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Metal-Support and Metal-Additive Effects in Catalysis, Volume 11, documents the proceedings of an international symposium organized by the Institut de Recherches sur la Catalyse - CNRS – Villeurbanne and sponsored by the Centre National de la Recherche Scientifique, Ecully (Lyon), September 14-16, 1982. This volume contains 40 manuscripts that cover a wide range of topics. Among these are studies of metal-support interactions involving Pt/Al2O3, Pt/TiO2,Fe/TiO2, Pt/MgO, Rh /Al2O3, and Pt/CeO2 catalysts. There are also separate chapters dealing with ethane, n-butane, and cyclohexane hydrogenolysis; skeletal isomerization of methylpentanes; the catalytic activity and selectivity of noble metals; CO hydrogenation over supported on SiO2, Al2O3, Ti O2,and Zr O2 nickel catalysts; and the role of promoters in Pd catalysts for methanol synthesis. Subsequent chapters cover the poisoning of platinum and nickel by sulfur; C6H6 and CO chemisorption on Pt78Ni22 (111) single crystal alloy; the surface composition of industrial ammonia synthesis catalysts; and the role of alkalis and electronegative promoters on Fe and Ni catalysts.
The production of useful materials and the removal of polluting substances are fundamental to chemical technology, and in this respect catalytic and separation processes play essential roles. In order to cope with increasing demands to find solutions for the shortage of natural resources and global environmental pollution, rapid and significant progress in the technology is required.This book results from the successful seminar on Selective Reactions and Separation, held at Oiso, Japan, in February 1988. The seminar was organised by ASPRONC (the Association for the Progress of New Chemistry) as the fourth in a series of seminars on Frontier Technology. ASPRONC was inaugurated in 1986 and its membership comprises major companies in the chemical industry and various other sectors interested in chemistry. The aim of this seminar was to explore the frontiers of catalytic and separation technology and to discuss the requirements for its future development. The many interesting lectures and active discussions which resulted stimulated the editors to prepare this book. Each lecturer has written a chapter which represents a significantly revised and extended version of his original lecture.The book will appeal to many readers and will undoubtedly help to make a positive contribution to the future development of chemical technology.
These proceedings are based on the third of a series of symposia devoted to the use of catalysis for the depollution of exhaust gases of motor vehicles. Although catalysts have been used for this purpose for some thirty years, the subject is still very topical because of its economic impact. The increasing number of submitted, accepted and published papers amply attests to this fact.
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In view of the substantial progress made in the last decade in the fields of zeolites and related materials it was decided to go for an extended 2nd Edition of "Introduction to Zeolite Science and Practice". Unfortunately - as often is the case - this process took more time than expected by the Editors.In the mean time some new texts on zeolites were issued. Nevertheless, the combination of data, discussion and dedication provided by the present book is a unique coverage of the field, in the opinion of the Editors.In the present Edition the number of chapters rose from 16-22. The contributions can be divided into three categories: updated chapters by the original authors, updated chapters by an expanded or new team of authors and completely new chapters. This 2nd Edition also contains new chapters on "Zeolite-based supramolecular assemblies" (by Dirk De Vos and Pierre Jacobs, experts in this area) and on "The use of bulky probe molecules" (by Paul Kunkeler, Roger Downing and one of the Editors).Finally, the super large pore zeolites and the fast growing area of ordered mesoporous materials are dealt with by Eelco Vogt, Charlie Kresge and and Jim Vartuli. The latter two authors belong to the discoverers of the M41S family of mesoporous materials.
Reaction Kinetics and the Development and Operation of Catalytic Processes is a trendsetter. The Keynote Lectures have been authored by top scientists and cover a broad range of topics like fundamental aspects of surface chemistry, in particular dynamics and spillover, the modeling of reaction mechanisms, with special focus on the importance of transient experimentation and the application of kinetics in reactor design. Fundamental and applied kinetic studies are well represented. More than half of these deal with transient kinetics, a new trend made possible by recent sophisticated experimental equipment and the awareness that transient experimentation provides more information and insight into the microphenomena occurring on the catalyst surface than steady state techniques. The trend is not limited to purely kinetic studies since the great majority of the papers dealing with reactors also focus on transients and even deliberate transient operation. It is to be expected that this trend will continue and amplify as the community becomes more aware of the predictive potential of fundamental kinetics when combined with detailed realistic modeling of the reactor operation.
Crystalline solids with highly structured micro-scale pores are called zeolites. Their well-defined structure and large contact surface make them extremely useful as catalysts. Their most common use is in washing powders. Different features are caused by the shape and size of the pores and the presence of different metals in the crystal structure. Research is conducted both towards better understanding of the relations between form and function and towards identifying new possible uses.This title presents a collection of contributions from internationally renowned researchers in the field of the Science and Technology of micro and mesoporous materials. The aim of the conference is to create an international forum where researchers from academia as well as from industry can discuss ideas and evaluate the impact of zeolites, and other porous materials, on new technologies at the beginning of the new millennium.·Gives the most recent developments in the origin, synthesis and characterisation of zeolitic materials·Outlines the impact and application of zeolites in various industrial processes·An adjourned state of art in the field of zeolites and other porous materials
This book offers an overview of the state of the art in the field of DeNOx catalysis in order to focus novel orientations, new technological developments, from laboratory to industrial scale. A particular attention has been paid towards the implementation of catalytic processes for minimising NOx emissions either from stationary or mobile sources under lean condition to meet future standard regulations of NOx emissions. In the first part of this book, critical aspects reported in the literature which usually make difficult the achievement of efficient catalytic technologies in those conditions are summarised and analysed in order two separate new perspectives. The second part deals with fundamental aspects at molecular level. A better understanding of the reactions involved under unsteady-state conditions is probably a pre-requisite step for improving the performances of the actual processes or developing original ones. The development of powerful in situ spectroscopic techniques is of fundamental interest for kinetic modelling. Correlations between spectroscopic and kinetic data with those obtained from theoretical calculations are reported. Some illustrations emphasise the fact that these comparisons may help in determining the nature of the catalytic active sites and building predictive tools for simulations under running conditions. The latter part of this book will be illustrated by different practical approaches covering various aspects related to the catalysts preparation and the development of alternative technologies which include industrial considerations.- New technological developments for investigating catalytic reactions in transient conditions (in situ and operando spectroscopic techniques)- Concerted approaches in DeNOx catalysis - How academic aspects (kinetic, in situ spectroscopic measurements) can provide useful information for practical applications- Comparison of different approaches provided by academic and industrial partners
Between the area known as surface science (which mainly deals with single crystal surfaces) and the vast area of the surface properties of dispersed solids (knowledge of which is widely applied in catalysis and materials science) there is still a remarkably wide, although gradually decreasing, gap. Because fundamental physico-chemical problems are involved, this borderline area needs to be explored. With this objective, the Trieste meeting brought together specialists with a variety of origins and backgrounds, with the aim of stimulating the growth of our knowledge in this area.This proceedings volume contains ninety-three papers, comprising plenary lectures, short communications, and poster contributions on the applications of physical and theoretical methods to perfect and dispersed (microcrystalline and amorphous) metals, oxides, and mixed systems. Special emphasis is given to metal-support interfaces.The book thus provides a wealth of up-to-date information on a topic of current interest which will be of value to researchers who use chemical and/or physical methods for the study of surfaces.
This 3rd volume of 'Gas Engineering' introduces the concept of liquefied natural gas and the concept gas-to-liquids and also presents a review of the uses of gas streams and the effects of the various gases on the environment. This volume also describes the properties gas streams as they are related to corrosion effects are also presented. The relationship of the properties of gas streams as they affect corrosion such as carburization and metal dusting as well as corrosion in steel and other materials used in refinery technology are also presented and the book summarizes key findings into corrosion processes in gas-processing equipment as well as corrosion in offshore structures. Each book contains references at the end of chapter which include information from the open literature and meeting proceedings to give a picture of where the gas processing technology stands as well as indicate some relatively new technologies that could become important in the future. Also, each book also contains a comprehensive glossary. The books are written in an easy-to-read style and offer a ready-at-hand (one-stop-shopping) guide to the many issues that are related to the engineering aspects of the properties and processing of natural gas as well as the effects of natural gas on various ecosystems as well as to pollutant mitigation and clean-up. The books present an overview, with a considerable degree of detail of the various aspects of natural gas technology. Any chemistry presented in the books is used as a means of explanation of a particular point but is maintained at an elementary level.