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This proceedings volume contains review articles on solid-state spectroscopies by leading researchers in Japan and Taiwan. Topics include excitons and biexcitons, size effects in quantum dots and microcrystals, nonlinear optical properties, optical spectra of disordered systems, electronic and optical properties of metal-dielectric and semiconductor superlattices, photoemission, Raman spectroscopy, and photoreflectance studies on solids.
Dynamical Properties of Solids, Volume 4: Disordered Solids, Optical Properties focuses on the lattice dynamical properties of noncrystalline and disordered solids and optical properties of crystalline solids. The selection first elaborates on the vibrational properties of amorphous solids and computer experiments and disordered solids. Topics include thermal and electrical transport, density of states, numerical methods, localization, low frequency modes, and theoretical background. The text then takes a look at the morphic effects in lattice dynamics, including normal coordinate formalism, electric-field-induced infrared absorption and Raman scattering, stress-induced changes in the phonon frequencies, and the effect of time reversal on the symmetry of the long-wavelength optical. The manuscript examines the absorption of infrared radiation by multiphonon processes in solids, as well as theoretical studies of infrared absorption in the multiphonon region and experimental studies of infrared absorption at frequencies above the characteristic lattice vibration frequencies. The selection is a dependable source of data for researchers interested in the optical properties of crystalline solids and lattice dynamical properties of noncrystalline and disordered solids.
Optical Properties of Solids covers the important concepts of intrinsic optical properties and photoelectric emission. The book starts by providing an introduction to the fundamental optical spectra of solids. The text then discusses Maxwell's equations and the dielectric function; absorption and dispersion; and the theory of free-electron metals. The quantum mechanical theory of direct and indirect transitions between bands; the applications of dispersion relations; and the derivation of an expression for the dielectric function in the self-consistent field approximation are also encompassed. The book further tackles current-current correlations; the fluctuation-dissipation theorem; and the effect of surface plasmons on optical properties and photoemission. People involved in the study of the optical properties of solids will find the book invaluable.
This book presents an account of the course "Disordered Solids: Structures and Processes" held in Erice, Italy, from June 15 to 29, 1987. This meeting was organized by the International School of Atomic and Molecular Spectroscopy of the "Ettore Majorana" Centre for Scientific Culture. The objective of this course was to present the advances in physical modelling, mathematical formalism and experimental techniques relevant to the interpretation of the structures of disordered solids and of the physical processes occurring therein. Traditional solid-state physics treats solids as perfect crystals and takes great advantage of their symmetry, by means of such mathematical formalisms as the reciprocal lattice, the Brillouin zone, and the powerful tools of group theory. Even if in reality no solid is a perfect crystal, this theoretical approach has been of great usefulness in describing solids: deviations from perfect order have been treated as perturbations of the ideal model. A new situation arises with truly disordered solids where any vestige of long range order has disappeared. The basic problem is that of describing these systems and gaining a scientific understanding of their physical properties without the mathematical formalism of traditional solid state physics. While some of the old approaches may occasionally remain valid (e. g. chemical bonding approach for amorphous solids), the old ways will not do. Disorder is not a perturbation: with disorder, something basically new may be expected to appear.
The first two volumes in this series published twenty years ago contained chapters devoted to anharmonic properties of solids, ab initio calculations of phonons in metals and insulators, and surface phonons. In the intervening years each of these important areas of lattice dynamics has undergone significant developments. This volume is therefore concerned with reviewing the current status of these areas.Chapter one deals with the path-integral quantum Monte-Carlo method as a numerical simulation approach and looks at how this has been applied successfully to the determination of low temperature thermodynamic properties of anharmonic crystals and to certain dynamical properties as well. Chapter two is concerned with the calculation of static and dynamic properties of anharmonic crystals in the quantum regime. Chapter three discusses intrinsic anharmonic localized modes that have been intensively studied recently. Two topics, ab initio calculations of phonons in metals, and surface phonons are dealt with in the next chapter. The remaining two chapters are devoted to topics that have not been treated in previous volumes. One is phonon transport and the second is phonons in disordered crystals.The work described in the six chapters of this volume testifies to the continuing vitality of the field of dynamical properties of solids nearly a century after its founding.
Introduction to Solid-State Theory is a textbook for graduate students of physics and materials science. It also provides the theoretical background needed by physicists doing research in pure solid-state physics and its applications to electrical engineering. The fundamentals of solid-state theory are based on a description by delocalized and localized states and - within the concept of delocalized states - by elementary excitations. The development of solid-state theory within the last ten years has shown that by a systematic introduction of these concepts, large parts of the theory can be described in a unified way. This form of description gives a "pictorial" formulation of many elementary processes in solids, which facilitates their understanding.
This book presents an account of the course "Optical Properties of Excited States in Solids" held in Erice, Italy, from June 16 to 3D, 1991. This meeting was organized by the International School of Atomic and Molecular Spectroscopy of the "Ettore Majorana" Centre for Scientific Culture. The purpose of this course was to present physical models, mathematical formalisms and experimental techniques relevant to the optical properties of excited states in solids. Some active physical species, such as ions or radicals, could survive indefinitely if they were completely 'isolated in space. Other active species, such as excited molecular and solid-state systems, are inherently unstable, even in isolation, due to the spontaneous mechanisms that may convert their excitation energies into radiation or heat. Physical parameters that may be used to characterize these excited systems are the localization or delocalization, and the coherence or incoherence, of their state excitations. In solids the excited states, whether they are localized (as for impurities in insulators) or delocalized (as they may occur in semiconductors), are relevant in several regards. Their de-excitation is extremely sensitive to the nature of the excitations of the systems, and a study of the de-excitation processes can yield a variety of information. For example, the excited states may represent the initial condition of the onset of such processes as Stokes-shifted emission, hot luminescence, symmetry-dependent Jahn-Teller and scattering processes, tunneling processes, energy transfer to like and unlike centers, superradiance, coherent radiation, and excited state absorption.
This second, thoroughly revised, updated and enlarged edition provides a straightforward introduction to spectroscopy, showing what it can do and how it does it, together with a clear, integrated and objective account of the wealth of information that may be derived from spectra. It also features new chapters on spectroscopy in nano-dimensions, nano-optics, and polymer analysis. Clearly structured into sixteen sections, it covers everything from spectroscopy in nanodimensions to medicinal applications, spanning a wide range of the electromagnetic spectrum and the physical processes involved, from nuclear phenomena to molecular rotation processes. In addition, data tables provide a comparison of different methods in a standardized form, allowing readers to save valuable time in the decision process by avoiding wrong turns, and also help in selecting the instrumentation and performing the experiments. These four volumes are a must-have companion for daily use in every lab.