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This volume is a collection of review articles by scientists who have pioneered many of the recent advances in studies of the optical effects of small particles. The book begins with a review of the multitude of sharp dielectric resonances which exist in all optical spectra as a result of particle size and shape. Latest advances in absorption and fluorescence spectroscopy of a single particle and/or an ensemble of particles are also discussed, as well as advances in the energy transfer mechanisms for molecules embedded in the particle. The effects of laser-induced heating on a single particle are reviewed in terms of the hydrodynamics and thermodynamics of the liquid droplet and its ambient gas surrounding. The limits of applying bulk optical constants to small particles which lie between the bulk substance and the quantum-sized substance are also presented.
A thorough and up-to-date treatment of electromagnetic scattering by small particles.
Optical Properties of Metal Clusters deals with the electronic structure of metal clusters determined optically. Clusters - as state intermediate between molecules and the extended solid - are important in many areas, e.g. in air pollution, interstellar matter, clay minerals, photography, heterogeneous catalysis, quantum dots, and virus crystals. This book extends the approaches of optical molecular and solid-state methods to clusters, revealing how their optical properties evolve as a function of size. Cluster matter, i.e. extended systems of many clusters - the most frequently occuring form - is also treated. The combination of reviews of experimental techniques, lists of results and detailed descriptions of selected experiments will appeal to experts, newcomers and graduate students in this expanding field.
This Festschrift is a tribute to an eminent scholar, scientist and engineer, Professor Richard Kounai Chang, on his retirement from Yale University on June 12, 2008. During approximately half of a century of scientific and technological exploration, Professor Chang contributed to the development of linear and nonlinear optics, novel photonic light localization devices, surface second harmonic generation, surface-enhanced Raman scattering, and novel optical methods for detecting airborne aerosol pathogens. This volume contains a collection of articles contributed by former students, collaborators, and colleagues of Professor Chang, who are leaders in academia, national laboratories and industrial research all over the world. The topics cover important optical science and technology areas including linear and nonlinear spectroscopy, linear and nonlinear optics in microparticles, linear and nonlinear spectroscopy of bioaerosols, optical microcavities and nanostructures, and photoscapes or multidisciplinary applications.
Absorption and Scattering of Light by Small Particles Treating absorption and scattering in equal measure, this self-contained, interdisciplinary study examines and illustrates how small particles absorb and scatter light. The authors emphasize that any discussion of the optical behavior of small particles is inseparable from a full understanding of the optical behavior of the parent material-bulk matter. To divorce one concept from the other is to render any study on scattering theory seriously incomplete. Special features and important topics covered in this book include: * Classical theories of optical properties based on idealized models * Measurements for three representative materials: magnesium oxide, aluminum, and water * An extensive discussion of electromagnetic theory * Numerous exact and approximate solutions to various scattering problems * Examples and applications from physics, astrophysics, atmospheric physics, and biophysics * Some 500 references emphasizing work done since Kerker's 1969 work on scattering theory * Computer programs for calculating scattering by spheres, coated spheres, and infinite cylinders
In the course of the development of surface science, advances have been identified with the introduction of new diagnostic probes for analytical characterization of the adsorbates and microscopic structure of surfaces and interfaces. Among the most recently de veloped techniques, and one around which a storm of controversy has developed, is what has now been earmarked as surface enhanced Raman scattering (SERS). Within this phenomenon, molecules adsorbed onto metal surfaces under certain conditions exhibit an anomalously large interaction cross section for the Raman effect. This makes it possible to observe the detailed vibrational signature of the adsorbate in the ambient phase with an energy resolution much higher than that which is presently available in electron energy loss spectroscopy and when the surface is in contact with a much larger amount of material than that which can be tolerated in infrared absorption experiments. The ability to perform vibrational spectroscopy under these conditions would lead to a new understanding about the chemical identity, geome try, and bonding of adsorbed material at a level previously unacces sible. It is for these reasons that the last few years have brought an explosion of activity surrounding the exploitation of SERS. The search for the origines) of the anomalous enhancement has given rise to a research sub-activity of its own. Efforts to explain the en hancement have led to an increased understanding of the whole range of phenomena associated with the interaction of photons with adsor bates and metal surfaces.
The control of optical modes in microcavities or in photonic bandgap (PBG) materials is coming of age! Although these ideas could have been developed some time ago, it is only recently that they have emerged, due to advances in both atomic physics and in fabrication techniques, be it on the high-quality dielectric mirrors required for high-finesse Fabry Perot resonators or in semiconductor multilayer deposition methods. Initially the principles of quantum electro-dynamics (QED) were demonstrated in elegant atomic physics experiments. Now solid-state implementations are being investigated, with several subtle differences from the atomic case such as those due to their continuum of electronic states or the near Boson nature of their elementary excitations, the exciton. Research into quantum optics brings us ever newer concepts with potential to improve system performance such as photon squeezing, quantum cryptography, reversible taps, photonic de Broglie waves and quantum computers. The possibility of implementing these ideas with solid-state systems gives us hope that some could indeed find their way to the market, demonstrating the continuing importance of basic research for applications, be it in a somewhat more focused way than in earlier times for funding.
Near-field optics, dealing with the interaction between optical field and matter in the nanometric region, has become an interdisciplinary field spaning physics, chemistry, materials science, electrical engineering and high density data storage. This book reflects the recent status of this rapidly growing field. It discusses the basic theories, instrumentation, novel probes, theoretical simulations, and the application of near-field optics to the fields of condensed matter physics, new materials, information storage, atom photonics, etc. It provides an overview of the research on near-field optics in the 1990s.
Co-authored by an experimentalist (Klaus M3ller-Dethlefs ) and theoretician (Pavel Hobza), the aim of this book is to provide a general introduction into the science behind non-covalent interactions and molecular complexes using some important experimental and theoretical methods and approaches.
Setting the pace for progress and innovation . . . "[Provides] a wealth of information on frontier photochemistry . . . could easily serve as a definitive source of background information for future researchers." —Journal of the American Chemical Society "The overall quality of the series and the timeliness of selections and authors warrants continuation of the series by any library wishing to maintain a first-rate reference series to the literature." —Physics Today ADVANCES IN PHOTOCHEMISTRY More than a simple survey of the current literature, Advances in Photochemistry offers critical evaluations written by internationally recognized experts. These pioneering scientists offer unique and varied points of view of the existing data. Their articles are challenging as well as provocative and are intended to stimulate discussion, promote further research, and encourage new developments in the field.