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This book provides an interdisciplinary review of one of the great unsolved mysteries that has fascinated scientists for over 150 years: the origin of chirality in biomolecules. It was Pasteur who first initiated the search for a deterministic theory to explain the 'handedness' of biomolecules. His theory, that a 'dissimetric' force was involved, was correct in essence but he never saw the fruits of his labour. Current thinking tells us that asymmetry in the universe has its origins in the forces that unfolded after the Big Bang and, more specifically, the weak force. Being 'left handed', the weak force imprinted its signature on the evolving Universe. However, at the molecular level, the weak force does not provide a straightforward explanation of biomolecular homochirality. In fact, it is yet to be proved beyond doubt that a causal link exists at all. Many alternative theories have been put forward, some of them resting on solid ground, but all lacking definitive experimental evidence to back them up. Some postulate that the handedness of molecules in the biosphere arose by chance but this is hard to test. Others rely on discovering life on similar planets and making comparisons with Earth. Alternative theories have emerged from a range of backgrounds including geology, biology, chemistry, physics and astronomy. Current advances in fields as diverse as space exploration, prebiotic chemistry and high-energy physics may help to provide an answer. Important pieces of information will come from observations at the two frontiers of science: outer space and the subatomic world. Observation of distant planets, galaxies, and even actual sampling of celestial objects from beyond the solar system are projects currently underway. At the other end of the spectrum, there are experiments that study the elemental properties of matter, such as symmetry, and interactions with the fundamental forces. All these efforts will render their fruits soon. This volume unifies all the theories of the origin of biomolecular homochirality together in one source. The various chapters focus on chance mechanisms, physical forces such as the 'weakinteraction', fluid dynamics, amplification of chirality, the organic contents of meteorites and comets and, finally, the physical view of an intrinsically asymmetric universe. This complete, interdisciplinary review of an intriguing subject condenses a large and disparate range of contributions from journals in almost every scientific field. The various theories have been organized, interrelated and explained in a unified way. One of the book's strengths is its extensive use of graphic material to aid understanding the many subjects covered. It is fundamental, comprehensive and structured to be accessible for educational purposes.
This book provides an interdisciplinary review of one of the great unsolved mysteries that has fascinated scientists for over 150 years: the origin of chirality in biomolecules. Current advances in fields as diverse as space exploration, prebiotic chemistry and high-energy physics may help to provide an answer. Important pieces of information will come from observations at the two frontiers of science: outer space and the subatomic world. Observation of distant planets, galaxies, and even actual sampling of celestial objects from beyond the solar system are projects currently underway. At the other end of the spectrum, there are experiments that study the elemental properties of matter, such as symmetry, and interactions with the fundamental forces. Completely revised and updated this new edition once again unifies all the theories of the origin of biomolecular homochirality together in a single source. This complete, interdisciplinary review of an intriguing subject condenses a large and disparate range of contributions from journals in almost every scientific field. The various theories have been organized, interrelated and explained in a unified way. It is fundamental, comprehensive and structured to be accessible for educational purposes.
Amplification of Chirality presents critical reviews of the present position and future trends in modern chemical research. The book contains short and concise reports on chemistry. Each is written by the world renowned experts. Still valid and useful after 5 or 10 years, more information as well as the electronic version of the whole content available at: springerlink.com.
"How did life originate and why were left-handed molecules selected for its architecture?" This question of high public and interdisciplinary scientific interest is the central theme of this book. It is widely known that in processes triggering the origin of life on Earth, the equal occurrence, the parity between left-handed amino acids and their right-handed mirror images, was violated. The balance was inevitably tipped to the left – as a result of which life's proteins today exclusively implement the left form of amino acids. Written in an engaging style, this book describes how the basic building blocks of life, the amino acids, formed. After a comprehensible introduction to stereochemistry, the author addresses the inherent property of amino acids in living organisms, namely the preference for left-handedness. What was the cause for the violation of parity of amino acids in the emergence of life on Earth? All the fascinating models proposed by physicists, chemists and biologist are vividly presented including the scientific conflicts. The author describes the attempt to verify any of those models with the chirality module of the ROSETTA mission, a probe built and launched with the mission to land on a comet and analyse whether there are chiral organic compounds that could have been brought to the Earth by cometary impacts. A truly interdisciplinary astrobiology book, "Amino Acids and the Asymmetry of Life" will fascinate students, researchers and all readers with backgrounds in natural sciences. With a foreword by Henri B. Kagan.
First comprehensive, beginning graduate level book on the emergent science of astrobiology.
Early History of the Recognition of Molecular Biochirality, by Joseph Gal, Pedro Cintas Synthesis and Chirality of Amino Acids Under Interstellar Conditions, by Chaitanya Giri, Fred Goesmann, Cornelia Meinert, Amanda C. Evans, Uwe J. Meierhenrich Chemical and Physical Models for the Emergence of Biological Homochirality, by son E. Hein, Dragos Gherase, Donna G. Blackmond Biomolecules at Interfaces: Chiral, Naturally, by Arántzazu González-Campo and David B. Amabilino Stochastic Mirror Symmetry Breaking: Theoretical Models and Simulation of Experiments, by Celia Blanco, David Hochberg Self-Assembly of Dendritic Dipeptides as a Model of Chiral Selection in Primitive Biological Systems, by Brad M. Rosen, Cécile Roche, Virgil Percec Chirality and Protein Biosynthesis, by Sindrila Dutta Banik, Nilashis Nandi
The year 2003 was the 50th anniversary of the seminal experiment of Stanley Miller. This was a unique opportunity for highlighting the current interest in this most interdisciplinary subject. The leading space agencies: the European Space Agency (ESA) as well as NASA, the American Space Agency, have planned missions that will elucidate some of the still unknown questions underlying research in the origin of life. New results are surpassing our ability to keep well informed: the reviews that we were presented at the Trieste meeting will bring the readers of this well-documented and timely book up to date in this fast-moving area. An important component of the conference was the review of the Cassini-Huygens mission due to arrive in the Saturn system just one year after the conference convened in Trieste. There was particular interest in the status of the experiments that will take place inside the atmosphere of Titan, the large satellite, which is a testing ground for the theories and experiments in the field of chemical evolution. The Jovian system is currently under study with the view of investigating the possibility of life underneath the frozen surface of the Galilean moon Europa; the ESA mission "Mars Express" and Mars Odyssey received special attention. Some of the world leaders in the field gathered in Trieste in September 2003 - that was a most timely date for reviewing recent data and discussing the prospects of future research.
This is the second of a divided two-part softcover edition of the "Lectures in Astrobiology Volume I" containing the sections "General Introduction", "From Prebiotic Chemistry to the Origin of Life on Earth" and "Appendices" including an extensive glossary on Astrobiology. "Lectures in Astrobiology" is the first comprehensive textbook at graduate level encompassing all aspects of the emerging field of astrobiology. Volume I of the Lectures in Astrobiology gathers a first set of extensive lectures that cover a broad range of topics, from the formation of solar systems to the quest for the most primitive life forms that emerged on the Early Earth.
Amino Acids are not only the essential constituents of all living organisms, they also provide vital clues about life in the past. This book of contributed papers updates the science of amino acid geochemistry and replaces a classic but now outdated work, The Biogeochemistry of Amino Acids (out of print). The new book will have a wider focus than its predecessor, covering preservation of ancient proteins and amino acids, diagenesis of proteins and amino acids through geologic time and on short time scales (relevant to the preservation of museum materials), stable isotope geochemistry of proteins and amino acids, amino acid racemization, the origin of life, the stability of amino acids at hgh temperatures and pressures, and extraterrestrial amino acids. The primary audience for this book will be academics and graduate students in geochemistry, organic chemistry, archaeology, geochronology, and stratigraphy, although it will also be of interest to workers in forensic science.