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The goal of this book is to provide a simple and conceptually intuitive introduction to nonlinear spectroscopy via the formalism of quantum processes and wavepacket dynamics.
The recent improvements in the techniques for producing very short duration pulses of laser light have allowed chemists to study processes taking place on similarly short timescales, now typically in the range of 10 to 10 seconds. This book describes methods for generating and characterising picosecond pulses, and then provides a discussion of current experimental techniques for the study of ultrafast chemical processes. The applications to specific chemical problems are divided into chapters on the vapour, liquid, and solid phases.
The embryonic development of femtoscience stems from advances made in the generation of ultrashort laser pulses. Beginning with mode-locking of glass lasers in the 1960s, the development of dye lasers brought the pulse width down from picoseconds to femtoseconds. The breakthrough in solid state laser pulse generation provided the current reliable table-top laser systems capable of average power of about 1 watt, and peak power density of easily watts per square centimeter, with pulse widths in the range of four to eight femtoseconds. Pulses with peak power density reaching watts per square centimeter have been achieved in laboratory settings and, more recently, pulses of sub-femtosecond duration have been successfully generated. As concepts and methodologies have evolved over the past two decades, the realm of ultrafast science has become vast and exciting and has impacted many areas of chemistry, biology and physics, and other fields such as materials science, electrical engineering, and optical communication. In molecular science the explosive growth of this research is for fundamental reasons. In femtochemistry and femtobiology chemical bonds form and break on the femtosecond time scale, and on this scale of time we can freeze the transition states at configurations never before seen. Even for n- reactive physical changes one is observing the most elementary of molecular processes. On a time scale shorter than the vibrational and rotational periods the ensemble behaves coherently as a single-molecule trajectory.
The advent of laser-based sources of ultrafast infrared pulses has extended the study of very fast molecular dynamics to the observation of processes manifested through their effects on the vibrations of molecules. In addition, non-linear infrared spectroscopic techniques make it possible to examine intra- and intermolecular interactions and how such interactions evolve on very fast time scales, but also in some instances on very slow time scales. Ultrafast Infrared Vibrational Spectroscopy is an advanced overview of the field of ultrafast infrared vibrational spectroscopy based on the scientific research of the leading figures in the field. The book discusses experimental and theoretical topics reflecting the latest accomplishments and understanding of ultrafast infrared vibrational spectroscopy. Each chapter provides background, details of methods, and explication of a topic of current research interest. Experimental and theoretical studies cover topics as diverse as the dynamics of water and the dynamics and structure of biological molecules. Methods covered include vibrational echo chemical exchange spectroscopy, IR-Raman spectroscopy, time resolved sum frequency generation, and 2D IR spectroscopy. Edited by a recognized leader in the field and with contributions from top researchers, including experimentalists and theoreticians, this book presents the latest research methods and results. It will serve as an excellent resource for those new to the field, experts in the field, and individuals who want to gain an understanding of particular methods and research topics.
The primary goal of this text book is to ensure that any physical science student, even one who has never heard of the subject, should be able to learn what ultrafast spectroscopy is, why optics related to the subject requires special attention, how to use the basic ideas of the subject in laboratory-based ultrafast spectroscopy experiments, how to interpret the experimental observations and so on. This book gives a more than adequate introduction to mathematical representation of an ultrafast pulse, chirp, time-band width product, nonlinear optical effects, dispersion effects, construction of ultrafast laser, ultrafast measurement techniques and different ultrafast processes of chemical interest.
A comprehensive treatment of ultrafast optics This book fills the need for a thorough and detailed account of ultrafast optics. Written by one of the most preeminent researchers in the field, it sheds new light on technology that has already had a revolutionary impact on precision frequency metrology, high-speed electrical testing, biomedical imaging, and in revealing the initial steps in chemical reactions. Ultrafast Optics begins with a summary of ultrashort laser pulses and their practical applications in a range of real-world settings. Next, it reviews important background material, including an introduction to Fourier series and Fourier transforms, and goes on to cover: Principles of mode-locking Ultrafast pulse measurement methods Dispersion and dispersion compensation Ultrafast nonlinear optics: second order Ultrafast nonlinear optics: third order Mode-locking: selected advanced topics Manipulation of ultrashort pulses Ultrafast time-resolved spectroscopy Terahertz time-domain electromagnetics Professor Weiner's expertise and cutting-edge research result in a book that is destined to become a seminal text for engineers, researchers, and graduate students alike.
SPECTROSCOPY FOR MATERIALS CHARACTERIZATION Learn foundational and advanced spectroscopy techniques from leading researchers in physics, chemistry, surface science, and nanoscience In Spectroscopy for Materials Characterization, accomplished researcher Simonpietro Agnello delivers a practical and accessible compilation of various spectroscopy techniques taught and used to today. The book offers a wide-ranging approach taught by leading researchers working in physics, chemistry, surface science, and nanoscience. It is ideal for both new students and advanced researchers studying and working with spectroscopy. Topics such as confocal and two photon spectroscopy, as well as infrared absorption and Raman and micro-Raman spectroscopy, are discussed, as are thermally stimulated luminescence and spectroscopic studies of radiation effects on optical materials. Each chapter includes a basic introduction to the theory necessary to understand a specific technique, details about the characteristic instrumental features and apparatuses used, including tips for the appropriate arrangement of a typical experiment, and a reproducible case study that shows the discussed techniques used in a real laboratory. Readers will benefit from the inclusion of: Complete and practical case studies at the conclusion of each chapter to highlight the concepts and techniques discussed in the material Citations of additional resources ideal for further study A thorough introduction to the basic aspects of radiation matter interaction in the visible-ultraviolet range and the fundamentals of absorption and emission A rigorous exploration of time resolved spectroscopy at the nanosecond and femtosecond intervals Perfect for Master and Ph.D. students and researchers in physics, chemistry, engineering, and biology, Spectroscopy for Materials Characterization will also earn a place in the libraries of materials science researchers and students seeking a one-stop reference to basic and advanced spectroscopy techniques.
Ultrafast spectroscopy of semiconductors and semiconductor nanostructures is currently one of the most exciting areas of research in condensed-matter physics. Remarkable recent progress in the generation of tunable femtosecond pulses has allowed direct investigation of the most fundamental dynamical processes in semiconductors. This second edition presents the most striking recent advances in the techniques of ultrashort pulse generation and ultrafast spectroscopy; it discusses the physics of relaxation, tunneling and transport dynamics in semiconductors and semiconductor nanostructures following excitation by femtosecond laser pulses.
This book provides fundamental knowledge in the fields of attosecond science and free electron lasers, based on the insight that the further development of both disciplines can greatly benefit from mutual exposure and interaction between the two communities. With respect to the interaction of high intensity lasers with matter, it covers ultrafast lasers, high-harmonic generation, attosecond pulse generation and characterization. Other chapters review strong-field physics, free electron lasers and experimental instrumentation. Written in an easy accessible style, the book is aimed at graduate and postgraduate students so as to support the scientific training of early stage researchers in this emerging field. Special emphasis is placed on the practical approach of building experiments, allowing young researchers to develop a wide range of scientific skills in order to accelerate the development of spectroscopic techniques and their implementation in scientific experiments. The editors are managers of a research network devoted to the education of young scientists, and this book idea is based on a summer school organized by the ATTOFEL network.
This is the second edition of this advanced textbook written for scientists who require further training in femtosecond science. Four years after pub- cation of the ?rst edition, femtosecond science has overcome new challenges and new application ?elds have become mature. It is necessary to take into account these new developments. Two main topics merged during this period that support important scienti?c activities: attosecond pulses are now gen- ated in the X-UV spectral domain, and coherent control of chemical events is now possible by tailoring the shape of femtosecond pulses. To update this advanced textbook, it was necessary to introduce these ?elds; two new ch- ters are in this second edition: “Coherent Control in Atoms, Molecules, and Solids”(Chap.11)and“AttosecondPulses”(Chap.12)withwell-documented references. Some changes, addenda, and new references are introduced in the ?rst edition’s ten original chapters to take into account new developments and updatethisadvancedtextbookwhichistheresultofascienti?cadventurethat started in 1991. At that time, the French Ministry of Education decided that, in view of the growing importance of ultrashort laser pulses for the national scienti?c community, a Femtosecond Centre should be created in France and devoted to the further education of scientists who use femtosecond pulses as a research tool and who are not specialists in lasers or even in optics.