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A selected set of reprints from the Optical Frequency Measurement Group of the Time and Frequency Div. of the Nat. Inst. of Standards and Technology and consists of work published between 1987 and 1997. The 2 programs represented are (1) development of tunable diode-laser technology for scientific applications and precision measurements, and (2) research toward the goal of realizing optical-frequency measurements and synthesis. The papers are organized in 5 categories: diode laser technology; tunable laser systems; laser spectroscopy; optical synthesis and extended wavelength coverage; and multi-photon interactions and optical coherence.
This volume is a collection of papers presented at the Fourteenth International Conference on Ultrafast Phenomena held in Niigata, Japan from July 25-30, 2004. The Ultrafast Phenomena Conferences are held every two years and provide a forum for discussion of the latest results in ultrafast optics and their applications in science and engineering. A total of more than 300 papers were presented, reporting the forefront of research in ultrashort pulse generation and characterization, including new techniques for shortening the duration of laser pulses, for stabilizing their absolute phase, and for improving tenability over broad wavelength ranges, output powers and peak intensities. Ultrafast spectroscopies, particularly time-resolved X-ray and electron diffraction and two-dimensional spectroscopy, continue to give new insights into fundamental processes in physics, chemistry and biology. Control and optimization of the outcome of ultrafast processes represent another important field of research. There are an increasing number of applications of ultrafast methodology in material diagnostics and processing, microscopy and medical imaging. The enthusiasm of the participants, the involvement of many students, the high quality of the papers in both oral and poster sessions made the conference very successful. Many people and organizations made invaluable contributions. The members of the international program committee reviewed the submissions and organized the program. The staff of the Optical Society of America deserves special thanks for making the meeting arrangements and running the meeting smoothly.
Over the last few years, there has been a convergence between the fields of ultrafast science, nonlinear optics, optical frequency metrology, and precision laser spectroscopy. These fields have been developing largely independently since the birth of the laser, reaching remarkable levels of performance. On the ultrafast frontier, pulses of only a few cycles long have been produced, while in optical spectroscopy, the precision and resolution have reached one part in Although these two achievements appear to be completely disconnected, advances in nonlinear optics provided the essential link between them. The resulting convergence has enabled unprecedented advances in the control of the electric field of the pulses produced by femtosecond mode-locked lasers. The corresponding spectrum consists of a comb of sharp spectral lines with well-defined frequencies. These new techniques and capabilities are generally known as “femtosecond comb technology. ” They have had dramatic impact on the diverse fields of precision measurement and extreme nonlinear optical physics. The historical background for these developments is provided in the Foreword by two of the pioneers of laser spectroscopy, John Hall and Theodor Hänsch. Indeed the developments described in this book were foreshadowed by Hänsch’s early work in the 1970s when he used picosecond pulses to demonstrate the connection between the time and frequency domains in laser spectroscopy. This work complemented the advances in precision laser stabilization developed by Hall.
"The Symposium on Frequency Standards and Metrology serves as an international forum for discussion of precision frequency standards throughout the electromagnetic spectrum and associated metrology. The symposium focuses on the fundamental aspects of the latest ideas, results and applications in relation to these frequency standards."--Provided by publisher
This text on precision frequency measurement and its key enabling techniques includes reviews written by some of the most experienced researchers in their respective fields. This text should prove useful to researchers just entering the field of frequency metrology and standards, or equally well to the experienced practitioner.
Optical frequency combs (OFC) have revolutionized various applications in applied and fundamental sciences that rely on the determination of absolute optical frequencies and frequency differences. The latter requires only stabilization of the spectral distance between the individual comb lines of the OFC, allowing to tailor and reduce system complexity of the OFC generator (OFCG). One such application is the quantum test of the universality of free fall within the QUANTUS experimental series. Within the test, the rate of free fall of two atomic species, Rb and K, in micro-gravity will be compared. The aim of this thesis was the development of a highly compact, robust, and space-suitable diode laser-based OFCG with a mode-locked optical spectrum in the wavelength range around 780 nm. A diode laser-based OFCG was developed, which exceeds the requirements with a spectral bandwidth > 16 nm at 20 dBc, a comb line optical power > 650 nW (at 20 dBc), a pulse repetition rate of 3.4 GHz, and an RF linewidth of the free-running pulse repetition rate < 10 kHz. To realize a proof-of-concept demonstrator module, the diode laser-based OFCG was hybrid-integrated into a space-suitable technology platform that has been developed for future QUANTUS experiments. Proof of sufficient RF stability of the OFCG was provided by stabilizing the pulse repetition rate to an external RF reference. This resulted in a stabilized pulse repetition rate with an RF linewidth smaller than 1.4 Hz (resolution limited), thus exceeding the requirement. The developed diode laser-based OFCG represents an important step towards an improved comparison of the rate of free fall of Rb and K quantum gases within the QUANTUS experiments in micro-gravity.
The embryonic development of femtoscience stems from advances made in the generation of ultrashort laser pulses. Beginning with mode-locking of glass lasers in the 1960s, the development of dye lasers brought the pulse width down from picoseconds to femtoseconds. The breakthrough in solid state laser pulse generation provided the current reliable table-top laser systems capable of average power of about 1 watt, and peak power density of easily watts per square centimeter, with pulse widths in the range of four to eight femtoseconds. Pulses with peak power density reaching watts per square centimeter have been achieved in laboratory settings and, more recently, pulses of sub-femtosecond duration have been successfully generated. As concepts and methodologies have evolved over the past two decades, the realm of ultrafast science has become vast and exciting and has impacted many areas of chemistry, biology and physics, and other fields such as materials science, electrical engineering, and optical communication. In molecular science the explosive growth of this research is for fundamental reasons. In femtochemistry and femtobiology chemical bonds form and break on the femtosecond time scale, and on this scale of time we can freeze the transition states at configurations never before seen. Even for n- reactive physical changes one is observing the most elementary of molecular processes. On a time scale shorter than the vibrational and rotational periods the ensemble behaves coherently as a single-molecule trajectory.