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Defect-Induced Magnetism in Oxide Semiconductors provides an overview of the latest advances in defect engineering to create new magnetic materials and enable new technological applications. First, the book introduces the mechanisms, behavior, and theory of magnetism in oxide semiconductors and reviews the methods of inducing magnetism in these materials. Then, strategies such as pulsed laser deposition and RF sputtering to grow oxide nanostructured materials with induced magnetism are discussed. This is followed by a review of the most relevant postdeposition methods to induce magnetism in oxide semiconductors including annealing, ion irradiation, and ion implantation. Examples of defect-induced magnetism in oxide semiconductors are provided along with selected applications. This book is a suitable reference for academic researchers and practitioners and for people engaged in research and development in the disciplines of materials science and engineering. Reviews the magnetic, electrical, dielectric and optical properties of oxide semiconductors with defect-induced magnetism Discusses growth and post-deposition strategies to grow oxide nanostructured materials such as oxide thin films with defect-induced magnetism Provides examples of materials with defect-induced magnetism such as zinc oxide, cerium dioxide, hafnium dioxide, and more
This work focuses on the impact of defects, intrinsic or artificially introduced, on the functional properties of thin, epitaxial oxide films. In the first part, the origin of the ferromagnetic properties of Mn-doped and undoped zinc oxide is studied. The deposition conditions are found to have a significant impact on the structural, transport and magnetic properties of the thin films. Combining x-ray magnetic circular dichroism and magnetometry experiments, it is established that the transition metal dopants (i.e. Mn) have no influence on the ferromagnetic nature of the zinc oxide, but that localised magnetic moments on intrinsic defects are in fact responsible for the ferromagnetic behaviour. A relation between strain (related to defect concentration) and magnetisation is established. In the second part of this dissertation, artificially introduced defects are employed in order to discover the fundamental conduction mechanism behind the two-dimensionally conductive LaAlO3/SrTiO3 interface. All experiments, from varying deposition temperature, to oxygen pressure, to laser fluence or to the insertion of (doped) perovskite layers, point towards a structurally governed conduction mechanism, although the exact details are still unclear. Distinct transitions in the resistance versus temperature curves are observed at different values than the bulk phase transformation temperature. These transitions form the boundaries of different conduction modes, with tendencies towards non-Fermi-liquid behaviour observed in certain two-dimensionally conducting samples in limited temperature regimes. By optimising the (defect) structure at the interface, i.e. by introducing a single unit cell of (La0.5,Sr0.5)TiO3 or SnTiO3, it is shown that the sheet carrier density can be dramatically enhanced, up to an order of magnitude higher than unmodified LaAlO3/SrTiO3 interfaces with a value of 1e14 cm-2 at 200 K. Finally, attempts at functionalising the conductive heterointerface by doping and inserting (anti)ferromagnetic layers are made.
This book provides an overview of the applications of ion beam techniques in oxide materials. Oxide materials exhibit defect-induced physical properties relevant to applications in sensing, optoelectronics and spintronics. Defects in these oxide materials also lead to magnetism in non-magnetic materials or to a change of magnetic ordering in magnetic materials. Thus, an understanding of defects is of immense importance. To date, ion beam tools are considered the most effective techniques for producing controlled defects in these oxides. This book will detail the ion beam tools utilized for creating defects in oxides.
This book provides an overview of the applications of ion beam techniques in oxide materials. Oxide materials exhibit defect-induced physical properties relevant to applications in sensing, optoelectronics and spintronics. Defects in these oxide materials also lead to magnetism in non-magnetic materials or to a change of magnetic ordering in magnetic materials. Thus, an understanding of defects is of immense importance. To date, ion beam tools are considered the most effective techniques for producing controlled defects in these oxides. This book will detail the ion beam tools utilized for creating defects in oxides.
One of the directions of nanotechnology is the production of nanopowders (NPs). Nanopowders, according to the currently widely used classification of nanomaterials, belong to zero-dimensional systems in which the limitation of wave functions occurs in all three directions. Biological methods are considered the most environmentally friendly way to synthesize NPs, but the possibility of biological contamination with mutated microorganisms cannot be ruled out. This book presents a new method for producing simple and complex metal oxide and fluoride NPs, based on the “evaporation-condensation” process using pulsed electron beam evaporation. It presents the results of more than 10 years of study of the characteristics of NPs produced using the aforementioned method. This eco-friendly method ensures the production of clean NPs, which are mesoporous and suitable for use in various applications such as medicine, spintronics, optoelectronics, dosimeters, photocatalysis, semiconductors, and ultraviolet and blue lasers. Importantly, these NPs have the potential to be used as a drug delivery system and in the creation of new nanostructures that do not contain noble metals. The book will be useful for the researchers in macromolecular science, nanotechnology, chemistry, biology, and medicine, especially those with an interest in drug delivery or cancer therapy.
This book summarizes the basic physics of graphite and newly discovered phenomena in this material. The book contains the knowledge needed to understand novel properties of functionalized graphite demonstrating the occurrence of remarkable phenomena in disordered graphite and graphite-based heterostructures. It also discusses applications of thin graphitic samples in future electronics. Graphite consists of a stack of nearly decoupled two-dimensional graphene planes. Because of the low dimensionality and the presence of Dirac fermions, much of graphite physics resembles that of graphene. On the other hand, the multi-layered nature of the graphite structure together with structural and/or chemical disorder are responsible for phenomena that are not observed yet in graphene, such as ferromagnetic order and superconductivity. Each chapter was written by one or more experts in the field whose contributions were relevant in the (re)discovery of (un)known phenomena in graphite. The book is intended as reference for beginners and experts in the field, introducing them to many aspects of the new physics of graphite, with a fresh overview of recently found phenomena and the theoretical frames to understand them.
Functional oxides are used both as insulators and metallic conductors in key applications across all industrial sectors. This makes them attractive candidates in modern technology ? they make solar cells cheaper, computers more efficient and medical instrumentation more sensitive. Based on recent research, experts in the field describe novel materials, their properties and applications for energy systems, semiconductors, electronics, catalysts and thin films. This monograph is divided into 6 parts which allows the reader to find their topic of interest quickly and efficiently. * Magnetic Oxides * Dopants, Defects and Ferromagnetism in Metal Oxides * Ferroelectrics * Multiferroics * Interfaces and Magnetism * Devices and Applications This book is a valuable asset to materials scientists, solid state chemists, solid state physicists, as well as engineers in the electric and automotive industries.
The book presents new results in the areas of nanomaterials, nanoparticles, ultra-small nanoparticles, plasmonic nanoparticles and coated nanoparticles for bio-medical applications. Emphasis is placed on (1) synthetic routes (quantum dots, thermal decomposition methods), (2) characterization methods (photo-physical techniques, X-ray diffraction, electron microscopy, light scattering, positron annihilation spectroscopy) and (3) bio-medical applications (nanomaterials and nanoparticles in physiology, medicine and bio-medicine).