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Dynamical Collision Theory and Its Applications reviews some of the powerful methods that have evolved for calculating the predictions of dynamical collision theory. Topics range from scattering theory to potential scattering, three- and four-particle scattering, multiparticle scattering, many-particle Lippmann-Schwinger equations, and the connected-kernel approach. This book is comprised of nine chapters; the first of which introduces the reader to the quantum theory of scattering. This topic is followed by a discussion on two-particle potential scattering and various methods for calculating off-shell two-body amplitudes as well as approximating them by finite-rank forms. The next chapters focus on the interpretation and applicability of the multichannel, multiparticle Lippmann-Schwinger equations, along with the known N-particle connected-kernel integral equations and their physical predictions. Descriptions of contemporary field-theoretical and relativistic approaches, such as the Dirac phenomenology for intermediate energy nucleon-nucleus scattering, are included. The singularity structure of multiparticle amplitudes and the associated dispersion-relation techniques are also considered. This book concludes by describing the relationship between the conventional (optical potentials, multiple-scattering theories, and the coupled-reaction channel and resonating-group methods) and the few-body approaches. This text is primarily intended for chemists, physicists, and graduate students interested in general scattering theory; intermediate and low-energy hadron and nuclear physics; atomic and molecular physics; statistical mechanics; and physical and quantum chemistry. There are a number of topics in this book that will be interesting to both mathematicians and particle physicists, as well as advanced graduate students in courses that involve collision theory.
Since the discovery of quantum mechanics,more than fifty years ago,the theory of chemical reactivity has taken the first steps of its development. The knowledge of the electronic structure and the properties of atoms and molecules is the basis for an un derstanding of their interactions in the elementary act of any chemical process. The increasing information in this field during the last decades has stimulated the elaboration of the methods for evaluating the potential energy of the reacting systems as well as the creation of new methods for calculation of reaction probabili ties (or cross sections) and rate constants. An exact solution to these fundamental problems of theoretical chemistry based on quan tum mechanics and statistical physics, however, is still impossible even for the simplest chemical reactions. Therefore,different ap proximations have to be used in order to simplify one or the other side of the problem. At present, the basic approach in the theory of chemical reactivity consists in separating the motions of electrons and nu clei by making use of the Born-Oppenheimer adiabatic approximation to obtain electronic energy as an effective potential for nuclear motion. If the potential energy surface is known, one can calculate, in principle, the reaction probability for any given initial state of the system. The reaction rate is then obtained as an average of the reaction probabilities over all possible initial states of the reacting ~artic1es. In the different stages of this calculational scheme additional approximations are usually introduced.
A systematic description of the basic principles of collision theory, this graduate-level text presents a detailed examination of scattering processes and formal scattering theory, the two-body problem with central forces, scattering by noncentral forces, lifetime and decay of virtual states, an introduction to dispersion theory, and more. 1964 edition.
Photodissociation induced by the absorption of single photons permits the detailed study of molecular dynamics such as the breaking of bonds, internal energy transfer and radiationless transitions. The availability of powerful lasers operating over a wide frequency range has stimulated rapid development of new experimental techniques which make it possible to analyse photodissociation processes in unprecedented detail. This text elucidates the achievements in calculating photodissociation cross-sections and fragment state distributions from first principles, starting from multi-dimensional potential energy surfaces and the Schrödinger equation of nuclear motion. Following an extended introduction in which the various types of observables are outlined, the book summarises the basic theoretical tools, namely the time-independent and the time-dependent quantum mechanical approaches as well as the classical picture of photodissociation. The discussions of absorption spectra, diffuse vibrational structures, the vibrational and rotational state distributions of the photofragments form the core of the book. More specific topics such as the dissociation of vibrationally excited molecules, emission during dissociation, or nonadiabatic effects are also discussed. It will be of interest to graduate students and senior scientists working in molecular physics, spectroscopy, molecular collisions and molecular kinetics.
Since the turn of the 21st century, the field of electron molecule collisions has undergone a renaissance. The importance of such collisions in applications from radiation chemistry to astrochemistry has flowered, and their role in industrial processes such as plasma technology and lighting are vital to the advancement of next generation devices. F
Covers both molecular and reaction dynamics. The work presents important theroetical and computational approaches to the study of energy transfer within and between molecules, discussing the application of these approaches to problems of experimental interest. It also describes time-dependent and time-independent methods, variational and perturbative techniques, iterative and direct approaches, and methods based upon the use of physical grids of finite sets of basic function.
This book contains invited review papers and short notes presented at the International Conference on Physics, Chemistry and Application of Nanostructures (Nanomeeting 2003).
This book highlights a major advance in low-energy scattering theory: the Multi-Channel Algebraic Scattering (MCAS) theory, which represents an attempt to unify structure and reaction theory. It solves the Lippmann–Schwinger equations for low-energy nucleon-nucleus and alpha-nucleus scattering in momentum space, allowing both the bound and scattering states in the compound nucleus formed to be described. Results of various cases are presented and discussed.
This book focuses on the latest theoretical and experimental results and future perspectives regarding electromagnetic and hadronic physics at intermediate energies. Nucleon form factors and spin structure functions, deep-inelastic scattering, excited baryons and mesons, and correlations in nuclei are discussed. Many new results and the scientific programmes of the different laboratories in Europe and North America are also presented. A special section is devoted to relativistic approaches to hadrons and nuclei at intermediate energies.
Chemical Kinetics and Reaction Dynamics brings together the major facts and theories relating to the rates with which chemical reactions occur from both the macroscopic and microscopic point of view. This book helps the reader achieve a thorough understanding of the principles of chemical kinetics and includes: Detailed stereochemical discussions of reaction steps Classical theory based calculations of state-to-state rate constants A collection of matters on kinetics of various special reactions such as micellar catalysis, phase transfer catalysis, inhibition processes, oscillatory reactions, solid-state reactions, and polymerization reactions at a single source. The growth of the chemical industry greatly depends on the application of chemical kinetics, catalysts and catalytic processes. This volume is therefore an invaluable resource for all academics, industrial researchers and students interested in kinetics, molecular reaction dynamics, and the mechanisms of chemical reactions.