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Atmospheric aerosols play a major role in regional atmospheric chemistry and air quality, while on a global scale, aerosol processes continue to represent the largest source of uncertainty related to climate change. An important aspect of understanding the role of aerosols in these areas is to document the vertical exchange of aerosols with the surface in both urban and rural landscapes since the vertical exchange represents important sources and sinks of aerosols on regional and global scales. In this dissertation, investigation of aerosol dynamics is described for three separate field studies. First, urban eddy covariance flux measurements were made from a building rooftop in Mexico City using a quadrupole aerosol mass spectrometer (Q-AMS) to determine the fluxes of aerosol species to/from the urban landscape. Second, conditional sampling of fine particles in updrafts and downdrafts was performed above a pine forest in Colorado using a thermal desorption chemical ionization mass spectrometer (TD-CIMS) to investigate the relative strengths of sources and sinks for speciated aerosol in a forest environment. Third, the aerosol and gas phase pollutant patterns, measured in Boise, ID during wintertime inversion conditions, were analyzed with respect to the daily evolution of the planetary boundary layer depth and surface meteorological conditions. This dissertation describes the methods used for each of the three studies and summarizes the analysis of the results.
Aerosol and clouds play important roles in determining the earth's climate, in ways that we are only beginning to comprehend. In conjunction with molecular scattering from gases, aerosol and clouds determine in part what fraction of solar radiation reaches the earth's surface, and what fraction of the longwave radiation from the earth escapes to space. This book provides an overview of the latest research on atmospheric aerosol and clouds and their effects on global climate. Subjects reviewed include the direct and indirect effects of aerosol on climate, the radiative properties of clouds and their effects on the Earth's radiation balance, the incorporation of cloud effects in numerical weather prediction models, and stratospheric aerosol and clouds.
Remote Sensing of Aerosols, Clouds, and Precipitation compiles recent advances in aerosol, cloud, and precipitation remote sensing from new satellite observations. The book examines a wide range of measurements from microwave (both active and passive), visible, and infrared portions of the spectrum. Contributors are experts conducting state-of-the-art research in atmospheric remote sensing using space, airborne, and ground-based datasets, focusing on supporting earth observation satellite missions for aerosol, cloud, and precipitation studies. A handy reference for scientists working in remote sensing, earth science, electromagnetics, climate physics, and space engineering. Valuable for operational forecasters, meteorologists, geospatial experts, modelers, and policymakers alike. - Presents new approaches in the field, along with further research opportunities, based on the latest satellite data - Focuses on how remote sensing systems can be designed/developed to solve outstanding problems in earth and atmospheric sciences - Edited by a dynamic team of editors with a mixture of highly skilled and qualified authors offering world-leading expertise in the field
Life on Earth is critically dependent upon the continuous cycling of water between oceans, continents and the atmosphere. Precipitation (including rain, snow, and hail) is the primary mechanism for transporting water from the atmosphere back to the Earth’s surface. It is also the key physical process that links aspects of climate, weather, and the global hydrological cycle. Changes in precipitation regimes and the frequency of extreme weather events, such as floods, droughts, severe ice/snow storms, monsoon fluctuations and hurricanes are of great potential importance to life on the planet. One of the factors that could contribute to precipitation modification is aerosol pollution from various sources such as urban air pollution and biomass burning. Natural and anthropogenic changes in atmospheric aerosols might have important implications for precipitation by influencing the hydrological cycle, which in turn could feed back to climate changes. From an Earth Science perspective, a key question is how changes expected in climate will translate into changes in the hydrological cycle, and what trends may be expected in the future. We require a much better understanding and hence predictive capability of the moisture and energy storages and exchanges among the Earth’s atmosphere, oceans, continents and biological systems. This book is a review of our knowledge of the relationship between aerosols and precipitation reaching the Earth's surface and it includes a list of recommendations that could help to advance our knowledge in this area.
The oceans and atmosphere interact through various processes, including the transfer of momentum, heat, gases and particles. In this book leading international experts come together to provide a state-of-the-art account of these exchanges and their role in the Earth-system, with particular focus on gases and particles. Chapters in the book cover: i) the ocean-atmosphere exchange of short-lived trace gases; ii) mechanisms and models of interfacial exchange (including transfer velocity parameterisations); iii) ocean-atmosphere exchange of the greenhouse gases carbon dioxide, methane and nitrous oxide; iv) ocean atmosphere exchange of particles and v) current and future data collection and synthesis efforts. The scope of the book extends to the biogeochemical responses to emitted / deposited material and interactions and feedbacks in the wider Earth-system context. This work constitutes a highly detailed synthesis and reference; of interest to higher-level university students (Masters, PhD) and researchers in ocean-atmosphere interactions and related fields (Earth-system science, marine / atmospheric biogeochemistry / climate). Production of this book was supported and funded by the EU COST Action 735 and coordinated by the International SOLAS (Surface Ocean- Lower Atmosphere Study) project office.
This dissertation investigates the modulating effects of land-atmosphere and aerosol interactions on meso-scale convective systems across the sub-Saharan West Africa region, and aims at providing a value-added contribution towards better understanding of the controlling mechanisms for these interactions, in order to improve predictability of the highly frequent, high-impact meso-scale convective systems. It is very well known that aerosols alter the surface energy budget resulting into complex and multi-scale interactions between the land-atmosphere and mesoscale convective systems, which are yet to be fully understood. In this study, we used a highly proven successful cognitive recognition artificial neural network intelligence problem solving tool -- Self-Organizing Maps (SOM) in investigating the modulating effects of aerosol-land-atmosphere interactions for enhancing the predictability of meso-scale convective systems. The SOM method is not yet commonly used by climate scientists for solving climate research problems. For the first time in this research -- at least to the best of our knowledge -- we used the SOM method to solve climate research problems over Africa. Our results show very strong seasonal influence in determining the dominant controlling variable (e.g. soil moisture, aerosols) on the interactions between atmospheric aerosols, meso-scale convective systems and land-surface properties across the study region. It was also found that these controlling variables are generally very significant in modulating atmospheric interactions across the region during the monsoon (wet) seasons than during the nonmonsoon (dry) seasons. Furthermore, results showed that even though there is noticeable control by aerosols on the interactions between land-atmosphere and meso-scale convective systems, available surface soil moisture exerts the most dominant control across the region especially during the active convective period (monsoon season) of the year. Results further showed that soil moisture has the potential to control the convective available potential energy (CAPE) up to about 79% during the monsoon season and up to about 67% during the non-monsoon seasons, while aerosols can control CAPE up to about 67% during monsoon and up to about 23% during the non-monsoon season.
The ever-diversifying field of aerosol effects on climate is comprehensively presented here, describing the strong connection between fundamental research and model applications in a way that will allow both experienced researchers and those new to the field to gain an understanding of a wide range of topics. The material is consistently presented at three levels for each topic: (i) an accessible "quick read" of the essentials, (ii) a more detailed description, and (iii) a section dedicated to how the processes are handled in models. The modelling section in each chapter summarizes the current level of knowledge and what the gaps in this understanding mean for the effects of aerosols on climate, enabling readers to quickly understand how new research fits into established knowledge. Definitions, case studies, reference data, and examples are included throughout. Aerosols and Climate is a vital resource for graduate students, postdoctoral researchers, senior researchers, and lecturers in departments of atmospheric science, meteorology, engineering, and environment. It will also be of interest to those working in operational centers and policy-facing organizations, providing strong reference material on the current state of knowledge. - Includes a section in each chapter that focuses on the treatment of relevant aerosol processes in climate models - Provides clear exposition of the challenges in understanding and reducing persistent gaps in knowledge and uncertainties in the field of aerosol-climate interaction, going beyond the fundamentals and existing knowledge - Authored by experts in modeling and aerosol processes, analysis or observations to ensure accessibility and balance
The book is divided into two sections. The first section presents characterization of atmospheric aerosols and their impact on regional climate from East Asia to the Pacific. Ground-based, air-born, and satellite data were collected and analyzed. Detailed information about measurement techniques and atmospheric conditions were provided as well. In the second section, authors provide detailed information about the organic and inorganic constituents of atmospheric aerosols. They discuss the chemical and physical processes, temporal and spatial distribution, emissions, formation, and transportation of aerosol particles. In addition, new measurement techniques are introduced. This book hopes to serve as a useful resource to resolve some of the issues associated with the complex nature of the interaction between atmospheric aerosols and climatology.
This book recommends the initiation of an "integrated" research program to study the role of aerosols in the predicted global climate change. Current understanding suggest that, even now, aerosols, primarily from anthropogenic sources, may be reducing the rate of warming caused by greenhouse gas emissions. In addition to specific research recommendations, this book forcefully argues for two kinds of research program integration: integration of the individual laboratory, field, and theoretical research activities and an integrated management structure that involves all of the concerned federal agencies.
Contained in this volume are the deliberations of the Experts Meeting on Interaction Between Clouds and Aerosols, held in Hampton, Virginia, 5-7 February 1991. Eight invited experts from universities, nonprofit institutions, research laboratories, and government agencies in France and the United States of America participated in the Meeting. Some of those who could not participate sent in their comments. The purpose of the Meeting was to bring together experts in measurements and impacts of interactions between clouds and aerosols to assess the current state of the art, and to make recommendations ofr developing a coordinated action plan for future work in these aspects of the International Global Aerosol Program (IGAP).--Preface.