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This book provides a pedagogical introduction to the emerging field of Polariton Chemistry, where optical cavities are utilized to control the physicochemical properties and dynamics of molecular systems. Given the early stages of this interdisciplinary research area, it is important to provide a common language and starting point for interested researchers across Chemistry, Physics, and Engineering This edited compendium fills a void given that there is currently no analogue in the current literature. Topics covered include Single-Molecule Strong Light-Matter Coupling; Collective Strong Light-Matter Coupling; and Ultrastrong Light-Matter Coupling
Polaritonic chemistry is an emergent interdisciplinary field in which the strong interaction of organic molecules with confined electromagnetic field modes is exploited in order to manipulate the chemical structure and reactions of the system. In the regime of strong light-matter coupling the interaction with the electromagnetic vacuum obliges us to redefine the concept of a molecule and consider the hybrid system as a whole. This thesis builds on the foundations of chemistry and quantum electrodynamics in order to provide a theoretical framework to describe these organic light-matter hybrids. By fully embracing the structural complexity of molecules, this theory allows us to employ long-established quantum chemistry methods to understand polaritonic chemistry. This leads to predictions of substantial structural changes in organic molecules and the possibility of significantly influencing chemical reactions both in the excited and ground states of the system.
The goal of this book is to provide a simple and conceptually intuitive introduction to nonlinear spectroscopy via the formalism of quantum processes and wavepacket dynamics.
Modern Problems in Condensed Matter Sciences, Volume I: Surface Polaritons: Electromagnetic Waves at Surfaces and Interfaces describes the basic properties of surface polaritons and the methods of generating these waves in the laboratory at frequencies of interest to condensed matter physicists. The selection first elaborates on surface phonon polaritons in dielectrics and semiconductors and surface exciton polaritons from the experimental viewpoint. Discussions focus on interface polaritons; surface vibrations in anisotropic crystals; experimental methods for the excitation and study of surface polaritons; and surface vibrations in isotropic crystals. The publication then ponders on surface electromagnetic wave propagation on metal surfaces; thermally stimulated emission of surface polaritons; and effects of the transition layer and spatial dispersion in the spectra of surface polaritons. The text takes a look at surface polaritons at metal surfaces and interfaces and resonance of transition layer excitations with surface polaritons. Topics include resonance of the film phonon with the substrate surface phonon polaritons; investigations of surface modifications in ultra-high vacuum; and use of surface plasma waves for the investigation of solid-liquid and solid-solid interfaces. The selection is a dependable reference for physicists and engineers wanting to conduct research on surface polaritons.
This book reviews progress towards quantum simulators based on photonic and hybrid light-matter systems, covering theoretical proposals and recent experimental work. Quantum simulators are specially designed quantum computers. Their main aim is to simulate and understand complex and inaccessible quantum many-body phenomena found or predicted in condensed matter physics, materials science and exotic quantum field theories. Applications will include the engineering of smart materials, robust optical or electronic circuits, deciphering quantum chemistry and even the design of drugs. Technological developments in the fields of interfacing light and matter, especially in many-body quantum optics, have motivated recent proposals for quantum simulators based on strongly correlated photons and polaritons generated in hybrid light-matter systems. The latter have complementary strengths to cold atom and ion based simulators and they can probe for example out of equilibrium phenomena in a natural driven-dissipative setting. This book covers some of the most important works in this area reviewing the proposal for Mott transitions and Luttinger liquid physics with light, to simulating interacting relativistic theories, topological insulators and gauge field physics. The stage of the field now is at a point where on top of the numerous theory proposals; experiments are also reported. Connecting to the theory proposals presented in the chapters, the main experimental quantum technology platforms developed from groups worldwide to realize photonic and polaritonic simulators in the laboratory are also discussed. These include coupled microwave resonator arrays in superconducting circuits, semiconductor based polariton systems, and integrated quantum photonic chips. This is the first book dedicated to photonic approaches to quantum simulation, reviewing the fundamentals for the researcher new to the field, and providing a complete reference for the graduate student starting or already undergoing PhD studies in this area.
This book offers an overview of polariton Bose–Einstein condensation and the emerging field of polaritonics, providing insights into the necessary theoretical basics, technological aspects and experimental studies in this fascinating field of science. Following a summary of theoretical considerations, it guides readers through the rich physics of polariton systems, shedding light on the concept of the polariton laser, polariton microcavities, and the technical realization of optoelectronic devices with polaritonic emissions, before discussing the role of external fields used for the manipulation and control of exciton–polaritons. A glossary provides simplified summaries of the most frequently discussed topics, allowing readers to quickly familiarize themselves with the content. The book pursues an uncomplicated and intuitive approach to the topics covered, while also providing a brief outlook on current and future work. Its straightforward content will make it accessible to a broad readership, ranging from research fellows, lecturers and students to interested science and engineering professionals in the interdisciplinary domains of nanotechnology, photonics, materials sciences and quantum physics.
Theoretical and Computational Photochemistry: Fundamentals, Methods, Applications and Synergy with Experimental Approaches provides a comprehensive overview of photoactive systems and photochemical processes. After an introduction to photochemistry, the book discusses the key computational chemistry methods applied to the study of light-induced processes over the past decade, and further outlines recent research topics to which these methods have been applied. By discussing the synergy between experimental and computational data, the book highlights how theoretical studies could facilitate understanding experimental findings. This helpful guide is for both theoretical chemists and experimental photochemistry researchers interested in utilizing computational photochemistry methods for their own work. - Reviews the fundamentals of photochemistry, helping those new to the field in understanding key concepts - Provides detailed guidance and comparison of computational and theoretical methods, highlighting the suitability of each method for different case studies - Outlines current applications to encourage discussion of the synergy between experimental and computational data, and inspiring further application of these methods to other photochemical processes
Vibrational Dynamics of Molecules represents the definitive concise text on the cutting-edge field of vibrational molecular chemistry. The chapter contributors are a Who's Who of world leaders in the field. The editor, Joel Bowman, is widely considered as one of the founding fathers of theoretical reaction dynamics. The included topics span the field, from fundamental theory such as collocation methods and vibrational CI methods, to interesting applications such as astrochemistry, supramolecular systems and virtual computational spectroscopy. This is a useful reference for theoretical chemists, spectroscopists, physicists, undergraduate and graduate students, lecturers and software developers.
Rapid development of microfabrication and assembly of nanostructures has opened up many opportunities to miniaturize structures that confine light, producing unusual and extremely interesting optical properties. This book addresses the large variety of optical phenomena taking place in confined solid state structures: microcavities. Realisations include planar and pillar microcavities, whispering gallery modes, and photonic crystals. The microcavities represent a unique laboratory for quantum optics and photonics. They exhibit a number of beautiful effects including lasing, superfluidity, superradiance, entanglement etc. Written by four practitioners strongly involved in experiments and theories of microcavities, it is addressed to any interested reader having a general physical background, but in particular to undergraduate and graduate students at physics faculties.
The book reviews the properties of surface plasmons that depict electromagnetic surface waves or surface plasma polaritons. Their propagation on smooth and corrugated surfaces (with rough or grating profiles) is considered. In the latter case, the corrugations can cause strong coupling of the surface plasmons with photons leading to resonances with a strong enhancement of the electromagnetic field in the surface. Coupling and field enhancement are the most prominent phenomena on corrugated surfaces and lead to numerous important applications. Attention has been focused on the explanation of the physics. To keep the text readable, sophisticated calculations have been avoided, and instead various applications dealing with enhanced light emission, nonlinear optics, SERS, and other cases of interest are discussed.