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The swelling of uranium and of a few selected uranium alloys on post-irradiation annealing was investigated by utilizing density measurements in conjunction with the observation of pores in the microstructures of annealed specimens. Specimens were irradiated to about 0.3 at.% burnup in a constrained condition at approximately 275 deg C and were subsequently pulse annealed. The amount of swelling was found to be less than 1% for U specimens that were pulse annealed up to 75 hr at temperatures below 550 deg C; the amount of swelling, however, increased considerably on annealing at temperatures between 550 and 650 deg C. Specimens pulse annealed up to 75 hr at 618 deg C decreased in density by approximately 18%. The swelling was accompanied by the formation of bubbles on grain boundaries in recrystallized regions. The observations suggest that recrystallization is a necessary prerequisite for pronounced swelling in the alpha phase.
The Metallurgy of Nuclear Fuel: Properties and Principles of the Technology of Uranium, Thorium and Plutonium is a systematic analysis of the metallurgy of nuclear fuel, with emphasis on the physical, mechanical, and chemical properties as well as the technology of uranium, thorium, and plutonium, together with their alloys and compounds. The minerals and raw material sources of nuclear fuel are discussed, along with the principles of the technology of the raw material processing and the production of the principal compounds, and of the pure metals and alloys. Comprised of three parts, this volume begins with an introduction to the history of the discovery of uranium and its position in the periodic system; its use as a nuclear fuel; radioactivity and isotopic composition; alloys and compounds; and physical, mechanical, and chemical properties. The effect of mechanical and thermal treatment, thermal cycling and irradiation on the physicochemical properties of uranium is also examined. The next two sections are devoted to thorium and plutonium and includes chapters dealing with their uses, alloys and compounds, and methods of recovery and purification. This book is written for university students, but should also prove useful to young production engineers and scientific workers who are concerned with problems in the metallurgy of nuclear fuel.