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A highly coveted objective of modern materials science is to optimize multiple coupled functionalities in the same single phase material and control the cross-response via multiple external fields. One important example of such multi-functionality are multiferroic materials where two or more ferroic properties are intrinsically coupled. They include, among others, the magneto-electric and magneto-structural materials, which are well understood at the nano- and continuum length (and time) scales. The next emerging frontier is to connect these two limiting scales by probing the mesoscale physics of these materials. This book not only attempts to provide this connection but also presents the state-of-the art of the present understanding and potential applications of many related complex multifunctional materials. The main emphasis is on the multiscale bridging of their properties with the aim to discover novel properties and applications in the context of materials by design. This interdisciplinary book serves both graduate students and expert researchers alike.
Synthesizing specific clusters as a component of useful nanostructures or controlling them as an assembly of nanocomposites is the ultimate aim. In order to understand how to synthesize individual clusters or to investigate its properties, a variety of first-principles and empirical calculations and related computer simulations have been performed alongside numerous experiments.
This book supplies a systematic description of the preparation, characterization, and manipulation of cluster beams for the synthesis of nanocrystalline materials. It addresses all issues relevant to the realization of nanophase structures, providing an excellent introduction for scientists working in different fields. Particular emphasis is placed on using the technique for nanostructured materials and on explaining the role of cluster beams within the context of other experimental techniques in surface-science.
Due to the interaction with the contact medium, the properties of clusters may change or even disappear. Thus the physics of cluster-on-surface systems -- the main subject of this book -- is of fundamental importance. The book addresses a wide audience, from the newcomer to the expert. Starting from fundamental concepts of adsorbate-surface interactions, the modification of electronic properties through electron confinement, and concepts of cluster production, it elucidates the distinct properties of the new metallic nanostructures.
The emergence and spectacularly rapid evolution of the field of atomic and molecular clusters are among the most exciting developments in the recent history of natural sciences. The field of clusters expands into the traditional disciplines of physics, chemistry, materials science, and biology, yet in many respects it forms a cognition area of its own. This book presents a cross section of theoretical approaches and their applications in studies of different cluster systems. The contributions are written by experts in the respective areas. The systems discussed range from weakly (van der Waals) bonded, through hydrogen- and covalently bonded, to semiconductor and metallic clusters. The theoretical approaches involve high-level electronic structure computations, more approximate electronic structure treatments, use of semiempirical potentials, dynamical and statistical analyses, and illustrate the utility of both classical and quantum mechanical concepts.
Clusters as mesoscopic particles represent an intermediate state of matter between single atoms and solid material. The tendency to miniaturise technical objects requires knowledge about systems which contain a "small" number of atoms or molecules only. This is all the more true for dynamical aspects, particularly in relation to the qick development of laser technology and femtosecond spectroscopy. Here, for the first time is a highly qualitative introduction to cluster physics. With its emphasis on cluster dynamics, this will be vital to everyone involved in this interdisciplinary subject. The authors cover the dynamics of clusters on a broad level, including recent developments of femtosecond laser spectroscopy on the one hand and time-dependent density functional theory calculations on the other.
Clusters represent a new class of materials with totally new applications. This broad-ranging book presents and evaluates some of the latest developments in this area. The authors present some of the important recent advances made through the use of new experimental techniques and theoretical approaches.
Cluster Materials is the fourth volume of the highly successful series Advances in Metal and Semiconductor Clusters. In this volume the focus is on the properties of clusters which determine their potential applications as new materials. Metal and semiconductor clusters have been proposed as precursors for materials or as actual materials since the earliest days of cluster research. In the last few years, a variety of techniques have made it possible to produce clusters in sizes varying from a few atoms up to several thousand atoms. While some measurements are performed in the gas phase on non-isolated clusters, many cluster materials can now be isolated in macroscopic quantities and more convenient studies of their properties become possible. In this volume the authors focus on measurement of optical, electronic, magnetic, chemical and mechanical properties of clusters or of cluster assemblies. All of these properties must fall into acceptable ranges of behaviour before useful materials composed of clusters can be put into practical applications. As evidenced by the various work described here, the realisation of practical products based on cluster materials seems to be approaching rapidly.
Advances in Quantum Chemistry publishes surveys of current developments in the rapidly developing field of quantum chemistry--a field that falls between the historically established areas of mathematics, physics, chemistry, and biology. With invited reviews written by leading international researchers, each presenting new results, this quality serial provides a single vehicle for following progress in this interdisciplinary area.
Mesoscopic physics refers to the physics of structures larger than a nanometer (one billionth of a meter) but smaller than a micrometer (one millionth of a meter). This size range is the stage on which the exciting new research on submicroscopic and electronic and mechanical devices is being done. This research often crosses the boundary between physics and engineering, since engineering such tiny electronic components requires a firm grasp of quantum physics. Applications for the future may include such wonders as microscopic robot surgeons that travel through the blood stream to repair clogged arteries, submicroscopic actuators and builders, and supercomputers that fit on the head of a pin. The world of the future is being planned and built by physicists, engineers, and chemists working in the microscopic realm. This book can be used as the main text in a course on mesoscopic physics or as a supplementary text in electronic devices, semiconductor devices, and condensed matter physics courses. For this new edition, the author has substantially updated and modified the material especially of chapters 3: Dephasing, 8: Noise in mesoscopic systems, and the concluding chapter 9.