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The main objective of this workshop was to review and discuss the electronic and chemical properties of layered cuprate superconductors. These are doped antiferromagnetic (AFM) insulators, and there is the possibility of a dynamic phase separation into metallic clusters and AFM areas. A clarification on the existence and the mechanism of such a phase separation is believed to be crucial for the understanding of high-Tc superconductivity in cuprates.On the one hand, theoretical and recent experimental indications in favor of this possibility were presented, on the other hand experimental papers expressing more skeptical views were also delivered. Related work on phase separations of chemical and structural origin was also included, followed by contributions on the question; “If phase separation is present, what is the pairing mechanism in the metallic clusters?”.
Phase separation has become a fascinating subject in the discussion of cuprate superconductors. All these materials have layered structures containing CU02 planes as the most important building blocks. They are coupled only weakly so that the electronic properties show a nearly two-dimensional behaviour. Due to correlations the undoped compounds are insulators of the Mott Hubbard type exhibiting long-range antiferromagnetic order. Upon doping a rich scenario of physical phenomena appears: Even at low hole concentra tions the antiferromagnetic ordering temperature is reduced drastically and spin-glass behaviour as well as a hopping type conductivity can be observed. Further doping leads to metallic-like conductivity and below Tc to super conductivity. In this doping regime antiferromagnetic fluctuations are still observed. At very high charge carrier densities superconductivity is lost and the systems show pure metallic conduction without ,magnetic correlations. One of the most interesting phenomena in high-T c research is the interplay between magnetism and conductivity or superconductivity. Especially the behaviour of charge carriers in the antiferromagnetic background raises a number of open questions. Two scenarios become possible: the carriers tend to delocalize over the whole crystal forming a homogeneous state with band-like structure or they separate into hole-rich (conducting, superconducting) and hole-poor (insulating, antiferromagnetic) phases leading to an inhomogeneous structure.
With this book, we wish to honor the lifework of K. Alex Müller and present him with this book on the occasion of his 94th birthday. We are convinced that he will very much enjoy reading it. We would like to thank all contributors to this book, who addressed topics complementary and related to his work. The articles of the book represent the efforts in solid state physics – spanning more than 60 years – which have been groundbreaking in scientific and applied sciences. Many of the current hot topics are derived from this earlier work which has pioneered the way toward new experimental tools and/or refined techniques. From this point of view, the book presents, on one hand, a historical review and, on the other hand, a directory of possible future research.
This volume will contain both invited and contributed papers which focus on the search for new high-Tc materials, characterization of their physical properties and microstructures, basic applications and the application of high-Tc superconductors.
After an introduction by J.G. Bednorz, describing the discovery of high Tc superconductivity and its consequences, the book goes on to describe modern research, dealing with general problems, new materials and structures, phase separation, electronic homogeneities and related problems, and applications. Specific systems dealt with include the La-cuprates. the Bi-cuprates and the Y-cuprates and related compounds.
Authored by many of the world's leading experts on high-Tc superconductivity, this volume presents a panorama of ongoing research in the field, as well as insights into related multifunctional materials. The contributions cover many different and complementary aspects of the physics and materials challenges, with an emphasis on superconducting materials that have emerged since the discovery of the cuprate superconductors, for example pnictides, MgB2, H2S and other hydrides. Special attention is also paid to interface superconductivity. In addition to superconductors, the volume also addresses materials related to polar and multifunctional ground states, another class of materials that owes its discovery to Prof. Müller's ground-breaking research on SrTiO3.
This book presents theoretical as well as experimental articles focused on recent new results in high temperature superconductivity. All contributors are high ranking scientists who have done major work to enhance the understanding of this phenomenon. A few articles deal with ferroelectricity and its applications. The book is dedicated to Prof. Dr. K. Alex Müller on his 80th birthday. During his scientific career he made major advances in the understanding of ferroelectricity.
A broad introduction to high Tc superconductors, their parent compounds and related novel materials, covering both fundamental questions of modern solid state physics (such as correlation effects, fluctuations, unconventional symmetry of superconducting order parameter) and applied problems related to short coherence length, grain boundaries and thin films. The information that can be derived from electron spectroscopy and optical measurements is illustrated and explained in detail. Descriptions widely employ the clear, relatively simple, phenomenological Ginzburg-Landau model of complex phenomena, such as vortex physics, vortex charge determination, plasmons in superconductors, Cooper pair mass, and wetting of surfaces. The first comprehensive reviews of several novel classes of materials are presented, including borocarbides and chain cuprates.
The problem of superconductors has been a central issue in Solid State Physics since 1987. After the discovery of superconductivity (HTSC) in doped perovskites, it was realized that the HTSC appears in an unknown complex electronic phase of c- densed matter. In the early years, all theories of HTSC were focused on the physics of a homogeneous 2D metal with large electron–electron correlations or on a 2D polaron gas. Only after 1990, a novel paradigm started to grow where this 2D metallic phase is described as an inhomogeneous metal. This was the outcome of several experimental evidences of phase separation at low doping. Since 1992, a series of conferences on phase separation were organized to allow scientists to get together to discuss the phase separation and related issues. Following the discovery by the Rome group in 1992 that “the charges move freely mainly in one direction like the water running in the grooves in the corrugated iron foil,” a new scenario to understand superconductivity in the superconductors was open. Because the charges move like rivers, the physics of these materials shifts toward the physics of novel mesoscopic heterostructures and complex electronic solids. Therefore, understanding the striped phases in the perovskites not only provides an opportunity to understand the anomalous metallic state of cuprate superconductors, but also suggests a way to design new materials of technological importance. Indeed, the stripes are becoming a field of general scientific interest.
As a spectroscopic method, Nuclear Magnetic Resonance (NMR) has seen spectacular growth over the past two decades, both as a technique and in its applications. Today the applications of NMR span a wide range of scientific disciplines, from physics to biology to medicine. Each volume of Nuclear Magnetic Resonance comprises a combination of annual and biennial reports which together provide comprehensive of the literature on this topic. This Specialist Periodical Report reflects the growing volume of published work involving NMR techniques and applications, in particular NMR of natural macromolecules which is covered in two reports: "NMR of Proteins and Acids" and "NMR of Carbohydrates, Lipids and Membranes". For those wanting to become rapidly acquainted with specific areas of NMR, this title provides unrivalled scope of coverage. Seasoned practitioners of NMR will find this an in valuable source of current methods and applications. Specialist Periodical Reports provide systematic and detailed review coverage in major areas of chemical research. Compiled by teams of leading authorities in the relevant subject areas, the series creates a unique service for the active research chemist, with regular, in-depth accounts of progress in particular fields of chemistry. Subject coverage within different volumes of a given title is similar and publication is on an annual or biennial basis.