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This thesis describes a search for the rare decay K{sub L} {yields} {pi}{sup 0}{pi}{sup 0}{gamma} using data from the KTeV experiment, using the topology K{sub L} {yields} {pi}{sup 0}{pi}{sub D}{sup 0}{gamma} (where {pi}{sub D}{sup 0} {yields} {gamma}e{sup +}e{sup -}). Due to Bose statistics and the real nature of the photon, the K{sub L} {yields} {pi}{sup 0}{pi}{sup 0}{gamma} decay can proceed at lowest order only by the Cp conserving direct emission of an E2 photon. The decay vanishes to O(p{sup 4}) in chiral perturbation theory and is a probe of the theory to the sixth order. The primary background to this decay consists of K{sub L} {yields} {pi}{sup 0}{pi}{sup 0}{pi}{sub D}{sup 0} events with one lost photon. The upper limit for the decay K{sub L} {yields} {pi}{sup 0}{pi}{sup 0}{gamma} presented in this thesis is 2.32 x 10{sup -7} at the 90% confidence level. This upper limit was derived from both 1997 and 1999 data, using a blind analysis. The upper limit was derived from a Feldman-Cousins method, based on a weighted total of 0.53 data events in the signal region with an expected K{sub L} {yields} {pi}{sup 0}{pi}{sup 0}{pi}{sub D}{sup 0} background of 0.37 {+-} 0.28 events. The previous upper limit for this decay was 5.6 x 10{sup -6} at the 90% confidence level.
The NA48/2 experiment at the CERN SPS has collected a large sample of K to pi pi0 gamma decays.Two amplitudes contribute to these decays. The dominant one comes from Inner Bremsstrahlung (IB) in the K to pi pi0 process. The second one is given by the Direct Emission (DE) of the photon at the weak vertex from an intermediate state of the decay. The simplest radiative transitions are electric dipole (E1) and magnetic dipole (M1). Electric amplitudes can interfere with IB, and CP violation and possible non-SM effects can show up in th e corresponding interference (INT) term.In this work a sub sample of the data has been analyzed. About 120000 K to pi pi0 gamma decays, with negligible background contamination have been reconstructed in the ranges 0.2