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The reactors around the world have produced more than 2000 tonnes of plutonium, contained in spent fuel or as separated forms through reprocessing. Disposition of fissile materials has become a primary concern of nuclear non-proliferation efforts worldwide. There is a significant interest in IAEA Member States to develop proliferation resistant nuclear fuel cycles for incineration of plutonium such as inert matrix fuels (IMFs). This publication reviews the status of potential IMF candidates and describes several identified candidate materials for both fast and thermal reactors: MgO, ZrO2, SiC, Zr alloy, SiAl, ZrN; some of these have undergone test irradiations and post irradiation examination. Also discussed are modelling of IMF fuel performance and safety analysis. System studies have identified strategies for both implementation of IMF fuel as homogeneous or heterogeneous phases, as assemblies or core loadings and in existing reactors in the shorter term, as well as in new reactors in the longer term.
This book provides a readable and thought-provoking analysis of the issues surrounding nuclear fuel reprocessing and fast-neutron reactors, including discussion of resources, economics, radiological risk and resistance to nuclear proliferation. It describes the history and science behind reprocessing, and gives an overview of the status of reprocessing programmes around the world. It concludes that such programs should be discontinued. While nuclear power is seen by many as the only realistic solution to the carbon emission problem, some national nuclear establishments have been pursuing development and deployment of sodium-cooled plutonium breeder reactors, and plutonium recycling. Its proponents argue that this system would offer significant advantages relative to current light water reactor technology in terms of greater uranium utilization efficiency, and that separating out the long-lived plutonium and other transuranics from spent fuel and fissioning them in fast reactors would greatly reduce the duration of the toxicity of radioactive waste. However, the history of efforts to deploy this system commercially in a number of countries over the last six decades has been one of economic and technical failure and, in some cases, was used to mask clandestine nuclear weapon development programs. Covering topics of significant public interest including nuclear safety, fuel storage, environmental impact and the spectre of nuclear terrorism, this book presents a comprehensive analysis of the issue for nuclear engineers, policy analysts, government officials and the general public. "Frank von Hippel, Jungmin Kang, and Masafumi Takubo, three internationally renowned nuclear experts, have done a valuable service to the global community in putting together this book, which both historically and comprehensively covers the “plutonium age” as we know it today. They articulate in a succinct and clear manner their views on the dangers of a plutonium economy and advocate a ban on the separation of plutonium for use in the civilian fuel cycle in view of the high proliferation and nuclear-security risks and lack of economic justification." (Mohamed ElBaradei, Director General, International Atomic Energy Agency (1997-2009), Nobel Peace Prize (2005)) "The 1960s dream of a ‘plutonium economy’ has not delivered abundant low-cost energy, but instead has left the world a radioactive legacy of nuclear weapons proliferation and the real potential for nuclear terrorism. Kang, Takubo, and von Hippel explain with power and clarity what can be done to reduce these dangers. The governments of the remaining countries whose nuclear research and development establishments are still pursuing the plutonium dream should pay attention.” (Senator Edward Markey, a leader in the US nuclear-disarmament movement as a member of Congress since 1976) "The authors have done an invaluable service by putting together in one place the most coherent analysis of the risks associated with plutonium, and the most compelling argument for ending the practice of separating plutonium from spent fuel for any purpose. They have given us an easily accessible history of the evolution of thinking about the nuclear fuel cycle, the current realities of nuclear power around the world and, arguably most important, a clear alternative path to deal with the spent fuel arising from nuclear reactors for decades to centuries to come." (Robert Gallucci, Chief US negotiator with North Korea (1994); Dean, Georgetown University School of Foreign Service (1996-2009); President, MacArthur Foundation (2009-2014))
The decay product of the medical isotope molybdenum-99 (Mo-99), technetium-99m (Tc-99m), and associated medical isotopes iodine-131 (I-131) and xenon-133 (Xe-133) are used worldwide for medical diagnostic imaging or therapy. The United States consumes about half of the world's supply of Mo-99, but there has been no domestic (i.e., U.S.-based) production of this isotope since the late 1980s. The United States imports Mo-99 for domestic use from Australia, Canada, Europe, and South Africa. Mo-99 and Tc-99m cannot be stockpiled for use because of their short half-lives. Consequently, they must be routinely produced and delivered to medical imaging centers. Almost all Mo-99 for medical use is produced by irradiating highly enriched uranium (HEU) targets in research reactors, several of which are over 50 years old and are approaching the end of their operating lives. Unanticipated and extended shutdowns of some of these old reactors have resulted in severe Mo-99 supply shortages in the United States and other countries. Some of these shortages have disrupted the delivery of medical care. Molybdenum-99 for Medical Imaging examines the production and utilization of Mo-99 and associated medical isotopes, and provides recommendations for medical use.