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Presents a unified formulation from first principles of the Hailtonian and statistical mechanics of metallic and insulating crystals, amorphous solids, and liquids.
This important book presents a unified formulation from first principles of the Hamiltonian and statistical mechanics of metallic and insulating crystals, amorphous solids, and liquids. Extensive comparison of theory and experiment provides an accurate understanding of the statistical properties of phonons, electrons, and phonon-phonon and electron-phonon interactions in elemental crystals and liquids. Questions are posed along the following lines: What is the “best” theory for a given property? How accurate is a good theory? What information is gained by a comparison of theory and experiment? How accurate is a good experiment?
Exploring important theories for understanding freezing and the liquid-glass transition, this book is useful for graduate students and researchers in soft-condensed matter physics, chemical physics and materials science. It details recent ideas and key developments, providing an up-to-date view of current understanding. The standard tools of statistical physics for the dense liquid state are covered. The freezing transition is described from the classical density functional approach. Classical nucleation theory as well as applications of density functional methods for nucleation of crystals from the melt are discussed, and compared to results from computer simulation of simple systems. Discussions of supercooled liquids form a major part of the book. Theories of slow dynamics and the dynamical heterogeneities of the glassy state are presented, as well as nonequilibrium dynamics and thermodynamic phase transitions at deep supercooling. Mathematical treatments are given in full detail so readers can learn the basic techniques.
This new edition of the classic text incorporates the many advances in knowledge about liquid crystals that have taken place since its initial publication in 1974. Entirely new chapters describe the types and properties of liquid crystals in terms of both recently discovered phases and current insight into the nature of local order and isotropic-to-nematic transition. There is an extensive discussion of the symmetrical, macroscopic, dynamic, and defective properties of smectics and columnar phases, with emphasis on order-of-magnitude considerations, all illustrated with numerous descriptions of experimental arrangements. The final chapter is devoted to phase transitions in smectics, including the celebrated analogy between smectic A and superconductors. This new version's topicality and breadth of coverage will ensure that it remains an indispensable guide for researchers and graduate students in mechanics and engineering, and in chemical, solid state, and statistical physics.
The aim of this book is to give a unified and critical account of the fundamental aspects of liquid crystals. Preference is given to discussing the assumptions made in developing theories and analyzing experimental data rather than to attempting to compile all the latest results. The book has four parts. Part I is quite descriptive in character and gives a general overview of the various liquid crystalline phases. Part II deals with the macroscopic continuum theory of liquid crystals and gives a systematic development of the theory from a tensorial point of view thus emphasizing the relevant symmetries. Part III concentrates on experiments that provide microscopic information on the orientational behaviour of the molecules. Finally Part IV discusses the theory of the various phases and their attendant phase transitions from both a Landau and a molecular-statistical point of view. Simplifying the various models as far as possible, it critically examines the merits of a molecular-statistical approach.
This book on liquid crystals reports on the new perspectives that have been brought about by the recent expansion of frontiers and overhaul of common beliefs. First, it explores the interaction of light with mesophases, when the light or matter is endowed with topological defects. It goes on to show how electrophoresis, electro-osmosis and the swimming of flagellated bacteria are affected by the anisotropic properties of liquid crystals. It also reports on the recent progress in the understanding of thermomechanical and thermohydrodynamical effects in cholesterics and deformed nematics and refutes the common belief that these effects could explain Lehmann’s observations of the rotation of cholesteric droplets subjected to a temperature gradient. It then studies the physics of the dowser texture, which has remarkable properties. This is of particular interest in regards to nematic monopoles, which can easily be generated, set into motion and collided within it. Finally, this book deals with the spontaneous emergence of chirality in nematics made of achiral molecules, and provides a brief historical context of chirality
Liquid crystals are partially ordered systems without a rigid, long-range structure. The study of these materials covers a wide area: chemical structure, physical properties and technical applications. Due to their dual nature -- anisotropic physical properties of solids and rheological behavior of liquids -- and easy response to externally applied electric, magnetic, optical and surface fields liquid crystals are of greatest potential for scientific and technological applications. The subject has come of age and has achieved the status of being a very exciting interdisciplinary field of scientific and industrial research. This book is an outgrowth of the enormous advances made during the last three decades in both our understanding of liquid crystals and our ability to use them in applications. It presents a systematic, self-contained and up-to-date overview of the structure and properties of liquid crystals. It will be of great value to graduates and research workers in condensed matter physics, chemical physics, biology, materials science, chemical and electrical engineering, and technology from a materials science and physics viewpoint of liquid crystals.
Current understanding of different phases as well as the phase transitions between them has only been achieved following recent theoretical advances on the effects of dimensionality in statistical physics. P S Pershan explains the connection between these two separate areas and gives some examples of problems where the understanding is still not complete. The most important example is the second order phase transition between the nematic and smectic-A phase. Others include the relation between the several hexatic phases that have been observed and the first order restacking transitions between phases that were all previously identified as smectic-B, but which should more properly be identified as crystalline-B. Some relatively recent experimental developments on the discotic phase, liquid crystal surfaces and lyotropic phases are also included. The book includes 41 major reprints of some of the recent seminal work on the structure of liquid crystals. They are introduced by a brief review of the symmetries and other properties of liquid crystalline phases. In addition, there is a discussion of the differences between true liquid crystalline phases and others that were described as liquid crystalline in the early literature, but which have since been shown to be true three-dimensional crystals. The progression from the isotropic fluid, through the nematic, smectic, and various crystalline phases can be understood in terms of a systematic decrease in symmetry, together with an accompanying variation in structure is explained. A guide to the selected reprints and a sort of ?Rosetta Stone? for these various phases is provided. The goal of this book is to explain the systematics of this progression to students and others that are new to this field, as well as to provide a useful handbook for people already working in the field.
Liquid crystals allow us to perform experiments that provide insight into fundamental problems of modern physics, such as phase transitions, frustration, elasticity, hydrodynamics, defects, growth phenomena, and optics (linear and non linear). This excellent volume meets the need for an up-to-date text on liquid crystals.Nematic and Cholesteric Liq
This book presents the theory of soft matter to students at the advanced undergraduate or beginning graduate level. It provides a basic introduction to theoretical physics as applied to soft matter, explaining the concepts of symmetry, broken symmetry, and order parameters; phases and phase transitions; mean-field theory; and the mathematics of variational calculus and tensors. It is written in an informal, conversational style, which is accessible to students from a diverse range of backgrounds. The book begins with a simple “toy model” to demonstrate the physical significance of free energy. It then introduces two standard theories of phase transitions—the Ising model for ferromagnetism and van der Waals theory of gases and liquids—and uses them to illustrate principles of statistical mechanics. From those examples, it moves on to discuss order, disorder, and broken symmetry in many states of matter, and to explain the theoretical methods that are used to model the phenomena. It concludes with a chapter on liquid crystals, which brings together all of these physical and mathematical concepts. The book is accompanied online by a set of “interactive figures”—some allow readers to change parameters and see what happens to a graph, some allow readers to rotate a plot or other graphics in 3D, and some do both. These interactive figures help students to develop their intuition for the physical meaning of equations. This book will prepare advanced undergraduate or early graduate students to go into more advanced theoretical studies. It will also equip students going into experimental soft matter science to be fully conversant with the theoretical aspects and have effective collaborations with theorists.