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This paper provides an overview of the photophysical processes and analytical applications of high-resolution luminescence spectroscopy using solid samples. Experimental results are discussed within the framework of a theoretical model involving isolated guest molecules weakly interacting with the host solid substrate. Examples are given to illustrate the spectral structure of luminescence spectra exhibiting zero-phonon lines and phonon wings. Effects of experimental parameters such as temperature are discussed. Analytical considerations on the various laser-based techniques in fluorescence and phosphorescence analysis are reviewed and discussed in detail.
This book presents an account of the course "Spectroscopy of Solid-State Laser-Type Materials" held in Erice, Italy, from June 16 to 30, 1985. This meeting was organized by the International School of Atomic and Molecular Spectroscopy of the "Ettore Majorana" Centre for Scientific Culture. The objective of the course was to present and examine the recent advances in spectroscopy and theoretical modelling relevant to the interpretation of luminescence and laser phenomena in several classes of solid-state materials. The available solid-state matrices (e.g. halides, oxides, glasses, semiconductors) and the full range of possible activators (transition ions, rare earth ions, post-transition ions, actinides, color centres) were considered. By bringing together specialists in the fields of solid-state luminescence and of solid-state laser materials, this course provided a much-needed forum for the critical . assessment of past developments in the R&D of solid-state lasers. Additional objectives of the meeting were to identify new classes of host/activator systems that show promise of laser operation; to alert researchers in solid-state luminescence to current technological needs for solid-state tunable lasers operating in the visible and infrared spectral regions; and generally to provide the scientific background for advanced work in solid state lasers. A total of 71 participants came from 54 laboratories and 21 nations (Austria, Belgium, Canada, F.R. of Germany, France, Greece, Ireland, Israel, Italy, the Netherlands, P.R. of China, Poland, Rumania, Sweden, Switzerland, South Korea, Spain, Turkey, United Kingdom, U.S.A. and U.S.S.R.).
Solid-state laser and luminescent materials activated by rare-earth or transition metals ions are widely used for solid-state lasers, luminescent lamps, flat displays, optical fibre communication systems, and other photonic devices. The unique solid-state electronic properties enable the activators in solids to emit photons efficiently in visible and IR regions. The rapid advances in both materials science and optoelectronics, particularly, the development of new methods of material synthesis and device fabrication, have been stimulating the growing interests in the deep insights of spectroscopic properties of solid-state laser and luminescent materials. This book brings together essential and practical knowledge of spectroscopic physics. This includes, atomic spectroscopy, mathematical theory, rare earth ions in materials, light emission and absorption, spectral properties, non-radiative transitions and energy migration.
Laser induced breakdown spectroscopy (LIBS) is basically an emission spectroscopy technique where atoms and ions are primarily formed in their excited states as a result of interaction between a tightly focused laser beam and the material sample. The interaction between matter and high-density photons generates a plasma plume, which evolves with time and may eventually acquire thermodynamic equilibrium. One of the important features of this technique is that it does not require any sample preparation, unlike conventional spectroscopic analytical techniques. Samples in the form of solids, liquids, gels, gases, plasmas and biological materials (like teeth, leaf or blood) can be studied with almost equal ease. LIBS has rapidly developed into a major analytical technology with the capability of detecting all chemical elements in a sample, of real- time response, and of close-contact or stand-off analysis of targets. The present book has been written by active specialists in this field, it includes the basic principles, the latest developments in instrumentation and the applications of LIBS . It will be useful to analytical chemists and spectroscopists as an important source of information and also to graduate students and researchers engaged in the fields of combustion, environmental science, and planetary and space exploration. * Recent research work* Possible future applications* LIBS Principles
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In this volume we have attempted to present a concise survey of the spectroscopic properties of insulators as derived from the application of tunable laser spectro scopic techniques. As has been the case in gaseous atomic spectroscopy, the use of tunable lasers has allowed the extension and the refmement of optical measure ments in the condensed phases to unprecedented resolutions in the frequency and temporal domains. In turn, this firmer base of empirical fmdings has led to a more sophisticated theoretical understanding of the spectroscopy of optically excited states with major modifications being apparent in the area of their dynamic be havior. Yet the revivalistic nature of these advances implies that additional advan ces are to be expected as the techniques and developments outlined in this volume are put to widespread use. Regardless, it is our hope and that of our distinguished colleagues in this venture that the reviews presented here will be useful to neo phytes and veterans to this field alike - to the former as a laissez-passer into solid-state spectroscopy, to the latter as a useful synopsis and reference of recent developments. We have also attempted to expose the reader to the concept that optically active materials, be they organic or inorganic, as universality would require, be have in a like manner and, though terminology may vary in detail, the outline and general features of all insulators remain constant.
Using lasers to induce and probe surface processes has the advantages of quantum state specificity, species selectivity, surface sensitivity, fast time-resolution, high frequency resolution, and accessibility to full pressure ranges. These advantages make it highly desirable to use light to induce, control, or monitor surface chemical and physical processes. Recent applications of laser based techniques in studying surface processes have stimulated new developments and enabled the understanding of fundamental problems in energy transfer and reactions. This volume will include discussions on spectroscopic techniques, energy transfer, desorption dynamics, and photochemistry.
Laser-based optical spectroscopies are powerful and versatile techniques that are continuing to evolve and find new applications. This book presents reviews of recent progress in our understanding of the spectra and dynamical processes of optically excited states of condensed matter, focusing on the advances made possible by the application of laser-based optical spectroscopies. Reviews are given of the optical properties of crystalline and amorphous semiconducting materials and structures, the properties of defect centers in insulators, two-photon nonlinear processes in insulators, optical energy diffusion in inorganic materials, and relaxation in organic materials. The individual chapters emphasize the methodology common to the various investigations. The volume is designed to be suitable as an introduction to applied laser spectroscopy of solids, as well as providing an update on the status of the field.
The first in-depth treatment of the synthesis, processing, and characterization of nanomaterials using lasers, ranging from fundamentals to the latest research results, this handy reference is divided into two main sections. After introducing the concepts of lasers, nanomaterials, nanoarchitectures and laser-material interactions in the first three chapters, the book goes on to discuss the synthesis of various nanomaterials in vacuum, gas and liquids. The second half discusses various nanomaterial characterization techniques involving lasers, from Raman and photoluminescence spectroscopies to light dynamic scattering, laser spectroscopy and such unusual techniques as laser photo acoustic, fluorescence correlation spectroscopy, ultrafast dynamics and laser-induced thermal pulses. The specialist authors adopt a practical approach throughout, with an emphasis on experiments, set-up, and results. Each chapter begins with an introduction and is uniform in covering the basic approaches, experimental setups, and dependencies of the particular method on different parameters, providing sufficient theory and modeling to understand the principles behind the techniques.