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Mathematical methods play a significant role in the rapidly growing field of nonlinear optical materials. This volume discusses a number of successful or promising contributions. The overall theme of this volume is twofold: (1) the challenges faced in computing and optimizing nonlinear optical material properties; and (2) the exploitation of these properties in important areas of application. These include the design of optical amplifiers and lasers, as well as novel optical switches. Research topics in this volume include how to exploit the magnetooptic effect, how to work with the nonlinear optical response of materials, how to predict laser-induced breakdown in efficient optical devices, and how to handle electron cloud distortion in femtosecond processes.
Nonlinear Optical Properties of Organic Molecules and Crystals, Volume 1 discusses the nonlinear optical effects in organic molecules and crystals, providing a classical distinction between quadratic and cubic processes. This book begins with a general overview of the basic properties of organic matter, followed by a review on the benefits derived from quantum-chemistry-based models and growth and characterization of high quality, bulk organic crystals and waveguided structures. A case study focusing on a specific material, namely urea, which exemplifies a situation in which transparency in the UV region has been purposely traded for nonlinear efficiency is also deliberated. This text concludes with a description of a type of trade-off between the unpredictable orientation of molecules in crystalline media, polarity of liquid-crystalline structures, and dominant electronic contribution to the electro-optic effect. This publication is beneficial to solid-state physicists and chemists concerned with nonlinear optical properties of organic molecules and crystals.
Organic Nonlinear Optical Materials provides an extensive description of the preparation and characterization of organic materials for applications in nonlinear and electro-optics. The book discusses the fundamental optimization and practical limitations of a number of figures of merit for various optical parameters and gives a clinical appraisal of the potential of organic materials for applicators in optical technology. Among the topics addressed are the basic molecular design of ;nonlinear optical chromophores, fundamentals and novel techniques of organic crystal growth, preparation and characterization of Langmuir-Blodgett and polymer films, experimental methods for determining microscopic and macroscopic optical properties. Also included is a discussion of first results of the photorefractive effect in organic crystals and the potential of organics for photorefractive applications, as well as an extensive review of published linear and nonlinear optical measurement of organic materials.
This volume exposes the chemistry community to the critical role that chemistry can and must play in nonlinear optics research. In addition, it brings together those researchers who synthesize and characterize materials from a variety of systems, with those who build devices, giving chemists, physicists, and engineers a greater appreciation for the opportunities that lie ahead in understanding and developing nonlinear optical materials. The volume begins with a discussion of polarizability and hyperpolarizability from the view of a chemist. Tutorial chapters dealing with the fundamental structures and properties of second- and third-order nonlinear optical materials, measurement and characterization of these systems, theoretical considerations, application of these systems to devices, and overviews of the current state of affairs in both organic and inorganic nonlinear optical materials follow.
Nonlinear Optical Crystals contains the most complete and up-to-date reference material on properties of nonlinear optical crystals including: Traditional and specific applications The mathematical formulas necessary for the calculation of the frequency conversion process A survey of 63 nonlinear optical crystals containing more than 1500 different references with full titles Recent applications of common and novel nonlinear materials, including quasi-phase matching Special consideration for periodically-poled and self-frequency-doubling materials Significant amount of crystallophysical, thermophysical, spectroscopic, electro-optic and magneto-optic information
UV-VIS spectroscopy is one of the oldest methods in molecular spectroscopy. The definitive formulation of the Bouguer-Lambert Beer law in 1852 created the basis for the quantitative evaluation of absorption measurements at an early date. This led firstly to colorimetry, then to photometry and finally to spectrophotometry. This evolution ran parallel with the development of detectors for measuring light intensities, i.e. from the human eye via the photo element and photocell, to the photomultiplier and from the photo graphic plate to the present silicon-diode detector both of which allow simultaneous measurement of the complete spectrum. With the development of quantum chemistry, increasing atten tion was paid to the correlation between light absorption and the structure of matter with the result that in recent decades a number of excellent discussions of the theory of electronic spectroscopy (UV-VIS and luminescence sp,~ctroscopy) have been published. Consequently, this extremely ivteresting aspect of molecular spec troscopy has dominated the teaching of the subject both in my own lectures and those of others. However, it is often overlooked that, in addition to the theory, applications of spectroscopic methods are of particular interest to scientists. For this reason, a lecture series about electronic spectroscopy given in the Institute for Physical Chemistry at the Heinrich-Heine-University in Dusseldorf was supplemented by one about "UV-VIS spectroscopy and its applications". This formed the basis of the present book.
Synthesis, Modelling and Characterization of 2D Materials and Their Heterostructures provides a detailed discussion on the multiscale computational approach surrounding atomic, molecular and atomic-informed continuum models. In addition to a detailed theoretical description, this book provides example problems, sample code/script, and a discussion on how theoretical analysis provides insight into optimal experimental design. Furthermore, the book addresses the growth mechanism of these 2D materials, the formation of defects, and different lattice mismatch and interlayer interactions. Sections cover direct band gap, Raman scattering, extraordinary strong light matter interaction, layer dependent photoluminescence, and other physical properties. - Explains multiscale computational techniques, from atomic to continuum scale, covering different time and length scales - Provides fundamental theoretical insights, example problems, sample code and exercise problems - Outlines major characterization and synthesis methods for different types of 2D materials
Describing progress achieved in the field of nonlinear optics and nonlinear optical materials, the Handbook treats selected topics such as photorefractive materials, third-order nonlinear optical materials and organic nonlinear optical crystals, as well as electro-optic polymers. Applications of photorefractive materials in optical memories, optical processing, and guided-wave nonlinear optics in hotorefractive waveguides are described. As light will play a more and more dominant role as an information carrier, the review of existing and new materials given here makes this a keystone book in the field.
Presents a clear systematic molecular-based description of nonlinear optical polarization analysis of chemical and biological assemblies.
: This book is based on research conducted on the growth and characterization of nonlinear optical crystals. Due to the significance of crystals in contemporary technology, crystal growth has been the focus of extensive research in both solid-state physics and materials science. This book serves as an introduction to the growth phenomena, specifics of growth processes, nonlinear optical phenomena, and characterization methods that are being used for the analysis. The book is divided into three chapters: The first chapter focuses on the experimental techniques of crystal growth. It outlines the several ways that crystals grow based on the phases they go through, such as solid-solid phase transition, liquid-solid phase transformation, and vapour-solid phase transformation. The optimization methods for growing high-quality single crystals are thoroughly presented. The benefits and drawbacks of methods of growth are reviewed. The second chapter explains the theory of nonlinear optical phenomena. The selection criteria for nonlinear optical materials are reviewed. The history of nonlinear optics and the various types of nonlinear optical materials are discussed. The role of amino acids in the formation of nonlinear optical crystals is well explained. The third chapter discusses characterization procedures that are essential in determining the quality of crystals. The several characterization mechanisms including the molecular structure, chemical composition, surface morphology, optical properties, dielectric properties, mechanical behavior, and thermal properties necessary for crystal analysis are described. We hope that this book will be valuable to researchers and students.