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Supercritical CO2 (sCO2) power cycle is an up-and-coming technology to produce electricity from various heat sources. Apart from power cycles, sCO2 can also be used as coolant in centralized cooling system and stand-alone cooling device. However, lack of accurate predication tools such as heat transfer coefficient correlations and insufficient knowledge behind fundamental heat transfer processes can hinder its practical realization in key energy and cooling systems. The overall objective of the study is to extend fundamental knowledge about heat transfer and fluid flow processes in conduits pertinent to sCO2 power cycle. The emphasis here is investigation of heat transfer effects of three testing parameters: heat flux, inlet mass flux and inlet temperature. Experimental setup for this heat transfer study is designed considering limitations due to high pressure rating requirements and thus follows unconventional approach to calculate heat transfer coefficient. Test section chosen is a horizontal stainless steel tubing of inner diameter of 9.4 mm and heated length of 1.23 m with uniform volumetric heat generation within tubing walls. The designed test apparatus and data reduction process are validated with high pressure air experiments. Nusselt numbers are calculated at top, bottom and sidewall locations to demonstrate effects of buoyancy. Enhancement of heat transfer at bottom wall surfaces and deterioration at top wall surfaces is observed as the main effect of buoyancy. It was observed that effects of buoyancy increase with heat flux and decrease with mass flux. Buoyancy effects are also decreased for fluid temperatures higher than pseudocritical temperature. Nusselt numbers calculated from experimental results are compared with Nusselt number from available correlations in literature. It is hinted that near critical region where property variations are significant, one correlation alone may not accurately predict heat transfer for different regimes of geometry, mass flux and heat flux.
An experimental analysis was conducted on a single circular tube heat exchanger using supercritical carbon dioxide as the working fluid. The heat exchanger was operated in two different orientations: vertically upward and downward. The experimental facility utilized two different mass flow rates: a low flow rate of 0.0183 kg/s and a high mass flow rate 0.03 kg/s, three system pressures: 7.5, 8.1 and 10.2 MPa and two different heat inputs: a low heat input of 540 W and a high heat input of 955 W. Inlet temperatures to the test section were varied from 20-55 °C. Thermocouples on the surface of the test section recorded the wall temperatures. Then, a one dimensional heat transfer analysis was conducted to calculate inner wall temperatures. Afterwards, the bulk temperature was calculated using a constant heat flux approximation and an energy balance on a differential control volume. Finally, the local heat transfer coefficient between the bulk and inner wall was calculated. Results showed that typically, for the 7.5 and 8.1 MPa cases, as the temperature reached the pseudocritical point, there was a heat transfer deterioration followed immediately by a substantially large heat transfer enhancement. After the critical temperature was reached, however, the heat transfer coefficient decreased. The results showed that the heat transfer coefficient, deterioration and enhancement were the greatest with the 7.5 MPa case and the downward orientation. Buoyancy effects seem to be present and have a significant impact on the heat transfer coefficient. In general, if heat exchangers are to be designed to be used with supercritical fluids, they should be designed, along with other important components, to be operated as close to the critical point as possible as well as have a downward flowing orientation to maximize heat transfer potential. The electronic version of this dissertation is accessible from http://hdl.handle.net/1969.1/152835
Supercritical fluids are increasingly being used in energy conversion and fluid dynamics studies for energy-related systems and applications. These new applications are contributing to both the increase of energy efficiency as well as greenhouse gas reduction. Such research is critical for scientific advancement and industrial innovations that can support environmentally friendly strategies for sustainable energy systems. The Handbook of Research on Advancements in Supercritical Fluids Applications for Sustainable Energy Systems is a comprehensive two-volume reference that covers the most recent and challenging issues and outlooks for the applications and innovations of supercritical fluids. The book first converts basic thermo-dynamic behaviors and “abnormal” properties from a thermophysical aspect, then basic heat transfer and flow properties, recent new findings of its physical aspect and indications, chemical engineering properties, micro-nano-scale phenomena, and transient behaviors in fast and critical environments. It is ideal for engineers, energy companies, environmentalists, researchers, academicians, and students studying supercritical fluids and their applications for creating sustainable energy systems.
In the vicinity of the pseudocritical point, supercritical carbon dioxide (sCO2) undergoes a steep change in properties from “liquid-like” to “gas-like” as it is heated at a constant pressure. At the same time, there is a large spike in specific heat which can yield high heat transfer coefficients and heat capacity rates. These unique properties have made sCO2 an attractive working fluid in next generation power and HVAC&R technologies. Microchannel heat exchangers are being used to safely and efficiently utilize the high pressure fluid in these applications. However, prior investigation of heating of supercritical CO2 has primarily focused on circular, uniformly heated channels at relatively low heat flux for nuclear power applications. Thus, it is unclear if models and correlations developed from large circular tube data can be scaled down to the smaller, non-circular channels, with non-uniform heating. In the present work, a methodology is developed to experimentally characterize heat transfer for multiple parallel microchannels with a hydraulic diameter of 0.75 mm and aspect ratio of 1. Experiments are conducted over a range of heat fluxes (20 ≤ q” ≤ 40 W cm−2), mass fluxes (500 ≤ G ≤ 1000 kg m−2 s−1), reduced pressure (1.03 ≤ P[subscript R] ≤ 1.1), and inlet temperatures (20 ≤ T[subscript in] ≤ 100°C) in a parallel square microchannel test article with a single-wall constant heat flux boundary condition. Local and average heat transfer coefficients are experimentally measured and the results are compared to previously developed correlations. The predictive capabilities for the supercritical models were poor, with the lowest mean absolute percent error (MAPE) of 55.3% for the range of bulk fluid temperatures, heat fluxes, and mass fluxes. Interestingly, subcritical correlations were also investigated and yielded much lower MAPE than 80% of the supercritical correlations even though the effects of variable fluid properties were not taken into account. The subcritical correlations did not incorporate property ratios to account for the variability in fluid properties; in some supercritical correlations it was found to add additional uncertainty for the case of the present study. The effects of buoyancy and flow acceleration were also evaluated. Based on dimensionless criteria, buoyancy was expected to play a role in heat transfer, especially when the bulk fluid temperature is below the pseudocritical temperature. However, the relative importance of flow acceleration was inconclusive. Despite the apparent importance of buoyancy effects, heat transfer was not degraded, as would be expected in larger, circular, uniformly heated tubes. The mixed convection could be inducing a density driven swirling with the stratification of low-density fluid near the top (unheated). This would ultimately improve the heat transfer at the bottom portion of the test section channels. Therefore, the flow geometry and the non-conventional heated boundary could be improving the heat transfer even with buoyancy driven effects under supercritical conditions.
Supercritical Fluid Technology for Energy and Environmental Applications covers the fundamental principles involved in the preparation and characterization of supercritical fluids (SCFs) used in the energy production and other environmental applications. Energy production from diversified resources — including renewable materials — using clean processes can be accomplished using technologies like SCFs. This book is focused on critical issues scientists and engineers face in applying SCFs to energy production and environmental protection, the innovative solutions they have found, and the challenges they need to overcome. The book also covers the basics of sub- and supercritical fluids, like the thermodynamics of phase and chemical equilibria, mathematical modeling, and process calculations. A supercritical fluid is any substance at a temperature and pressure above its critical point where distinct liquid and gas phases do not exist. At this state the compound demonstrates unique properties, which can be "fine-tuned," making them suitable as organic solvents in a range of industrial and laboratory processes. This volume enables readers to select the most appropriate medium for a specific situation. It helps instructors prepare course material for graduate and postgraduate courses in the area of chemistry, chemical engineering, and environmental engineering. And it helps professional engineers learn supercritical fluid-based technologies and use them in solving the increasingly challenging environmental issues. Relates theory, chemical characteristics, and properties of the particular supercritical fluid to its various applications Covers the fundamentals of supercritical fluids, like thermodynamics of phase and chemical equilibria, mathematical modeling, and process calculations Includes the most recent applications of supercritical fluids, including energy generation, materials synthesis, and environmental protection
Heat transfer inside microscale geometries is a complex and a challenging phenomenon. As supercritical fluids display large variations in their properties in the vicinity of the critical point, their usage could be more beneficial than traditional coolants. This numerical study, in two parts, primarily focuses on the physics that drives the enhanced heat transfer characteristics of carbon dioxide (CO2) near its critical state and in its supercritical state. In the first part of the study, the flow of supercritical Carbon Dioxide (sCO2) over a heated surface inside a microchannel of hydraulic diameter 0.3 mm was studied using three-dimensional computational fluid dynamics (CFD) model. The temperature of the heated surface was then compared and validated with available experimental results. Also, the heat transfer coefficients were predicted and compared with experiments. Additionally, the acceleration and pressure drop of the fluid were estimated and it was found that the available correlations for conventional fluids failed to predict the flow characteristics of the CO2 due to its supercritical nature. In the second part of the analysis, a relatively new phenomenon known as the Piston Effect (PE), also known as the fourth mode of heat transfer, was studied numerically inside a microchannel of depth 0.1 mm using a two-dimensional CFD model, and it was found that the adiabatic thermalization caused by PE was significant in microgravity and terrestrial conditions and that the time scales associated with the PE are faster than the diffusion time scales by a factor of 5 to 6400. In addition, this study revealed the presence of PE in laminar forced convective conditions. A new correlation was developed to predict the temperature raise of the bulk fluid that is farthest from the heated surface.
Using SuperCritical Fluids (SCFs) in various processes is not new, because Mother Nature has been processing minerals in aqueous solutions at critical and supercritical pressures for billions of years. Somewhere in the 20th century, SCFs started to be used in various industries as working fluids, coolants, chemical agents, etc. Written by an international team of experts and complete with the latest research, development, and design, Advanced Supercritical Fluids Technologies is a unique technical book, completely dedicated to modern and advanced applications of supercritical fluids in various industries.Advanced Supercritical Fluids Technologies provides engineers and specialists in various industries dealing with SCFs as well as researchers, scientists, and students of the corresponding departments with a comprehensive overview of the current status, latest trends and developments of these technologies.Dr Igor Pioro is a professor at the University of Ontario Institute of Technology, Canada, and the Founding Editor of the ASME Journal of Nuclear Engineering and Radiation Science.
This book presents contributions from renowned experts addressing research and development related to the two important areas of heat exchangers, which are advanced features and applications. This book is intended to be a useful source of information for researchers, postgraduate students, academics, and engineers working in the field of heat exchangers research and development.