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Electron transfer is the most important process to take place in natural and artificial chemical systems, playing a fundamental role, for example, in photosynthesis as well as in photography. Electron transfer reactions - oxidations and reductions - are involved in, among others, a variety of energy conversion processes, analytical methods, synthetic strategies, and information processing systems. This five-volume work is the only comprehensive yet up-to-date reference on electron transfer processes. Following a foreword by Nobel prize-winner R. A. Marcus, renowned experts from all over the world provide an interdisciplinary overview of every aspect of electron transfer including theoretical-physicochemical backgrounds, latest analytical techniques to identify, monitor and measure the rate of electron transfer, utilizing electron transfer reactions in organic synthesis and catalysis, electron transfer in the gas phase or in special heterogeneous systems such as zeolites or sensitized electrodes. Other central issues are the study of biological systems and the biomimetic electron transfer processes in artificial supramolecular systems. Finally, a complete volume is dedicated to the application of electron transfer in molecular-level electronics, imaging processes and energy conversion. Each chapter is complemented by numerous tables, formulae and illustrations providing an indispensable wealth of information. All references are cross-indexed throughout the work for easy access to this highly complex topic. Whether for quickly looking-up a keyword or as a thorough introduction to a special aspect, this is an essential handbook for everyone working in the field, from experts to postgraduates, from synthetic chemists, physicochemists or biochemists to research groups in material sciences.
Electron transfer is the most important process to take place in natural and artificial chemical systems, playing a fundamental role, for example, in photosynthesis as well as in photography. Electron transfer reactions - oxidations and reductions - are involved in, among others, a variety of energy conversion processes, analytical methods, synthetic strategies, and information processing systems. This five-volume work is the only comprehensive yet up-to-date reference on electron transfer processes. Following a foreword by Nobel prize-winner R. A. Marcus, renowned experts from all over the world provide an interdisciplinary overview of every aspect of electron transfer including theoretical-physicochemical backgrounds, latest analytical techniques to identify, monitor and measure the rate of electron transfer, utilizing electron transfer reactions in organic synthesis and catalysis, electron transfer in the gas phase or in special heterogeneous systems such as zeolites or sensitized electrodes. Other central issues are the study of biological systems and the biomimetic electron transfer processes in artificial supramolecular systems. Finally, a complete volume is dedicated to the application of electron transfer in molecular-level electronics, imaging processes and energy conversion. Each chapter is complemented by numerous tables, formulae and illustrations providing an indispensable wealth of information. All references are cross-indexed throughout the work for easy access to this highly complex topic. Whether for quickly looking-up a keyword or as a thorough introduction to a special aspect, this is an essential handbook for everyone working in the field, from experts to postgraduates, from synthetic chemists, physicochemists or biochemists to research groups in material sciences.
Electron transfer is the most important process to take place in natural and artificial chemical systems, playing a fundamental role, for example, in photosynthesis as well as in photography. Electron transfer reactions - oxidations and reductions - are involved in, among others, a variety of energy conversion processes, analytical methods, synthetic strategies, and information processing systems. This five-volume work is the only comprehensive yet up-to-date reference on electron transfer processes. Following a foreword by Nobel prize-winner R. A. Marcus, renowned experts from all over the world provide an interdisciplinary overview of every aspect of electron transfer including theoretical-physicochemical backgrounds, latest analytical techniques to identify, monitor and measure the rate of electron transfer, utilizing electron transfer reactions in organic synthesis and catalysis, electron transfer in the gas phase or in special heterogeneous systems such as zeolites or sensitized electrodes. Other central issues are the study of biological systems and the biomimetic electron transfer processes in artificial supramolecular systems. Finally, a complete volume is dedicated to the application of electron transfer in molecular-level electronics, imaging processes and energy conversion. Each chapter is complemented by numerous tables, formulae and illustrations providing an indispensable wealth of information. All references are cross-indexed throughout the work for easy access to this highly complex topic. Whether for quickly looking-up a keyword or as a thorough introduction to a special aspect, this is an essential handbook for everyone working in the field, from experts to postgraduates, from synthetic chemists, physicochemists or biochemists to research groups in material sciences.
Electron transfer is the most important process to take place in natural and artificial chemical systems, playing a fundamental role, for example, in photosynthesis as well as in photography. Electron transfer reactions - oxidations and reductions - are involved in, among others, a variety of energy conversion processes, analytical methods, synthetic strategies, and information processing systems. This five-volume work is the only comprehensive yet up-to-date reference on electron transfer processes. Following a foreword by Nobel prize-winner R. A. Marcus, renowned experts from all over the world provide an interdisciplinary overview of every aspect of electron transfer including theoretical-physicochemical backgrounds, latest analytical techniques to identify, monitor and measure the rate of electron transfer, utilizing electron transfer reactions in organic synthesis and catalysis, electron transfer in the gas phase or in special heterogeneous systems such as zeolites or sensitized electrodes. Other central issues are the study of biological systems and the biomimetic electron transfer processes in artificial supramolecular systems. Finally, a complete volume is dedicated to the application of electron transfer in molecular-level electronics, imaging processes and energy conversion. Each chapter is complemented by numerous tables, formulae and illustrations providing an indispensable wealth of information. All references are cross-indexed throughout the work for easy access to this highly complex topic. Whether for quickly looking-up a keyword or as a thorough introduction to a special aspect, this is an essential handbook for everyone working in the field, from experts to postgraduates, from synthetic chemists, physicochemists or biochemists to research groups in material sciences.
The subject of the book is electron transfer reactions in organic chemistry, with the emphasis on mechanistic aspects. The theoretical framework is that of the Marcus theory, well-known from its extensive use in inorganic chemistry. The book deals with definitions of electron transfer, theory of electron transfer reactions (Marcus' and Pross-Shaik's approach) experimental diagnosis of electron transfer reactions, examples from inorganic/organic reactants and purely organic reactants, electro- and photochemical electron transfer, electron transfer catalyzed reactions, connections between electron transfer and polar mechanisms, and applications of electron transfer, such as electrosynthesis of organic chemicals, photochemical energy storage, conducting organic materials and chemiluminescence. The approach is new in so far as no comparable book has been published. The book will be of value to anyone interested in keeping track of developments in physical organic chemistry.
Electron transfer is the most important process to take place in natural and artificial chemical systems, playing a fundamental role, for example, in photosynthesis as well as in photography. Electron transfer reactions - oxidations and reductions - are involved in, among others, a variety of energy conversion processes, analytical methods, synthetic strategies, and information processing systems. This five-volume work is the only comprehensive yet up-to-date reference on electron transfer processes. Following a foreword by Nobel prize-winner R. A. Marcus, renowned experts from all over the world provide an interdisciplinary overview of every aspect of electron transfer including theoretical-physicochemical backgrounds, latest analytical techniques to identify, monitor and measure the rate of electron transfer, utilizing electron transfer reactions in organic synthesis and catalysis, electron transfer in the gas phase or in special heterogeneous systems such as zeolites or sensitized electrodes. Other central issues are the study of biological systems and the biomimetic electron transfer processes in artificial supramolecular systems. Finally, a complete volume is dedicated to the application of electron transfer in molecular-level electronics, imaging processes and energy conversion. Each chapter is complemented by numerous tables, formulae and illustrations providing an indispensable wealth of information. All references are cross-indexed throughout the work for easy access to this highly complex topic. Whether for quickly looking-up a keyword or as a thorough introduction to a special aspect, this is an essential handbook for everyone working in the field, from experts to postgraduates, from synthetic chemists, physicochemists or biochemists to research groups in material sciences.
Electron transfer is the most important process to take place in natural and artificial chemical systems, playing a fundamental role, for example, in photosynthesis as well as in photography. Electron transfer reactions - oxidations and reductions - are involved in, among others, a variety of energy conversion processes, analytical methods, synthetic strategies, and information processing systems. This five-volume work is the only comprehensive yet up-to-date reference on electron transfer processes. Following a foreword by Nobel prize-winner R. A. Marcus, renowned experts from all over the world provide an interdisciplinary overview of every aspect of electron transfer including theoretical-physicochemical backgrounds, latest analytical techniques to identify, monitor and measure the rate of electron transfer, utilizing electron transfer reactions in organic synthesis and catalysis, electron transfer in the gas phase or in special heterogeneous systems such as zeolites or sensitized electrodes. Other central issues are the study of biological systems and the biomimetic electron transfer processes in artificial supramolecular systems. Finally, a complete volume is dedicated to the application of electron transfer in molecular-level electronics, imaging processes and energy conversion. Each chapter is complemented by numerous tables, formulae and illustrations providing an indispensable wealth of information. All references are cross-indexed throughout the work for easy access to this highly complex topic. Whether for quickly looking-up a keyword or as a thorough introduction to a special aspect, this is an essential handbook for everyone working in the field, from experts to postgraduates, from synthetic chemists, physicochemists or biochemists to research groups in material sciences.
Developed from a symposium sponsored by the International Chemical Congress of Pacific Basin Societies, Honolulu, Hawaii, December 17-22, 1989.
Photosensitization and photocatalysis refer to processes by which permanent chemical transformations are induced on substrates (organic/inorganic) by radiation to which the substrates themselves are transparent. Such transformations can be highly specific, very efficient, and occur under mild conditions. Herein lies the power of photochemical methods for possible applications in the field of conversion and storage of solar energy. This book provides a recent survey of the progress in this important area in catalysis, with an emphasis on inorganic complexes and organometallic compounds as the key light aborbers. The book is organized in three parts: fundamentals, followed by applications. Discussions cover a wide variety of photosensitized or photocatalyzed reactions: decomposition of water, reduction of CO2 and CO; spectral sensitization in photoelectrochemical cells; transformations (oxidation, reduction, isomerization, hydrogenation, dehydrogenation, carbonylation, etc.) of organics such as alkanes, alkenes, alcohols, etc. In view of the variety of systems (sensitizers, substrates) and the topics covered, the volume is unique in the field of photochemistry and will appeal to academic and industrial researchers in various subdisciplines of chemistry, material science and catalysis.