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The sodium fast reactor is under consideration for consuming the transuranic waste in the spent nuclear fuel generated by light water reactors. This work is concerned with specialized target assemblies for an oxide-fueled sodium fast reactor that are designed exclusively for burning the americium and higher mass actinide component of light water reactor spent nuclear fuel (SNF). The associated gamma and neutron radioactivity, as well as thermal heat, associated with decay of these actinides may significantly complicate fuel handling and fabrication of recycled fast reactor fuel. The objective of using targets is to isolate in a smaller number of assemblies these concentrations of higher actinides, thus reducing the volume of fuel having more rigorous handling requirements or a more complicated fabrication process. This is in contrast to homogeneous recycle where all recycled actinides are distributed among all fuel assemblies. Several heterogeneous core geometries were evaluated to determine the fewest target assemblies required to burn these actinides without violating a set of established fuel performance criteria. The DIF3D/REBUS code from Argonne National Laboratory was used to perform the core physics and accompanying fuel cycle calculations in support of this work. Using the REBUS code, each core design was evaluated at the equilibrium cycle condition.
A 1000 MWth commercial-scale Sodium Fast Reactor (SFR) design was selected as the baseline in this scenario study. Traditional approaches to Light Water Reactor (LWR) Spent Nuclear Fuel (SNF) transuranic waste (TRU) burning in a fast spectrum system have typically focused on the continual homogeneous recycling (reprocessing) of the discharge fast reactor fuel. The effective reduction of transuranic inventories has been quantified through the use of the transuranics conversion ratio (TRU CR). The implicit assumption in the use of this single parameter is a homogeneous fast reactor option where equal weight is given to the destruction of transuranics, either by fission or eventual fission via transmutation. This work explores the potential application of alternative fast reactor fuel cycles in which the minor actinide (MA) component of the TRU is considered 'waste', while the plutonium component is considered as fuel. Specifically, a set of potential designs that incorporate radial heterogeneous target assemblies is proposed and results relevant to transmutation and system analysis are presented. In this work we consider exclusively minor actinide-bearing radial targets in a continual reprocessing scenario (as opposed to deep-burn options). The potential use of targets in a deep burn mode is not necessarily ruled out as an option. However, due to work scope constraints and material limit considerations, it was preferred to leave the target assemblies reach either the assumed limit of 200 DPA at discharge or maximum allowable gas pressure caused by helium production from transmutation. The number and specific design of the target assemblies was chosen to satisfy the necessary core symmetry and physical dimensions (available space for a certain amount of mass in an assembly based on an iterated mass density).
The threshold-fission (fertile) nature of Am-241 is used to destroy this minor actinide by capitalizing upon neutron capture instead of fission within a sodium fast reactor. This neutron-capture and its subsequent decay chain leads to the breeding of even mass number plutonium isotopes. A slightly moderated target design is proposed for breeding plutonium in an axial blanket located above the active "fast reactor" driver fuel region. A parametric study on the core height and fuel pin diameter-to-pitch ratio is used to explore the reactor and fuel cycle aspects of this design. This study resulted in both a non-flattened and a pancake core geometry. Both of these designs demonstrated a high capacity for removing americium from the fuel cycle. A reactivity coefficient analysis revealed that this heterogeneous design will have comparable safety aspects to a homogeneous reactor of the same size.
In sodium fast reactor designs, the fuel related inherent negative reactivity feedback is accomplished mainly through parasitic capture in U-238. However for an efficient minor actinide burning system, it is desirable to reduce or eliminate U-238 entirely to suppress further transuranic actinide generation. Consequently, reactivity feedback is accomplished by enhancing axial neutron streaming during a loss of coolant void situation. This is done by flattening "pancake" the active core geometry. Flattening the reactor also increases axial leakage which removes neutrons that could otherwise be used to destroy minor actinides. Therefore, it is important to tailor the neutron spectrum in the core for optimized feedback and minor actinide destruction simultaneously by using minor actinide and fission product targets.
The once-through fuel cycle strategy in the United States for the past six decades has resulted in an accumulation of Light Water Reactor (LWR) Spent Nuclear Fuel (SNF). This SNF contains considerable amounts of transuranic (TRU) elements that limit the volumetric capacity of the current planned repository strategy. A possible way of maximizing the volumetric utilization of the repository is to separate the TRU from the LWR SNF through a process such as UREX+1a, and convert it into fuel for a fast-spectrum Advanced Burner Reactor (ABR). The key advantage in this scenario is the assumption that recycling of TRU in the ABR (through pyroprocessing or some other approach), along with a low capture-to-fission probability in the fast reactor's high-energy neutron spectrum, can effectively decrease the decay heat and toxicity of the waste being sent to the repository. The decay heat and toxicity reduction can thus minimize the need for multiple repositories. This report summarizes the work performed by the fuel cycle analysis group at the Idaho National Laboratory (INL) to establish the specific technical capability for performing fast reactor fuel cycle analysis and its application to a high-priority ABR concept. The high-priority ABR conceptual design selected is a metallic-fueled, 1000 MWth SuperPRISM (S-PRISM)-based ABR with a conversion ratio of 0.5. Results from the analysis showed excellent agreement with reference values. The independent model was subsequently used to study the effects of excluding curium from the transuranic (TRU) external feed coming from the LWR SNF and recycling the curium produced by the fast reactor itself through pyroprocessing. Current studies to be published this year focus on analyzing the effects of different separation strategies as well as heterogeneous TRU target systems.
"Based on a recommendation from the Technical Working Group on Fast Reactors, this publication is a regular update of previous publications on fast reactor technology. The publication provides comprehensive and detailed information on the technology of fast neutron reactors. The focus is on practical issues that are useful to engineers, scientists, managers, university students and professors. The main issues of discussion are experience in design, construction, operation and decommissioning, various areas of research and development, engineering, safety and national strategies, and public acceptance of fast reactors. In the summary the reader will find national strategies, international initiatives on innovative (i.e. Generation IV) systems and an assessment of public acceptance as related to fast reactors."--Résumé de l'éditeur.
Sodium Fast Reactors with Closed Fuel Cycle delivers a detailed discussion of an important technology that is being harnessed for commercial energy production in many parts of the world. Presenting the state of the art of sodium-cooled fast reactors with closed fuel cycles, this book:Offers in-depth coverage of reactor physics, materials, design, s
The Generation IV Forum is an international nuclear energy research initiative aimed at developing the fourth generation of nuclear reactors, envisaged to enter service halfway the 21st century. One of the Generation IV reactor systems is the Gas Cooled Fast Reactor (GCFR), the subject of study in this thesis. The Generation IV reactor concepts should improve all aspects of nuclear power generation. Within Generation IV, the GCFR concept specifically targets sustainability of nuclear power generation. The Gas Cooled Fast Reactor core power density is high in comparison to other gas cooled reactor concepts. Like all nuclear reactors, the GCFR produces decay heat after shut down, which has to be transported out of the reactor under all circumstances. The layout of the primary system therefore focuses on using natural convection Decay Heat Removal (DHR) where possible, with a large coolant fraction in the core to reduce friction losses.
Molten Salt Reactors and Thorium Energy, Second Edition is a fully updated comprehensive reference on the latest advances in MSR research and technology. Building on the successful first edition, Tom Dolan and the team of experts have fully updated the content to reflect the impressive advances from the last 5 years, ensuring this book continues to be the go-to reference on the topic. This new edition covers progress made in MSR design, details innovative experiments, and includes molten salt data, corrosion studies and deployment plans. The successful case studies section of the first edition have been removed, expanded, and fully updated, and are now published in a companion title called Global Case Studies on Molten Salt Reactors. Readers will gain a deep understanding of the advantages and challenges of MSR development and thorium fuel use, as well as step-by-step guidance on the latest in MSR reactor design. Each chapter provides a clear introduction, covers technical issues and includes examples and conclusions, while promoting the sustainability benefits throughout. A fully updated comprehensive handbook on Molten Salt Reactors and Thorium Energy, written by a team of global experts Covers MSR applications, technical issues, reactor types and reactor designs Includes 3 brand new chapters which reflect the latest advances in research and technology since the first edition published Presents case studies on molten salt reactors which aid in the transition to net zero by providing abundant clean, safe energy to complement wind and solar powe
Proceedings of an International Conference organized by the British Nuclear Energy Society and co-sponsored by the Royal Society of Chemistry and the Institution of Metallurgists LONDON, 9-12 NOVEMBER 1981