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An exciton is an electronic excitation wave consisting of an electron-hole pair which propagates in a nonmetallic solid. Since the pioneering research of Fren kel, Wannier and the Pohl group in the 1930s, a large number of experimental and theoretical studies have been made. Due to these investigations the exciton is now a well-established concept and the electronic structure has been clarified in great detail. The next subjects for investigation are, naturally, dynamical processes of excitons such as excitation, relaxation, annihilation and molecule formation and, in fact, many interesting phenomena have been disclosed by recent works. These excitonic processes have been recognized to be quite important in solid-state physics because they involve a number of basic interactions between excitons and other elementary excitations. It is the aim of this quasi monograph to describe these excitonic processes from both theoretical and experimental points of view. we take a few To discuss and illustrate the excitonic processes in solids, important and well-investigated insulating crystals as playgrounds for excitons on which they play in a manner characteristic of each material. The selection of the materials is made in such a way that they possess some unique properties of excitonic processes and are adequate to cover important interactions in which excitons are involved. In each material, excitonic processes are described in detail from the experimental side in order to show the whole story of excitons in a particular material.
A unifying element that links the apparently diverse phenomena observed in optical processes is the dielectric dispersion of matter. It describes the response of matter to incoming electromagnetic waves and charged particles, and thus predicts their behavior in the self-induced field of matter, known as polariton and polaron effects. The energies of phonon, exciton and plasmon, quanta of collective motions of charged particles constituting the matter, are also governed by dielectric dispersion. Since the latter is a functional of the former, one can derive useful relations for their self-consistency. Nonlinear response to laser light inclusive of multiphoton processes, and excitation of atomic inner shells by synchrotron radiation, are also described. Within the configuration coordinate model, photo-induced lattice relaxation and chemical reaction are described equally to both ground and relaxed excited states, to provide a novel and global perspective on structural phase transitions and the nature of interatomic bonds. This book was first published in 2003.
At Yamada Conference LIII, papers on many novel materials and on novel phenomena in condensed matter physics were presented — for instance, the achievement of simultaneous creation of excitons and free-electron-hole pairs in rare gas solids, and a low frequency fluctuation of the spectral shift of indirect excitons in GaAs coupled quantum wells. Single molecule spectroscopy is a powerful tool for studying molecules including biological systems; the study of delocalization of excitons in the photosynthetic light harvesting antenna system was also reported. The proceedings thus contain many excellent papers dealing with current research topics on the excitonic processes in bulk, quantum wells, quantum dots and other confined systems. This book will serve as an excellent source of recent references and reviews for a wide range of researchers in physics, chemistry, engineering and biological sciences.The proceedings have been selected for coverage in:• Index to Scientific & Technical Proceedings (ISTP CDROM version / ISI Proceedings)
Provides a semi-quantitative approach to recent developments in the study of optical properties of condensed matter systems Featuring contributions by noted experts in the field of electronic and optoelectronic materials and photonics, this book looks at the optical properties of materials as well as their physical processes and various classes. Taking a semi-quantitative approach to the subject, it presents a summary of the basic concepts, reviews recent developments in the study of optical properties of materials and offers many examples and applications. Optical Properties of Materials and Their Applications, 2nd Edition starts by identifying the processes that should be described in detail and follows with the relevant classes of materials. In addition to featuring four new chapters on optoelectronic properties of organic semiconductors, recent advances in electroluminescence, perovskites, and ellipsometry, the book covers: optical properties of disordered condensed matter and glasses; concept of excitons; photoluminescence, photoinduced changes, and electroluminescence in noncrystalline semiconductors; and photoinduced bond breaking and volume change in chalcogenide glasses. Also included are chapters on: nonlinear optical properties of photonic glasses; kinetics of the persistent photoconductivity in crystalline III-V semiconductors; and transparent white OLEDs. In addition, readers will learn about excitonic processes in quantum wells; optoelectronic properties and applications of quantum dots; and more. Covers all of the fundamentals and applications of optical properties of materials Includes theory, experimental techniques, and current and developing applications Includes four new chapters on optoelectronic properties of organic semiconductors, recent advances in electroluminescence, perovskites, and ellipsometry Appropriate for materials scientists, chemists, physicists and electrical engineers involved in development of electronic materials Written by internationally respected professionals working in physics and electrical engineering departments and government laboratories Optical Properties of Materials and Their Applications, 2nd Edition is an ideal book for senior undergraduate and postgraduate students, and teaching and research professionals in the fields of physics, chemistry, chemical engineering, materials science, and materials engineering.
Self-Trapped Excitons discusses the structure and evolution of the self-trapped exciton (STE) in a wide range of materials. It includes a comprehensive review of experiments and extensive tables of data. Emphasis is given throughout to the unity of the basic physics underlying various manifestations of self-trapping, with the theory being developed from a localized, atomistic perspective. The topics treated in detail in relation to STE relaxation include spontaneous symmetry breaking, lattice defect formation, radiation damage, and electronic sputtering.
At Yamada Conference LIII, papers on many novel materials and on novel phenomena in condensed matter physics were presented OCo for instance, the achievement of simultaneous creation of excitons and free-electron-hole pairs in rare gas solids, and a low frequency fluctuation of the spectral shift of indirect excitons in GaAs coupled quantum wells. Single molecule spectroscopy is a powerful tool for studying molecules including biological systems; the study of delocalization of excitons in the photosynthetic light harvesting antenna system was also reported. The proceedings thus contain many excellent papers dealing with current research topics on the excitonic processes in bulk, quantum wells, quantum dots and other confined systems. This book will serve as an excellent source of recent references and reviews for a wide range of researchers in physics, chemistry, engineering and biological sciences. The proceedings have been selected for coverage in: . OCo Index to Scientific & Technical Proceedings (ISTP CDROM version / ISI Proceedings). Contents: Dynamical Process of Photoionization in Semiconductor Nanocrystals (M Y Shen et al.); Excitons on a 1D Periodic Conjugated Polymer Chain: Two Electronic Structures of Polydiacetylene Chains (C Lapersonne-Meyer); Anomalous Spectral Shifts of Indirect Excitons in Coupled GaAs Quantum Wells (D W Snoke et al.); Infrared Absorption by Excitons in Cuprous Oxide (M GAppert et al.); Theory of Excitation-Energy Transfer Processes Involving Optically Forbidden Exciton States in Antenna Systems of Photosynthesis (K Mukai et al.); Transient Grating Induced by Excitonic Polaritons in Thin Film Semiconductors (K Akiyama et al.); Excitonic Photoluminescence of Pentacene Single Crystal (T Aoki-Matsumoto et al.); Scanning Near-Field Optical Microspectroscopy of Single Perylene Microcrystals (J Niitsuma et al.); and other papers. Readership: Condensed matter physicists, materials scientists, chemists and biologists."
Applying a unified quantum approach, contributors offer fresh insights into the theoretical developments in the excitation energy transfer processes in condensed matter. This comprehensive volume examines Frenkel and Wannier excitonic processes; rates of excitonic processes; theory of laser sputter and polymer ablation; and polarons, excitonic polarons and self-trapping.