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Superionic conductors are solids whose ionic conductivities approach, and in some cases exceed, those of molten salts and electrolyte solutions. This implies an un usual state of matter in which some atoms have nearly liquidlike mobility while others retain their regular crystalline arrangement. This liquid-solid duality has much appeal to condensed matter physicists, and the coincident development of powerful new methods for studying disordered solids and interest in superionic conductors for technical applications has resulted in a new surge of activity in this venerable field. It is the purpose of this book to summarize the current re search in the physics of superionic conduction. with special emphasis on those aspects which set these materials apart from other solids. The volume is aimed to wards the materials community and will, we expect, stimulate further research on these potentially useful substances. The usual characterization of the superionic phase lists high ionic conductivity; low activation energy; and the open structure of the crystal, with its interconne ted network of vacant sites available to one ionic species. To these, as we demon strate in this volume, should be added important dynami~ and collective effect~: the absence of well-defined optical lattice modes, the presence of a pervasive, low-energy excitation, an infrared peak in the frequency-dependent conductivity, unusual NMR prefactors, phase transitions, and a strong tendency for the mobile ion to be found between allowed sites.
The book presents basic studies on ion transport properties of ionic conductive solid. It describes research on theory, modeling, simulation, crystalline structure, nuclear magnetic resonance, electric conduction, optical properties, and thermal measurement in this field. Superionic conductors are highly promising functional materials. As a stepping stone in the development of new superionic conductors that can be utilized as functinal materials efforts to reevaluate solid-interior diffusion and conduction phenomena of ions and molecules in a superionic conductor on the basis of basic physical properties, and to clarify mechanism governing these phenomena from a microscopic standpoint are important.How are diffusing ions associated with material structures within a superionic conductor? What types of interaction are diffusing ions undergoing with the host ions surrounding them? How important is the correlation among diffusing ions in their motion? The carefully presented detail of this book will be of value to research devoted to the understanding and control of functional materials such as superionic conductors.
The following chapters present most of the lectures delivered at the NATO Advanced Studies Institute on "The Physics of Super ionic Conductors and Electrode Materials", held at Odense Univer sity's Mathematics Department between the 4th and 22nd of August, 1980. The aim of the organizing committee was to present in a rather detailed fashion the most recent advances in the computa tional mathematics and physics of condensed matter physics and to see how these advances could be applied to the study of ionically conducting solids. The first half of the meeting was mainly taken up with lectures. In the second week, working groups on the various aspects were set up, the students joining these groups being helped in the implementation of the lecture material. The leaders of these groups deserve special mention for the tremendous effort they put into this aspect of the meeting, particularly: Dr. Aneesur Rahman (Molecular Dynamics group) Dr. Fred Horne (Ion Transport group) Drs. Nick Quirke and David Adams (Monte Carlo methods) Dr. Heinz Schulz (Diffraction group) Dr. John Harding (Defect Calculations group) The Molecular Dynamics group achieved a certain amount of notoriety within the University by appearing to live in the terminal room.
Introduction to Solid State Ionics: Phenomenology and Applications presents a pedagogical, graduate-level treatment of the science and technology of superionic conductors, also known as fast ion conductors or solid electrolytes. Suitable for physics, materials science, and engineering researchers and students, the text emphasizes basic physics and
In 1966, E.H. Lieb and D.C. r1attis published a book on "Mathematical Physics in One Dimension" [Academic Press, New York and London] which is much more than just a collection of reprints and which in fact marked the beginnings of the rapidly growing interest in one-dimensional problems and materials in the 1970's. In their Foreword, Lieb and r~attis made the observation that " ... there now exists a vast literature on this subject, albeit one which is not indexed under the topic "one dimension" in standard indexing journals and which is therefore hard to research ... ". Today, the situation is even worse, and we hope that these Proceedings will be a valuable guide to some of the main current areas of one-dimensional physics. From a theoretical point of view, one-dimensional problems have always been very attractive. Many non-trivial models are soluble in one dimension, while they are only approximately understood in three dimensions. Therefore, the corresponding exact solutions serve as a useful test of approximate ma thematical methods, and certain features of the one-dimensional solution re main relevant in higher dimensions. On the other hand, many important phe nomena are strongly enhanced, and many concepts show up especially clearly in one-dimensional or quasi -one-dimensional systems. Among them are the ef fects of fluctuations, of randomness, and of nonlinearity; a number of in teresting consequences are specific to one dimension.
The main motivation for the organization of the Advanced Research Workshop in Belgirate was the promotion of discussions on the most recent issues and the future perspectives in the field of Solid State lonics. The location was chosen on purpose since Belgirate was the place were twenty years ago, also then under the sponsorship of NATO, the very first international meeting on this important and interdisciplinary field took place. That meeting was named "Fast Ion Transport in Solids" and gathered virtually everybody at that time having been active in any aspect of motion of ions in solids. The original Belgirate Meeting made for the first time visible the technological potential related to the phenomenon of the fast ionic transport in solids and, accordingly, the field was given the name "Solid State lonics". This field is now expanded to cover a wide range of technologies which includes chemical sensors for environmental and process control, electrochromic windows, mirrors and displays, fuel cells, high performance rechargeable batteries for stationary applications and electrotraction, chemotronics, semiconductor ionics, water electrolysis cells for hydrogen economy and other applications. The main idea for holding an anniversary meeting was that of discussing the most recent issues and the future perspectives of Solid State lonics just twenty years after it has started at the same location on the lake Maggiore in North Italy.
Strongly Coupled Plasma Physics covers the proceedings of the 24th Yamada Conference on Strongly Coupled Plasma Physics, held from August 29 to September 2, 1989 at Hotel Mount Fuji near Lake Yamanaka on the outskirts of Tokyo. The book focuses on the reactions, technologies, interactions, and transformations of charged particles. The selection first offers information on phase transitions in dense astrophysical plasmas and plasma thermodynamics and the evolution of brown dwarfs and planets, as well as solidification of dense astrophysical plasmas, evolution of brown dwarfs, and structure of Jupiter. The text then examines the discovery of low mass objects in Taurus and topics in X-ray astronomy from observations with GINGA. The publication ponders on proton abundance in hot neutron star matter; thermonuclear reaction rates of dense carbon-oxygen mixtures in white dwarfs; and quantum simulation of superconductivity. The text also examines dynamic simulation of mixed quantum-classical systems and Monte-Carlo simulations for the surface properties of the strongly coupled one-component plasma. The selection is a dependable reference for readers interested in strongly coupled plasma physics.
Uses an integrated, scientists' approach to the principles regulating the synthesis, structure and physical characteristics of crystalline solids. Mathematical derivations are kept to a minimum. Covers electrical properties of metals and band semiconductors, superionic conductors, ferrites and solid electrolytes. Features end-of-chapter problem sets.
Charged particles in dense matter exhibit strong correlations due to the exchange and Coulomb interactions, and thus make a strongly coupled plasma. Examples in laboratory and astrophysical settings include solid and liquid metals, semiconductors, charged particles in lower dimensions such as those trapped in interfacial states of condensed matter or beams, dense multi-ionic systems such a superionic conductors and inertial-confinement-fusion plasmas . The aim of the conference was to elucidate the various physical processes involved in these dense materials. The subject areas covered include plasma physics, atomic and molecular physics, condensed matter physics and astrophysics.
This book describes, for the first time in a modern text, the fundamental principles on which solid state electrochemistry is based. In this sense it is in contrast to other books in the field which concentrate on a description of materials. Topics include solid (ceramic) electrolytes, glasses, polymer electrolytes, intercalation electrodes, interfaces and applications. The different nature of ionic conductivity in ceramic, glassy and polymer electrolytes is described as are the thermodynamics and kinetics of intercalation reactions. The interface between solid electrolytes and electrodes is discussed and contrasted with the more conventional liquid state electrochemistry. The text provides an essential foundation of understanding for postgraduates or others entering the field for the first time and will also be of value in advanced undergraduate courses.