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Applying a unified quantum approach, contributors offer fresh insights into the theoretical developments in the excitation energy transfer processes in condensed matter. This comprehensive volume examines Frenkel and Wannier excitonic processes; rates of excitonic processes; theory of laser sputter and polymer ablation; and polarons, excitonic polarons and self-trapping.
Provides a semi-quantitative approach to recent developments in the study of optical properties of condensed matter systems Featuring contributions by noted experts in the field of electronic and optoelectronic materials and photonics, this book looks at the optical properties of materials as well as their physical processes and various classes. Taking a semi-quantitative approach to the subject, it presents a summary of the basic concepts, reviews recent developments in the study of optical properties of materials and offers many examples and applications. Optical Properties of Materials and Their Applications, 2nd Edition starts by identifying the processes that should be described in detail and follows with the relevant classes of materials. In addition to featuring four new chapters on optoelectronic properties of organic semiconductors, recent advances in electroluminescence, perovskites, and ellipsometry, the book covers: optical properties of disordered condensed matter and glasses; concept of excitons; photoluminescence, photoinduced changes, and electroluminescence in noncrystalline semiconductors; and photoinduced bond breaking and volume change in chalcogenide glasses. Also included are chapters on: nonlinear optical properties of photonic glasses; kinetics of the persistent photoconductivity in crystalline III-V semiconductors; and transparent white OLEDs. In addition, readers will learn about excitonic processes in quantum wells; optoelectronic properties and applications of quantum dots; and more. Covers all of the fundamentals and applications of optical properties of materials Includes theory, experimental techniques, and current and developing applications Includes four new chapters on optoelectronic properties of organic semiconductors, recent advances in electroluminescence, perovskites, and ellipsometry Appropriate for materials scientists, chemists, physicists and electrical engineers involved in development of electronic materials Written by internationally respected professionals working in physics and electrical engineering departments and government laboratories Optical Properties of Materials and Their Applications, 2nd Edition is an ideal book for senior undergraduate and postgraduate students, and teaching and research professionals in the fields of physics, chemistry, chemical engineering, materials science, and materials engineering.
Physical Processes in Radiation Biology covers the proceedings of an International Symposium on Physical Processes in Radiation Biology, held at the Kellogg Center for Continuing Education, Michigan State University on May 6-8, 1963, sponsored by the U.S. Atomic Energy Commission. The symposium aims to address the core problems of radiation biology concerning the absorption, distribution, and utilization of high energy packets in biological systems. This book is composed of 21 chapters, and begins with an introduction to the absorption, excitation, and transfer processes in molecular solids. The subsequent chapters discuss the nature of exciton processes; the mechanisms of charge transport in biological materials; the interactions of fast and slow electrons with model systems; the importance of liquid structures in determining the development of radiation damage; and the nature of the metastable species formed. The concluding chapters explore the importance of charge migration in energy transfer processes in different biological systems and the significance of higher excited levels in charge migration and energy transfer. These chapters also describe the nature of the hydration of electrons and protons in aqueous systems. This book will be of great value to radiation biologists, biophysicists, physical chemists, and physicists.
Dynamics of Molecular Excitons provides a comprehensive, but concise description of major theories on the dynamics of molecular excitons, intended to serve as a self-contained resource on the topic. Designed to help those new to this area gain proficiency in this field, experts will also find the book useful in developing a deeper understanding of the subject. The starting point of the book is the standard microscopic definition of molecular Hamiltonians presented in commonly accepted modern quantum mechanical notations. Major assumptions and approximations involved in constructing Frenkel-type exciton Hamiltonians, which are well established, but are often hidden under arcane notations and approximations of old publications, are presented in detail. This will help quantum chemists understand the major assumptions involved in the definition of commonly used exciton models. Rate theories of exciton dynamics, such as Förster and Dexter theories and their modern generalizations, are presented in a unified and detailed manner. In addition, important aspects that are often neglected, such as local field effect and the role of fluctuating environments, are discussed. Various quantum dynamics methods allowing coherent dynamics of excitons are presented in a systematic manner in the context of quantum master equations or path integral formalisms. The author also provides a detailed theoretical explanation for the major spectroscopic techniques probing exciton dynamics, including modern two-dimensional electronic spectroscopy, with a critical assessment of the implications of these spectroscopic measurements. Finally, the book includes a brief overview of major applications including an explanation of organic photovoltaic materials and natural light harvesting complexes. - Covers major theories of exciton dynamics in a consciously concise and easily readable way - Bridges the gap between quantum dynamics working with phenomenological exciton Hamiltonian and quantum chemistry construct reliable models amenable for dynamics calculations from ab initio calculations - Explores modern nonlinear electronic spectroscopy techniques to probe exciton dynamics, showing how it is applied
This work brings together quantum theory and spectroscopy to convey excitation processes to advanced students and specialists wishing to conduct research and understand the entire fi eld rather than just single aspects. Written by experienced authors and recognized authorities in the field, this text covers numerous applications and offers examples taken from different disciplines. As a result, spectroscopists, molecular physicists, physical chemists, and biophysicists will all fi nd this a must-have for their research. Also suitable as supplementary reading in graduate level courses.
This volume concentrates on the controversy within the scientific community over how to explain, understand and describe the photophysics/photochemistry of this class of materials.This controvery is of such a fundamental nature that the solution of the problem might be in a unification of the semiconductor and metal physics with the molecular quantum chemistry. Thus, a wide-ranging and comprehensive discussion of this very crucial issue has not been written down yet.This volume brings together the most prominent scientists specializing in this controversial topic. Each contributor addresses the opponents' arguments. After short introductory chapters, the contributors discuss their own speciality area and compare the results with both models and explain their position on why one of the models is more appropriate. Special emphasis is given to comparative discussions with other conjugated molecular systems as well as inorganic semiconductors.
At Yamada Conference LIII, papers on many novel materials and on novel phenomena in condensed matter physics were presented OCo for instance, the achievement of simultaneous creation of excitons and free-electron-hole pairs in rare gas solids, and a low frequency fluctuation of the spectral shift of indirect excitons in GaAs coupled quantum wells. Single molecule spectroscopy is a powerful tool for studying molecules including biological systems; the study of delocalization of excitons in the photosynthetic light harvesting antenna system was also reported. The proceedings thus contain many excellent papers dealing with current research topics on the excitonic processes in bulk, quantum wells, quantum dots and other confined systems. This book will serve as an excellent source of recent references and reviews for a wide range of researchers in physics, chemistry, engineering and biological sciences. The proceedings have been selected for coverage in: . OCo Index to Scientific & Technical Proceedings (ISTP CDROM version / ISI Proceedings). Contents: Dynamical Process of Photoionization in Semiconductor Nanocrystals (M Y Shen et al.); Excitons on a 1D Periodic Conjugated Polymer Chain: Two Electronic Structures of Polydiacetylene Chains (C Lapersonne-Meyer); Anomalous Spectral Shifts of Indirect Excitons in Coupled GaAs Quantum Wells (D W Snoke et al.); Infrared Absorption by Excitons in Cuprous Oxide (M GAppert et al.); Theory of Excitation-Energy Transfer Processes Involving Optically Forbidden Exciton States in Antenna Systems of Photosynthesis (K Mukai et al.); Transient Grating Induced by Excitonic Polaritons in Thin Film Semiconductors (K Akiyama et al.); Excitonic Photoluminescence of Pentacene Single Crystal (T Aoki-Matsumoto et al.); Scanning Near-Field Optical Microspectroscopy of Single Perylene Microcrystals (J Niitsuma et al.); and other papers. Readership: Condensed matter physicists, materials scientists, chemists and biologists."
At Yamada Conference LIII, papers on many novel materials and on novel phenomena in condensed matter physics were presented — for instance, the achievement of simultaneous creation of excitons and free-electron-hole pairs in rare gas solids, and a low frequency fluctuation of the spectral shift of indirect excitons in GaAs coupled quantum wells. Single molecule spectroscopy is a powerful tool for studying molecules including biological systems; the study of delocalization of excitons in the photosynthetic light harvesting antenna system was also reported. The proceedings thus contain many excellent papers dealing with current research topics on the excitonic processes in bulk, quantum wells, quantum dots and other confined systems. This book will serve as an excellent source of recent references and reviews for a wide range of researchers in physics, chemistry, engineering and biological sciences.The proceedings have been selected for coverage in:• Index to Scientific & Technical Proceedings (ISTP CDROM version / ISI Proceedings)