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This book offers historical and state-of-the-art molecular spectroscopy methods and applications in dynamic compression science, aimed at the upcoming generation in physical sciences involved in studies of materials at extremes. It begins with addressing the motivation for probing shock compressed molecular materials with spectroscopy and then reviews historical developments and the basics of the various spectroscopic methods that have been utilized. Introductory chapters are devoted to fundamentals of molecular spectroscopy, overviews of dynamic compression technologies, and diagnostics used to quantify the shock compression state during spectroscopy experiments. Subsequent chapters describe all the molecular spectroscopic methods used in shock compression research to date, including theory, experimental details for application to shocked materials, and difficulties that can be encountered. Each of these chapters also includes a section comparing static compression results. The last chapter offers an outlook for the future, which leads the next-generation readers to tackling persistent problems.
Developing and testing novel energetic materials is an expanding branch of the materials sciences. Reaction, detonation or explosion of such materials invariably produce extremely high pressures and temperatures. To study the equations-of-state (EOS) of energetic materials in extreme regimes both shock and static high pressure studies are required. The present volume is an introduction and review of theoretical, experimental and numerical aspects of static compression of such materials. Chapter 1 introduces the basic experimental tool, the diamond anvil pressure cell and the observational techniques used with it such as optical microscopy, infrared spectrometry and x-ray diffraction. Chapter 2 outlines the principles of high-nitrogen energetic materials synthesis. Chapters 3 and 4, examine and compare various EOS formalisms and data fitting for crystalline and non-crystalline materials, respectively. Chapter 5 details the reaction kinetics of detonating energetic materials. Chapter 6 investigates the interplay between static and dynamic (shock) studies. Finally, Chapters 7 and 8 introduce numerical simulations: molecular dynamics of energetic materials under either hydrostatic or uni-axial stress and ab-inito treatments of defects in crystalline materials. This timely volume meets the growing demand for a state-of-the art introduction and review of the most relevant aspects of static compression of energetic materials and will be a valuable reference to researchers and scientists working in academic, industrial and governmental research laboratories.
Shock Waves in Condensed Matter – 1983 covers the proceedings of the American Physical Society Topical Conference, held in Santa Fe, New Mexico on July 18-21, 1983. The book focuses on the response of matter to dynamic high pressure and temperature. The selection first elaborates on the review of theoretical calculations of phase transitions and comparisons with experimental results; theoretical and experimental studies of shock-compressed benzene and polybutene; and theory of the iron equation of state and melting curve to very high pressures. The text then ponders on nonhydrostatic effects in stress-wave induced phase transformation of calcite; Bauschinger effect model suitable for use in large computer codes; and strain rate sensitivity prediction for porous bed compaction. The manuscript takes a look at flaw nucleation and energetics of dynamic fragmentation, shock loading behavior of fused quartz, and aluminum damage simulation in high-velocity impact. Shock wave diagnostics by time-resolved infrared radiometry and non-linear Raman spectroscopy; Raman scattering temperature measurement behind a shock wave; and experiments and simulation on laser-driven shock wave evolution in aluminum targets are also discussed. The selection is a dependable reference for scientists and readers interested in the response of matter when exposed to dynamic high pressure and temperature.
For more than two decades time-resolved vibrational spectroscopy (TRVS) was only part of general conferences on solid-state physics, molecular spec troscopy, photochemistry and photobiology. It was in 1982 when the first meeting on TRVS was organized at Lake Placid. The conference met a strong need among the workers in the field, and it was decided to continue with spe cial conferences on this topic. The 2nd International Conference on Time-Resolved Vibrational Spec troscopy was held June 3-i, 1985 at Bayreuth-Bischofsgrun, Germany. Sci entists from many disciplines came together to discuss their common interest in time-resolved techniques and spectroscopic applications. The high qual ity of the research presented, the enthusiasm of the participants, and the attractive surroundings combined to an enjoyable atmosphere. Ample time for discussions and the limited number of participants (approximately 100) stimulated the formal and informal exchange of ideas. "\'umerous people helped to make the conference run smoothly. Special thanks are due to Mrs. Lenich for making the technical arrangements, and to the program committee for the selection of the scientific presentations. The meeting has benefited from several financial souces. The generous sup port by the Emil-Warburg-Stiftung was particularly helpful. Financial aid of the "Deutsche Forschungsgemeinschaft" and of the "Bayerisches Staatsmini sterium fur U nterricht und K ultus" is also gratefully acknowledged.
It is known that the Chapman-Jouguet theory of detonation is based on the assumption of an instantaneous and complete transformation of explosives into detonation products in the wave front. Therefore, one should not expect from the theory any interpretations of the detonation limits, such as shock initiation of det onation and kinetic instability and propagation (failure diameter). The Zeldovich-Von Neuman-Doring (ZND) theory of detonation appeared, in fact, as a response to the need for a theory capable of interpreting such limits, and the ZND detonation theory gave qualitative interpretations to the detonation limits. These interpretations were based essentially on the theoretical notion that the mechanism of explosives transformation at detonation is a combustion of a layer of finite thickness of shock-compressed explosive behind the wave shock front with the velocity of the front. However, some experimental findings turned out to be inconsistent with the the ory. A very small change of homogeneous (liquid) explosives detonation velocity with explosive charge diameter near the rather sizable failure diameter is one of the findings. The elucidation of the nature of this finding has led to the discovery of a new phenomenon. This phenomenon has come to be known as the breakdown (BD) of the explosive self-ignition behind the front of shock waves under the effect of rarefaction waves.
Reviews the latest theory, techniques, and applications Surface vibrational spectroscopy techniques probe the structure and composition of interfaces at the molecular level. Their versatility, coupled with their non-destructive nature, enables in-situ measurements of operating devices and the monitoring of interface-controlled processes under reactive conditions. Vibrational Spectroscopy at Electrified Interfaces explores new and emerging applications of Raman, infrared, and non-linear optical spectroscopy for the study of charged interfaces. The book draws from hundreds of findings reported in the literature over the past decade. It features an internationally respected team of authors and editors, all experts in the field of vibrational spectroscopy at surfaces and interfaces. Content is divided into three parts: Part One, Nonlinear Vibrational Spectroscopy, explores properties of interfacial water, ions, and biomolecules at charged dielectric, metal oxide, and electronically conductive metal catalyst surfaces. In addition to offering plenty of practical examples, the chapters present the latest measurement and instrumental techniques. Part Two, Raman Spectroscopy, sets forth highly sensitive approaches for the detection of biomolecules at solid-liquid interfaces as well as the use of photon depolarization strategies to elucidate molecular orientation at surfaces. Part Three, IRRAS Spectroscopy (including PM-IRRAS), reports on wide-ranging systems from small fuel molecules at well-defined surfaces to macromolecular complexes that serve as the building blocks for functional interfaces in devices designed for chemical sensing and electric power generation. The Wiley Series on Electrocatalysis and Electrochemistry is dedicated to reviewing important advances in the field, exploring how these advances affect industry. The series defines what we currently know and can do with our knowledge of electrocatalysis and electrochemistry as well as forecasts where we can expect the field to be in the future.
Laser ablation describes the interaction of intense optical fields with matter, in which atoms are selectively driven off by thermal or nonthermal mechanisms. The field of laser ablation physics is advancing so rapidly that its principal results are seen only in specialized journals and conferences. This is the first book that combines the most recent results in this rapidly advancing field with authoritative treatment of laser ablation and its applications, including the physics of high-power laser-matter interaction. Many practical applications exist, ranging from inertial confinement fusion to propulsion of aerostats for pollution monitoring to laser ignition of hypersonic engines to laser cleaning nanoscale contaminants in high-volume computer hard drive manufacture to direct observation of the electronic or dissociative states in atoms and molecules, to studying the properties of materials during 200kbar shocks developed in 200fs. Selecting topics which are representative of such a broad field is difficult. Laser Ablation and its Applications emphasizes the wide range of these topics rather than - as is so often the case in advanced science – focusing on one specialty or discipline. The book is divided into four sections: theory and modeling, ultrafast interactions, material processing and laser-matter interaction in novel regimes. The latter range from MALDI to ICF, SNOM’s and femtosecond nanosurgery to laser space propulsion. The book arose from the SPIE series of High Power Laser Ablation Symposia which began in 1998. It is intended for a graduate course in laser interactions with plasmas and materials, but it should be accessible to anyone with a graduate degree in physics or engineering. It is also intended as a major reference work to familiarize scientists just entering the field with laser ablation and its applications.
This unique and encyclopedic reference work describes the evolution of the physics of modern shock wave and detonation from the earlier and classical percussion. The history of this complex process is first reviewed in a general survey. Subsequently, the subject is treated in more detail and the book is richly illustrated in the form of a picture gallery. This book is ideal for everyone professionally interested in shock wave phenomena.
This book constitutes the Proceedings of the Conference of the American Physical Society Topical Group on Shock Compression of Condensed Matter, Baltimore, Maryland USA, 2005. The volume embodies the most recent research on shock compression of condensed matter and includes 363 plenary, invited, and contributed papers, all peer-reviewed. Topics include: equations of state, phase transitions, chemical reactions, warm dense matter, fracture, geophysics and planetary science, energetic materials, optical studies, and more.