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This volume constitutes the proceedings of the second symposium on Catalysis and Automotive Pollution Control. CAPoC 2 was a great success from the point of view of its scientific interest, as evidenced by the content of this book, and also from the high participation, some 260 scientists. About two-thirds of the contributors came from the industrial world, mainly the car and oil industries and catalyst manufacturers. This is ample proof that exhaust catalysis remains a major topic of interest. The first part of the book is a general introduction to the problem of automotive pollution. The second, strictly catalytic, part is devoted to fundamental and applied studies on pollution control, with emphasis on exhaust catalytic converters.
In spite of the energy crises and the recession, there has been a global, explosive growth in the amount of motor vehicles. In the past 50 years, the amount has increased from 50 to 700 million vehicles. For economical reasons they will probably continue to be used for a considerable number of years, despite the poor yield of internal combustion engines resulting in the inevitable production of some gaseous pollutants. The subsequent increase of gaseous pollutants in our atmosphere caused by exhaust gas from automobiles has enhanced the problem of the elimination of these pollutants produced by internal combustion engines. Catalysis has proven to be the best solution to lower the content of exhaust gas in pollutants.As its predecessors, CAPoC4 proved to be a suitable platform for discussing technological improvements and developments along with future perspectives and challenges. In the light of new results and further legislative regulations, the following topics were intensely discussed: *low light-off behaviour based on improved catalysts and substrate formulations *efficient adsorber systems for storage of hydrocarbon emissions *electrically heated catalyst systems ahead the main catalyst or, alternatively, close coupled catalysts (at the manifold of the engine) • lean DeNOx catalysts allowing for decomposition of NOx in the oxygen-rich exhaust of direct injection gasoline engines and high speed injection diesel engines or, alternatively, NOx trapping/reduction in a hybrid approach * collection and destruction of dry particulates or soot.There is no doubt that clean vehicle technology is a vital part of improving air quality. Challenges remain and call for technological answers. Catalytic air pollution control is still an area providing a considerable incentive for innovative work.
In June 1984 the EEC Commission proposed new standards of permissible exhaust gas from motor vehicles to be introduced in Europe; these standards were approved by the Ministers of the Environment one year later. As the control of automotive pollution is at present mainly a catalytic problem, it was decided to hold an International Symposium on the subject, and an organizing committee composed of people engaged in catalytic research in the different Belgian Universities was constituted. This was the first Symposium of its kind to be held on an international level, and the quality and scientific interest of the papers presented was exceptional. It is planned to hold a follow-up Symposium in 2 to 3 years' time.The first part of the book is a general introduction to the problem of automotive pollution. The second, properly catalytic, part is devoted to fundamental and applied studies on pollution control, with emphasis on exhaust catalytic converters.
These proceedings are based on the third of a series of symposia devoted to the use of catalysis for the depollution of exhaust gases of motor vehicles. Although catalysts have been used for this purpose for some thirty years, the subject is still very topical because of its economic impact. The increasing number of submitted, accepted and published papers amply attests to this fact.
Catalytic Air Pollution Control: Commercial Technology is the primary source for commercial catalytic air pollution control technology, offering engineers a comprehensive account of all modern catalytic technology. This Third Edition covers all the new advances in technology in automotive catalyst control technology, diesel engine catalyst control technology, small engine catalyst control technology, and alternate sustainable fuels for auto and diesel.
New and Future Developments in Catalysis is a package of seven books that compile the latest ideas concerning alternate and renewable energy sources and the role that catalysis plays in converting new renewable feedstock into biofuels and biochemicals. Both homogeneous and heterogeneous catalysts and catalytic processes will be discussed in a unified and comprehensive approach. There will be extensive cross-referencing within all volumes.The various sources of environmental pollution are the theme of this volume. The volume lists all current environmentally friendly catalytic chemical processes used for environmental remediation and critically compares their economic viability. - Offers in-depth coverage of all catalytic topics of current interest and outlines future challenges and research areas - A clear and visual description of all parameters and conditions, enabling the reader to draw conclusions for a particular case - Outlines the catalytic processes applicable to energy generation and design of green processes
Plasma catalysis is gaining increasing interest for various gas conversion applications, such as CO2 conversion into value-added chemicals and fuels, N2 fixation for the synthesis of NH3 or NOx, methane conversion into higher hydrocarbons or oxygenates. It is also widely used for air pollution control (e.g., VOC remediation). Plasma catalysis allows thermodynamically difficult reactions to proceed at ambient pressure and temperature, due to activation of the gas molecules by energetic electrons created in the plasma. However, plasma is very reactive but not selective, and thus a catalyst is needed to improve the selectivity. In spite of the growing interest in plasma catalysis, the underlying mechanisms of the (possible) synergy between plasma and catalyst are not yet fully understood. Indeed, plasma catalysis is quite complicated, as the plasma will affect the catalyst and vice versa. Moreover, due to the reactive plasma environment, the most suitable catalysts will probably be different from thermal catalysts. More research is needed to better understand the plasma–catalyst interactions, in order to further improve the applications.
In spite of the energy crises and the recession, there has been a global, explosive growth in the amount of motor vehicles. In the past 50 years, the amount has increased from 50 to 700 million vehicles. For economical reasons they will probably continue to be used for a considerable number of years, despite the poor yield of internal combustion engines resulting in the inevitable production of some gaseous pollutants. The subsequent increase of gaseous pollutants in our atmosphere caused by exhaust gas from automobiles has enhanced the problem of the elimination of these pollutants produced by internal combustion engines. Catalysis has proven to be the best solution to lower the content of exhaust gas in pollutants. As its predecessors, CAPoC4 proved to be a suitable platform for discussing technological improvements and developments along with future perspectives and challenges. In the light of new results and further legislative regulations, the following topics were intensely discussed: *low light-off behaviour based on improved catalysts and substrate formulations*efficient adsorber systems for storage of hydrocarbon emissions*electrically heated catalyst systems ahead the main catalyst or, alternatively, close coupled catalysts (at the manifold of the engine). lean DeNOx catalysts allowing for decomposition of NOx in the oxygen-rich exhaust of direct injection gasoline engines and high speed injection diesel engines or, alternatively, NOx trapping/reduction in a hybrid approach* collection and destruction of dry particulates or soot. There is no doubt that clean vehicle technology is a vital part of improving air quality. Challenges remain and call for technological answers. Catalytic air pollution control is still an area providing a considerable incentive for innovative work.
The use of catalytic converters for the purification of automotive exhaust gases is a relatively new technology which was brought into existence by social pressures for the preservation of acceptable environmental conditions. The majority of catalytic practitioners have been able to watch the growth of this technology from its inception to its current state of sophistication. Automotive catalytic converter technology is now in a mature state, and this chapter from Vol. 5 Catalysis: Science and Technology by Dr. K. C. Taylor provides a review which covers both the process chemistry and the most important converter design factors. Contents 1. Introduction. . . . . . . . . . . . . . 2. Emission Regulations in the United States. 3. Exhaust Emission Characteristics. . 3 4. 1981 Emission Control Technology. 5 A. Converters. . . 5 B. Control System. 7 8 ~. Catalyst Screening . 6. Laboratory Testing. .10 7. The Chemical Reactions 13 8. Composition of Three-Way Catalysts. 16 A. Rhodium 17 21 B. Platinum. C. Palladium 22 D. Iridium . 22 23 E. Ruthenium and Nickel. F. Cerium Oxide ..... 23 G. Search for Alternatives to Nohle Metals 24 9. Catalyst Supports . 25 A. Pellets .... 26 B. Monoliths . . 26 10. The Transient Behavior of Three-Way Catalysts 27 II. Deterioration of Three-Way Catalysts. 35 A. Thermal Effects. . . . 35 B. Phosphorus Poisoning. . . 37 C. Lead Poisoning. . . . . . · 38 D. Catalyst Poisoning by Sulfur · 40 12. The 0.4 NO,; Research Objective. · 41 13. Control of Diesel Particulate Emissions.
Introduces major catalytic processes including products from the petroleum, chemical, environmental and alternative energy industries Provides an easy to read description of the fundamentals of catalysis and some of the major catalytic industrial processes used today Offers a rationale for process designs based on kinetics and thermodynamics Alternative energy topics include the hydrogen economy, fuels cells, bio catalytic (enzymes) production of ethanol fuel from corn and biodiesel from vegetable oils Problem sets of included with answers available to faculty who use the book Review: "In less than 300 pages, it serves as an excellent introduction to these subjects whether for advanced students or those seeking to learn more about these subjects on their own time...Particularly useful are the succinct summaries throughout the book...excellent detail in the table of contents, a detailed index, key references at the end of each chapter, and challenging classroom questions..." (GlobalCatalysis.com, May 2016)