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Uranium and its alloys are capable of being processed, fabricated and heat treated by many different methods. The deleterious effects of hydrogen on the mechanical properties of uranium and its alloys are well established. In this study the effects of certain processing procedures on hydrogen absorption and removal were investigated. Both unalloyed uranium and uranium-3/4 wt % titanium were involved in this work. The tensile test data for both materials clearly show the adverse effects of hydrogen absorption.
In a continuing program, fabrication characteristics, physical and mechanical properties, and corrosion behavior in air, CO2, NaK, water, and steam were studied for . binary niobium fuel alloys containing 10, 20, 30, 40, 50, and 60 wt.% uranium To evaluate the effects of two major impurities of niobium, oxygen, and zirconium, three niobium base stocks, differing according to the level of these impurities, were used for each alloy. The impurity combinations employed were 600 ppm oxygen and 0.74 wt.% zirconium, 700 ppm oxygen, and 0.17 wt.% zirconium, and 300 ppm oxygen and 0.02 wt.% zirconium, Representative specimens of these alloys retained their hardness up to 900 deg C The 10 and 20 wt.% uraniuin alloys were successfully rorged at 2500 deg F and rolled at 1800 deg F to sheet. Fabrication characteristics of the remaining alloys are under investigation. The 0.2% offset yield strength of the 10 wt.% uranium alloy was 57,200 psi at room temperature and 36,900 psi at 1600 deg F. For the 20 wt.% uranium alloy it was 93,200 psi at room temperature and 71.000 psi at 1600 deg F. The corrosion life of all of the alloys in air at 572 deg F and in CO2 at 600 deg F was superior to that of unalloyed niobium. In 1000- hr exposures to 600 deg F water most of the alloys exhibited corrosion rates only two or three times greater than that of Zircaloy-2. All oi the alloys appear compatible with NaK at 1600 deg F. The impurity combinations employed in the base niobium appeared to have no effect on the corrosion behavior and mechanical properties of the alloys. (auth).
The effects of pile irradiations on the physical properties and corrosion resistance of U-- Mo, U-- Nb; and U--Si alloys are reported. The dimensional stability under irradiation of the gamma phase U-- Mo and U-- Nb alloys is excellent; however, an isotropic volume increase of 4 to 6% per wt.% burnup may limit the ultimate fuel element life. Corrosion resistance of the gamma-phase alloys appesrs to be improved when subjected to s neutron field; this is attributed to an irrsdiation induced stabilization of the gamma phases. The U/ sub 3/Si alloy, on the other hand, suffered severe deterioration, particularly of corrosion resistance. Changes in electrical resistivity, hardness, mechanical properties, and crystal structure are presented and the mechanisms producing the observed changes discussed.