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In a giant step toward managing today's pollution problems more effectively, this report lays out a framework to coordinate an interdisciplinary and international investigation of the chemical composition and cycles of the troposphere. The approach includes geographical surveys, field measurements, the development of appropriate models, and improved instrumentation.
Praise for Guy P. Brasseur's Atmospheric Chemistry in a Changing World American Meteorological Society "This volume summarizes and integrates more than a decade of atmospheric chemistry research. During the period under consideration, great progress has been made in computing, modeling, and observational techniques, and methods have also improved. Here, suggestions for the highest priority research for the next decade are made, and important information is related regarding impacts on the environment."
Atmospheric Chemistry and Global Change presents an integrated examination of chemical processes in the atmosphere, focusing on global-scale problems and their role in the evolution of the Earth system. Taking a largely interdisciplinary approach, it features the collective efforts of a group of scientists at the National Center for Atmospheric Research (NCAR), as well as other experts from several universities and national laboratories. Topics discussed include the fundamental physical, chemical, and biological processes that affect the atmospheric composition; the chemical mechanisms that affect the production and the fate of important chemical compounds; and the techniques used to investigate the chemical processes in the atmosphere. The book concludes with discussions on global problems related to the atmosphere (stratospheric ozone depletion, changes in greenhouse gases, and global chemical pollution), the relationship between the atmosphere and the global climate, and the long-term chemical evolution of the atmosphere. Each chapter features a brief essay by a leader in the field and includes a large number of current references. Ideal for graduate courses in atmospheric chemistry and atmospheric science, Atmospheric Chemistry and Global Change also serves as an authoritative and practical reference for scientists studying the Earth's atmosphere. Support materials for the book are available via the website http: //acd.ucar.edu/textbook
Here is the most comprehensive and up-to-date treatment of one of the hottest areas of chemical research. The treatment of fundamental kinetics and photochemistry will be highly useful to chemistry students and their instructors at the graduate level, as well as postdoctoral fellows entering this new, exciting, and well-funded field with a Ph.D. in a related discipline (e.g., analytical, organic, or physical chemistry, chemical physics, etc.). Chemistry of the Upper and Lower Atmosphere provides postgraduate researchers and teachers with a uniquely detailed, comprehensive, and authoritative resource. The text bridges the "gap" between the fundamental chemistry of the earth's atmosphere and "real world" examples of its application to the development of sound scientific risk assessments and associated risk management control strategies for both tropospheric and stratospheric pollutants. Serves as a graduate textbook and "must have" reference for all atmospheric scientists Provides more than 5000 references to the literature through the end of 1998 Presents tables of new actinic flux data for the troposphere and stratospher (0-40km) Summarizes kinetic and photochemical date for the troposphere and stratosphere Features problems at the end of most chapters to enhance the book's use in teaching Includes applications of the OZIPR box model with comprehensive chemistry for student use
This volume contains the invited papers and a transcript of the final panel discussion in the First Scientific Conference of the International Global Atmospheric Chemistry (lGAC) Project, held in Eilat, Israel from April 18-22, 1993. The conference was hosted by the Israeli Institute for Biological Research (IIBR) and was the 37th in the prestigious OHOLO Conference series in Israel. The conference was devoted to the subject of "Global Atmospheric-Biospheric Chemistry" and was a landmark event in this area. It provided the first comprehensive report of progress under IGAC toward improving our understanding of the chemical and biological processes that determine the changing composition of the earth's atmosphere. This work is an essential component of the comprehensive International Geosphere Biosphere Program (lGBP) devoted to measuring and understanding global changes in the past and present, and predicting the future evolution of our planet. I want to devote this brief foreword to thanking several people who worked especially hard to make the conference a success and who helped to produce this volume as a record of the event. Paul Crutzen, Amram Golombek, Pamela Matson and Henning Rodhe did sterling service on the conference organizing committee. Special thanks go to Amram Golombek and Dr. Cohen, the Director of IIBR, who hosted the event in Israel. Anne Slinn did an excellent job in producing the Abstract book and helping with administrative matters. Alex Pszenny helped capably to critically review the Abstracts.
Atmospheric Chemistry has been a rapidly growing field with a recent focus on the major aspects of global environmental change, including stratospheric ozone depletion, UV-B change, and global warming. This book describes recent developments in our understanding of the global aspects of the chemistry in the main parts of the atmosphere, troposphere, and stratosphere, as obtained from field observations, laboratory investigations, and modeling studies. Although this chemistry is largely driven by reactions between gas phase species, recent progress made in the understanding of chemical reactions occuring in clouds and on the surface of aerosols is also reported.
Atmospheric chemistry is one of the fastest growing fields in the earth sciences. Until now, however, there has been no book designed to help students capture the essence of the subject in a brief course of study. Daniel Jacob, a leading researcher and teacher in the field, addresses that problem by presenting the first textbook on atmospheric chemistry for a one-semester course. Based on the approach he developed in his class at Harvard, Jacob introduces students in clear and concise chapters to the fundamentals as well as the latest ideas and findings in the field. Jacob's aim is to show students how to use basic principles of physics and chemistry to describe a complex system such as the atmosphere. He also seeks to give students an overview of the current state of research and the work that led to this point. Jacob begins with atmospheric structure, design of simple models, atmospheric transport, and the continuity equation, and continues with geochemical cycles, the greenhouse effect, aerosols, stratospheric ozone, the oxidizing power of the atmosphere, smog, and acid rain. Each chapter concludes with a problem set based on recent scientific literature. This is a novel approach to problem-set writing, and one that successfully introduces students to the prevailing issues. This is a major contribution to a growing area of study and will be welcomed enthusiastically by students and teachers alike.
The Arctic troposphere (0 to ca. 8 km) plays an important role in environmental concerns for global change. It is a unique chemical reactor influenced by human activity and the Arctic ocean. It is surrounded by industrialized continents that in winter contribute gaseous and particulate pollution (Arctic haze). It is underlain by the flat Arctic ocean from which it is separated by a crack-ridden ice membrane 3 to 4 m thick. Ocean to atmosphere exchange of heat, water vapor and marine biogenic gases influence the composition of the reactor. From September 21 to December 21 to March 21, the region north of the Arctic circle goes from a completely sunlit situation to a completely dark one and then back to light. At the same time the lower troposphere is stably stratified. This hinders vertical mixing. During this light period, surface temperature reaches as low as -40°C. In this environment, chemical reactions involving sunlight are generally much slower than further south. Thus, the abundance of photochemically reactive compounds in the atmosphere can be high prior to polar sunrise. Between complete dark in February and complete light in April, a number of chemical changes in the lower troposphere take place.