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Physical Chemistry: An Advanced Treatise: Reactions in Condensed Phases, Volume VII, deals with reactions in condensed phases. The purpose of this treatise is to present a comprehensive treatment of physical chemistry for advanced students and investigators in a reasonably small number of volumes. An attempt has been made to include all important topics in physical chemistry together with borderline subjects which are of particular interest and importance. The book begins by discussing the basic principles of reaction rates in solution. This is followed by separate chapters on estimating the rate parameters of elementary reactions; the use of correlation diagrams to interpret organic reactions; perturbation of reaction rates by substituents; and inorganic reactions. Subsequent chapters cover the important field of free radicals, including chain reactions and solvent effects; heterogeneous catalysis; various types of surface reactions; surface annealing; electron reactions; nucleation; and radiation chemistry. The book presents a broad picture of current developments in reaction rates in condensed phases in a form accessible to all students of chemical kinetics. This treatment, by experts in widely different areas, will hopefully meet many student needs and provide a useful overview for all.
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In this new textbook on physical chemistry, fundamentals are introduced simply yet in more depth than is common. Topics are arranged in a progressive pattern, with simpler theory early and more complicated theory later. General principles are induced from key experimental results. Some mathematical background is supplied where it would be helpful. Each chapter includes worked-out examples and numerous references. Extensive problems, review, and discussion questions are included for each chapter. More detail than is common is devoted to the nature of work and heat and how they differ. Introductory Caratheodory theory and the standard integrating factor for dGrev are carefully developed. The fundamental role played by uncertainty and symmetry in quantum mechanics is emphasized. In chemical kinetics, various methods for determined rate laws are presented. The key mechanisms are detailed. Considerable statistical mechanics and reaction rate theory are then surveyed. Professor Duffey has given us a most readable, easily followed text in physical chemistry.
For Researchers, Students, Industrial Professionals, and ManufacturersElectrochemical Reduction of Carbon Dioxide: Fundamentals and Technologies is your guide to improved catalytic performance in the electrochemical reduction of carbon dioxide (CO2). Written by electrochemical energy scientists actively involved in environmental research and develo
Los Alamos National Laboratory is an incredible place. It was conceived and born amidst the most desperate of circumstances. It attracted some of the most brilliant minds, the most innovative entrepreneurs, and the most c- ative tinkerers of that generation. Out of that milieu emerged physics and engineering that beforehand was either unimagined, or thought to be f- tasy. One of the ?elds essentially invented during those years was the science of precision high explosives. Before 1942, explosives were used in munitions and commercial pursuits that demanded proper chemistry and con?nement for the necessary e?ect, but little else. The needs and requirements of the Manhattan project were of a much more precise and speci?c nature. Spatial and temporal speci?cations were reduced from centimeters and milliseconds to micrometers and nanoseconds. New theory and computational tools were required along with a raft of new experimental techniques and novel ways of interpreting the results. Over the next 40 years, the emphasis was on higher energy in smaller packages, more precise initiation schemes, better and safer formulations, and greater accuracy in forecasting performance. Researchers from many institutions began working in the emerging and expanding ?eld. In the midst of all of the work and progress in precision initiation and scienti?c study, in the early 1960s, papers began to appear detailing the ?rst quantitative studies of the transition from de?agration to detonation (DDT), ?rst in cast, then in pressed explosives, and ?nally in propellants.
This book highlights the latest experimental and theoretical developments in the field of femtochemistry, with papers describing the physics and chemistry of ultrafast processes in small molecules, complex molecular systems, clusters, biological systems, solids, matrices, liquids and at surfaces and interfaces. The recent developments in frequency-domain studies of femtodynamics are also presented. In addition, the latest achievements in femtosecond control of chemical reactions are presented, together with the newest techniques in real-time probing of reactions such as ultrafast x-ray or electron diffraction. The papers are rich in references giving a clearcut state-of-the-art of the topics being discussed. The book should be a valuable tool to all persons in the field and to young scientists.Contributors include: A H Zewail, J Jortner, V S Letokhov, J Manz, R S Berry, C Wittig, K B Eisenthal, A W Castleman Jr., J T Hynes, W H Gadzuk, R Kosloff, S Mukamel, K R Wilson; G Fleming, D Wiersma, K Yoshihara, V Sundström, A Apkarian, N Scherer, A Myers, R Schinke, J R Huber, R B Gerber, G Gerber and P M Champion.