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This thesis lays the groundwork for producing a new class of ultracold molecule by associating an alkali-metal atom and a closed-shell alkaline-earth-like atom, specifically Cs and Yb. Such molecules exhibit both a magnetic dipole moment and an electric dipole moment in their ground state. This extra degree of freedom opens up new avenues of research including the study of exotic states of matter, the shielding of molecular collisions and the simulation of lattice spin models. In detail, the thesis reports the first and only ultracold mixture of Cs and Yb in the world, giving details of the methods used to cool such contrasting atomic species together. Using sensitive two-colour photoassociation measurements to measure the binding energies of the near-threshold CsYb molecular levels in the electronic ground state has allowed the previously unknown scattering lengths to be accurately determined for all the Cs–Yb isotopic combinations. As part of this work, the one-photon photoassociation of ultracold Cs*Yb is also studied, yielding useful information on the excited-state potential. Knowledge of the scattering lengths enables a strategy to be devised to cool both species to quantum degeneracy and, crucially, determines the positions of interspecies Feshbach resonances required for efficient association of ground-state CsYb molecules. With these results, the prospect of bringing a new molecule into the ultracold regime has become considerably closer.
Electric dipole moments (EDMs) have interested physicists since 1950, when it was first suggested that there was no experimental evidence that nuclear forces are symmetric under parity (P) transformation. This question was regarded as speculative because the existence of an EDM, in addition to P violation, requires a violation of time-reversal (T) symmetry. In 1964 it was discovered that the invariance under CP transformation, which combines charge conjugation (C) with parity, is violated in K-meson decays. This provided a new incentive for EDM searches. Since the combined operations of CPT are expected to leave a system invariant, breakdown of CP invariance should be accompanied by a violation of time-reversal symmetry. Thus there is a reason to expect that EDMs should exist at some level. The original neutron EDM experiments were later supplemented with checks of T invariance in atoms and molecules. These investigations are pursued now by many groups. Over the years, the upper limit on the neutron EDM has been improved by seven orders of magnitude, and the upper limit on the electron EDM obtained in atomic experiments is even more strict.
Recent years have seen tremendous progress in research on cold and controlled molecular collisions, both in theory and in experiment. The advent of techniques to prepare cold and ultracold molecules and ions, to store them in optical lattices or in charged quasicristalline structures, and to use them in crossed or merged beam experiments have opened many new possibilities to study the most fundamental aspects of molecular interactions. At the same time, theoretical work has made progress in tackling these problems and accurately describing quantum effects in complex systems, and in proposing viable options to control chemical reactions at ultralow energies. Through tutorials on both the theoretical and experimental aspects of research in cold and ultracold molecular collisions, this book provides advanced undergraduate students, graduate students and researchers with the foundations needed to understand this exciting field.
Arising from a workshop, this book surveys the physics of ultracold atoms and molecules taking into consideration the latest research on ultracold phenomena, such as Bose Einstein condensation and quantum computing. Several reputed authors provide an introduction to the field, covering recent experimental results on atom and molecule cooling as well as the theoretical treatment.