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Generation of reproducible attosecond (10−18s) pulses is an exciting goal: in the same way as femtosecond pulses were used to make "movies" of the atomic motion in molecules, attosecond pulses could "uncover" the motion of electrons around nuclei. In this dissertation, we have suggested new ideas that will allow improving one scheme for obtaining such ultra-short pulses: The molecular modulation technique. In a theoretical proposal called Raman Additive technique, we have suggested a method that will allow (with a proper phase stabilization of generated sidebands) to obtain reproducible waveforms of arbitrary shape. An exciting range of possibilities could open up - not only for absolute phase control or sub-cycle shape control, but also for investigation of multiphoton ionization rates as a function of the sub-cycle shape. We have elaborated on the latter subject in another theoretical project, where we have exploited the unique feature of such ultrashort laser pulses, which is synchronization with molecular motion (rotational or vibrational), in order to investigate photoionization of molecules. From experimental point of view, a different construction of driving lasers than previously employed led to establishment of larger molecular coherences at higher operating pressure than in previous experiments. This resulted in simultaneous generation of rotational and vibrational sidebands with only two fields applied. In another experimental proposal using rotational transition in deuterium we have shown that employing a hollow waveguide instead of normal Raman cell improves the efficiency of the generation process. By optimizing gas pressure and waveguide geometry to compensate the dispersion, the method can be extended to efficiently generate Raman sidebands at a much lower energy of driving fields than previously employed. At the end, a very exciting possibility for controlling the molecular motion in a Raman driven system will be shown. Based on the interference effects (EIT like) that take place inside of a molecule, selectivity of different degrees of freedom can be achieved (for example switching from rotational-vibrational motion to pure rotational).
Frontiers and Advances in Molecular Spectroscopy once again brings together the most eminent scientists from around the world to describe their work at the cutting-edge of molecular spectroscopy. Much of what we know about atoms, molecules and the nature of matter has been obtained using spectroscopy over the last one hundred years or so. Going far beyond the topics discussed in Jaan Laane’s earlier book on the subject, these chapters describe new methodologies and applications, instrumental developments and theory, which are taking spectroscopy into still new frontiers. The robust range of topics once again demonstrates the wide utility of spectroscopic techniques. New topics include ultrafast spectroscopy of the transition state, SERS/far-uv spectroscopy, femtosecond coherent anti-Stokes Raman spectroscopy, high-resolution laser induced fluorescence spectroscopy, Raman spectroscopy and biosensors, vibrational optical activity, ultrafast two-dimensional spectroscopy, biology with x-ray lasers, isomerization dynamics and hydrogen bonding, single molecule imaging, spectra of intermediates, matrix isolation spectroscopy and more. Covers spectroscopic investigations on the cutting edge of science Written and edited by leading experts in their respective fields Allows researchers to access a broad range of essential modern spectroscopy content from a single source rather than wading through hundreds of scattered journal articles
Much of what we know about atoms, molecules, and the nature of matter has been obtained using spectroscopy over the last one hundred years or so. In this book we have collected together twenty chapters by eminent scientists from around the world to describe their work at the cutting edge of molecular spectroscopy. These chapters describe new methodology and applications, instrumental developments, and theory which is taking spectroscopy into new frontiers. The range of topics is broad. Lasers are utilized in much of the research, but their applications range from sub-femtosecond spectroscopy to the study of viruses and also to the investigation of art and archeological artifacts. Three chapters discuss work on biological systems and three others represent laser physics. The recent advances in cavity ringdown spectroscopy (CRDS), surface enhanced Raman spectroscopy (SERS), two-dimensional correlation spectroscopy (2D-COS), and microwave techniques are all covered. Chapters on electronic excited states, molecular dynamics, symmetry applications, and neutron scattering are also included and demonstrate the wide utility of spectroscopic techniques. Provides comprehensive coverage of present spectroscopic investigations Features 20 chapters written by leading researchers in the field Covers the important role of molecular spectroscopy in research concerned with chemistry, physics, and biology
"Extreme Photonics & Applications" arises from the 2008 NATO Advanced Study Institute in Laser Control & Monitoring in New Materials, Biomedicine, Environment, Security and Defense. Leading experts in the manipulation of light offered by recent advances in laser physics and nanoscience were invited to give lectures in their fields of expertise and participate in discussions on current research, applications and new directions. The sum of their contributions to this book is a primer for the state of scientific knowledge and the issues within the subject of photonics taken to the extreme frontiers: molding light at the ultra-finest scales, which represents the beginning of the end to limitations in optical science for the benefit of 21st Century technological societies. Laser light is an exquisite tool for physical and chemical research. Physicists have recently developed pulsed lasers with such short durations that one laser shot takes the time of one molecular vibration or one electron rotation in an atom, which makes it possible to observe their internal electronic structure, thereby enabling the study of physical processes and new chemical reactions. In parallel, advances in micro- and nano-structured photonic materials allow the precise manipulation of light on its natural scale of a wavelength. Photonic crystals, plasmons and related metamaterials - composed of subwavelength nanostructures - permit the manipulation of their dispersive properties and have allowed the experimental confirmation of bizarre new effects such as slow light and negative refraction. These advances open a vista on a new era in which it is possible to build lasers and engineer materials to control and use photons as precisely as it is already possible to do with electrons. http://www.photonics.uottawa.ca/nato-asi-2008/
The papers in this volume cover the major areas of research activity in the field of ultrafast optics at the present time, and they have been selected to provide an overview of the current state of the art. The purview of the field is the methods for the generation, amplification, and characterization of electromagnetic pulses with durations from the pieo-to the attosecond range, as well as the technical issues surrounding the application of these pulses in physics, chemistry, and biology. The contributions were solicited from the participants in the Ultrafast Optics IV Conference, held in Vienna, Austria, in June 2003. The purpose of the conference is similar to that of this book: to provide a forum for the latest advances in ultrafast optical technology. Ultrafast light sources provide a means to observe and manipulate events on the scale of atomic and molecular dynamics. This is possible either through appropriate shaping of the time-dependent electrie field, or through the ap plication of fields whose strength is comparable to the binding forces of the electrons in atoms and molecules. Recent advances discussed here include the generation of pulses shorter than two optical cycles, and the ability to measure and to shape them in all degrees of freedom with unprecedented 2 21 2 precision, and to amplify them to the Zettawatt/cm (10 W /cm ) range.
Deals with both the ultrashort laser-pulse technology in the few- to mono-cycle region and the laser-surface-controlled scanning-tunneling microscopy (STM) extending into the spatiotemporal extreme technology. The former covers the theory of nonlinear pulse propagation beyond the slowly-varing-envelope approximation, the generation and active chirp compensation of ultrabroadband optical pulses, the amplitude and phase characterization of few- to mono-cycle pulses, and the feedback field control for the mono-cycle-like pulse generation. In addition, the wavelength-multiplex shaping of ultrabroadband pulses, and the carrier-phase measurement and control of few-cycle pulses are described. The latter covers the CW-laser-excitation STM, the femtosecond-time-resolved STM and atomic-level surface phenomena controlled by femtosecond pulses.
The most comprehensive and up-to-date optics resource available Prepared under the auspices of the Optical Society of America, the five carefully architected and cross-referenced volumes of the Handbook of Optics, Third Edition, contain everything a student, scientist, or engineer requires to actively work in the field. From the design of complex optical systems to world-class research and development methods, this definitive publication provides unparalleled access to the fundamentals of the discipline and its greatest minds. Individual chapters are written by the world's most renowned experts who explain, illustrate, and solve the entire field of optics. Each volume contains a complete chapter listing for the entire Handbook, extensive chapter glossaries, and a wealth of references. This pioneering work offers unprecedented coverage of optics data, techniques, and applications. Volume IV covers optical properties of materials, nonlinear optics, and quantum optics.