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A comprehensive overview of graphene-based membrane materials and its applications.
There is great interest in the novel mass-transport properties of graphene-based membrane materials, especially for environmental applications such as wastewater treatment and reuse, gas separation and water desalination. Graphene-based Membranes for Mass Transport Applications is a comprehensive overview of the research in this area. Starting with current state-of-the-art membrane-based filtration and separation technologies, the book then explores the structure, composition and general properties of graphene-based membranes including nanoporous graphene and graphene oxide followed by the selective mass transport properties of the membranes. The final chapters look at their specific use in barrier applications, purification and separation applications and water desalination. Edited by leading researchers, the book provides an introduction and reference to physicists, chemists, material scientists, chemical engineers and students who are entering or already working in the field of graphene-based membrane materials.
Filtration membranes are required to be thin, robust, energy efficient, and accurate on selectivity. Graphene oxide (GO) is believed to be a potential next generation material for industrial membrane applications because of its unique properties such as strong mechanical strength, excellent aqueous solution processability, and great flexibility for membrane fabrication. Research on the transport models, the separation performance, and the functionalization of GO membranes has been developed. However, many mechanisms of mass transport through GO membranes still remain debatable. In this work, GO was synthesized, and then functionalized with linear amine-terminated poly(ethylene glycol) (PEG) and aluminum ions (Al). The fabrication and characterizations of GO, PEG-GO, and Al-GO membranes were demonstrated in this work. Water and water/ethanol binary mixture transport through GO, PEG-GO, and Al-GO membranes were studied to investigate the permeation and the rejection rates of solvents through GO-based membranes. The total volumetric flux of water/ethanol mixture through GO membranes was inversely proportional to the viscosity of the solvent mixtures. The steric hindrance effect and the interactions between the solvent molecules and the membrane surfaces dominated the rejection rate of ethanol through GO membranes. The functionalization of GO modified the pore size and the porosity of the membranes, resulting in faster permeation of solvents and reduced rejection rates of ethanol through PEG-GO and Al-GO membranes. Deformation of nanochannels within the functionalized GO membranes was observed when the membranes were operated under highly pressurized conditions. Diffusive transport of two charge equivalent and structurally similar ruthenium complex ions Ru(bpy)32+ and iv Ru(phen)32+ through GO, PEG-GO, and Al-GO membranes were also studied. Our data showed high similarity with the results reported previously in the literature, indicating that the GO and functionalized GO membranes used in this work were highly consistent. Due to the enlarged pore sizes and the reduced interactions between ions and the membrane surfaces, the flux of ions through PEG-GO membranes was 300% higher than that through GO membranes. In contrast, permeation of ions through Al-GO membranes was slower than that through GO membranes. The blocked nanopores and the electrostatic repulsion between the intercalated aluminum ions and complex ions were the main reasons for this observation. In addition, the main reason for the significant permeance difference between Ru(bpy)32+ and Ru(phen)32+ ions was confirmed as the steric hindrance effect. This work contributes to the basic research on GO membranes in potential applications. It can be beneficial to the academic laboratories for understanding the mechanism of mass transport through GO-based membranes. These new membrane materials could replace traditional membrane materials in many industrial applications in the future.
This book covers newly emerging two-dimensional nanomaterials which have been recently used for the purpose of water purification. It focuses on the synthesis methods of 2D materials and answers how scientists/engineers/nanotechnologist/environmentalists could use these materials for fabricating new separation membranes and most probably making commercially feasible technology. The chapters are written by a collection of international experts ensuring a broad view of each topic. The book will be of interest to experienced researchers as well as young scientists looking for an introduction into 2D materials-based cross-disciplinary research.
Current Trends and Future Developments on (Bio-) Membranes: Microporous Membrane and Membrane Reactors focuses on the structure, preparation, characterization and applications of microporous membranes and membrane reactors, including transport mechanisms through a range of microporous membranes. It is a key reference text for R&D managers who are interested in the development of gas separation and water/waste treatment technologies, but is also well-suited for academic researchers and postgraduate students working in the broader area of strategic material production, separation and purification. Users will find comprehensive coverage of current methods, their characterization and properties, and various applications in gas separation and water treatment. Reviews gas separation and water treatment processes and relates them to various applications Outlines the use of microporous membranes in gas separations and water treatment Introduces the various types of microporous membranes (graphene, polymeric, etc.) and their mechanism of action Provides simulation models of the various processes
Novel nanoscale materials are now an essential part of meeting the current and future needs for clean water, and are at the heart of the development of novel technologies to desalinate water. The unique properties of nanomaterials and their convergence with current treatment technologies present great opportunities to revolutionize water and wastewater treatment. Nanoscale Materials for Water Purification brings together sustainable solutions using novel nanomaterials to alleviate the physical effects of water scarcity. This book covers a wide range of nanomaterials, including noble metal nanoparticles, magnetic nanoparticles, dendrimers, bioactive nanoparticles, polysaccharidebased nanoparticles, nanocatalysts, and redox nanoparticles for water purification. Significant properties and characterization methods of nanomaterials such as surface morphology, mechanical properties, and adsorption capacities are also investigated Explains how the unique properties of a range of nanomaterials makes them important water purification agents Shows how the use of nanotechnology can help create cheaper, more reliable, less energy-intensive, more environmentally friendly water purification techniques Includes case studies to show how nanotechnology has successfully been integrated into water purification system design
This ready reference on Membrane Technologies for Water Treatment, is an invaluable source detailing sustainable, emerging processes, to provide clean, energy saving and cost effective alternatives to conventional processes. The editors are internationally renowned leaders in the field, who have put together a first-class team of authors from academia and industry to present a highly approach to the subject. The book is an instrumental tool for Process Engineers, Chemical Engineers, Process Control Technicians, Water Chemists, Environmental Chemists, Materials Scientists and Patent Lawyers.
Water is a vital element for life and the environment. Water pollution has been documented as a contributor to a wide range of health problems. In recent years, the water quality levels have suffered great deterioration because of rapid social and economic development and because it is used to “dump” a wide range of pollutants.This book entitled “Membranes for Water and Wastewater Treatment” contains featured research papers dealing with recent developments and advances in all aspects related to membranes for water and wastewater treatment: membrane processes, combined processes (including one membrane step), modified membranes, new materials, and the possibility to reduce fouling and to improve the efficiency of enhanced processes. The papers compiled in this Special Issue can be read as a response to the current needs and challenges in membrane development for water and wastewater treatment.Half of the research articles correspond to concrete and practical applications of the use of membrane processes in different fields of the industry, with the aim of treating and conditioning water and wastewater. The studies reveal the treatment of industrial streams, mining, recycled paper industry, olive mill, urban wastewater, etc. Another important percentage of studies are related to membrane modification processes, with the aim of obtaining new materials with better performance in the separation processes, thus describing the use of membranes modified with chitosan, nanoparticles, and other organic compounds. This field also includes studies related to fouling and its modeling.