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In this study, by applying a salt metathesis approach between Ce(OtBu3)2(NO3)2(THF)2 and the potassium salts of mono- and ditrimethylsilyl substituted cyclopentadienes, we were able to isolate two new Ce(IV) metallocenes, including to the best of our knowledge, the first structurally characterized bis-cyclopentadiene Ce(IV) compound.
Lanthanides: Fundamentals and Applications provides the fundamentals, new research, promising applications and future outlooks of lanthanide compounds and lanthanide-based materials. The book begins with an introduction, including key concepts, oxidation states and sources, extraction and separation of the lanthanides, followed by spectroscopic and magnetic properties, and metals, crystals and compounds. Organometallic compounds, coordination compounds, molecular magnetic materials and luminescent materials are covered before a discussion of specific lanthanide applications. Spintronics, bioimaging, photoelectric materials, catalysis and nuclear applications are discussed. This comprehensive resource is ideal for researchers and students studying inorganic and materials chemistry, in both academia and industry. Includes comprehensive and in-depth coverage of lanthanides Features the most current research progress on lanthanides Covers a combination view of fundamental research and specific applications of the lanthanides, including spintronics, bioimaging and additives for photoelectric materials
The f-elements and their compounds often possess an unusually complex electronic structure, governed by the high number of electronic states arising from open f-shells as well as large relativistic and electron correlation effects. A correct theoretical description of these elements poses the highest challenges to theory. Computational Methods in Lanthanide and Actinide Chemistry summarizes state-of-the-art electronic structure methods applicable for quantum chemical calculations of lanthanide and actinide systems and presents a broad overview of their most recent applications to atoms, molecules and solids. The book contains sixteen chapters, written by leading experts in method development as well as in theoretical investigations of f-element systems. Topics covered include: Relativistic configuration interaction calculations for lanthanide and actinide anions Study of actinides by relativistic coupled cluster methods Relativistic all-electron approaches to the study of f- element chemistry Relativistic pseudopotentials and their applications Gaussian basis sets for lanthanide and actinide elements Applied computational actinide chemistry This book will serve as a comprehensive reference work for quantum chemists and computational chemists, both those already working in, and those planning to enter the field of quantum chemistry for f-elements. Experimentalists will also find important information concerning the capabilities of modern quantum chemical methods to assist in the interpretation or even to predict the outcome of their experiments.
Almost all branches of chemistry and material science now interface with organometallic chemistry--the study of compounds containing carbon-metal bonds. This widely acclaimed serial contains authoritative reviews that address all aspects of organometallic chemistry, a field that has expanded enormously since the publication of Volume 1 in 1964. Informs and updates on all the latest developments in the field Contributions from leading authorities and industry experts