifested through their effects on the vibrations of molecules. In addition, non-linear infrared spectroscopic techniques make it possible to examine intra- and intermolecular interactions and how such interactions evolve on very fast time scales, but also in some instances on very slow time scales. Ultrafast Infrared Vibrational Spectroscopy is an advanced overview of the field of ultrafast infrared vibrational spectroscopy based on the scientific research of the leading figures in the field. The book discusses experimental and theoretical topics reflecting the latest accomplishments and understanding of ultrafast infrared vibrational spectroscopy. Each chapter provides background, details of methods, and explication of a topic of current research interest. Experimental and theoretical studies cover topics as diverse as the dynamics of water and the dynamics and structure of biological molecules. Methods covered include vibrational echo chemical exchange spectroscopy, IR-Raman spectroscopy, time resolved sum frequency generation, and 2D IR spectroscopy. Edited by a recognized leader in the field and with contributions from top researchers, including experimentalists and theoreticians, this book presents the latest research methods and results. It will serve as an excellent resource for those new to the field, experts in the field, and individuals who want to gain an understanding of particular methods and research topics.