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This conference on both the physics and chemistry of laser-induced processes in molecules was organized by the Quantum Electronics Divisional Board of the European Physical Society whose membership is given on p.367. The confer ence aim, to mix physicists and chemists interested in this exciting field both from Europe and further afield, was well fulfilled by the attendance of around 250 participants and the submission of about 100 papers, which dre presented here. Numerous people at both the Physics Department, Heriot-Watt University, Edinburgh, and at the Projektgruppe fUr Laserforschung, MPI, Garching, con tributed hard work to the organization; in addition to Dr. Bob Harrison, who bore the biggest burden with conspicuous success, we particularly thank Hugh MacKenzie, Richard Dennis and last but not least Miss Joanne Askham and the secretaries in Edinburgh together with Frau Doris Maischberger and the secretaries in Garching. December 1978 K.L. Kompa S.D. Smith Conren~ Part I. Study of Lasers and Related Techniques Suitable for Applications in Chemistry and Spectroscopy Rare Gas Halogen Lasers and Photochemical Applications. By S.D. Rockwood ... 3 Group VI Molecular Photolytic Dissociation Studies Using Rare Gas Halide Lasers. By M.C. Gower, A.J. Kearsley, and C.E. Webb ... 8 Broadly Tunable UV Source Based on Stimulated Raman Scattering.
The possibility of initiating chemical reactions by high-intensity laser exci tation has captured the imagination of chemists and physicists as well as of industrial scientists and the scientifically informed public in general ever since the laser first became available. Initially, great hopes were held that laser-induced chemistry would revolutionize synthetic chemistry, making possible "bond-specific" or "mode-specific" reactions that were impos sible to achieve under thermal equilibrium conditions. Indeed, some of the early work in this area, typically employing high-power continuous-wave sources, was interpreted in just this way. With further investigation, however, a more conservative picture has emerged, with the laser taking its place as one of a number of available methods for initiation of high-energy chemical transformations. Unlike a number of these methods, such as flash photolysis, shock tubes, and electron-beam radiolysis, the laser is capable of a high degree of spatial and molecular localization of deposited energy, which in turn is reflected in such applications as isotope enrichment or localized surface treatments. The use of lasers to initiate chemical processes has led to the discovery of several distinctly new molecular phenomena, foremost among which is that of multiple-photon excitation and dissociation of polyatomic molecules. This research area has received the greatest attention thus far and forms the focus of the present volume.
Laser application in chemistry and related fields is an area growing at rapid pace in line with new developments in laser technology. The fields of application range from fundamental chemical research to sophisticated analytical methods in chemical and biotechnological industry and in environmental chemistry. This book demonstrates the breadth of applications of lasers in chemistry, with particular reference to analytical and research applications. David L. Andrews presents the subject matter at a level amenable to the general chemist, the novice and the practising specialists as well. The 3rd edition of this successful book has been completely revised and updated.
This volume contains lectures and seminars presented at the Nato Advanced Study Institute on "Laser Applications to Chemistry" held at San Miniato (Pisa) Italy, June 27 - July 11, 1982. We would like to give our recognition to all who contributed to the superb scientific quality and to the stimulating atmosphere of this summer school. In particular, we thank all speakers and participants in the discussions. We acknowledge the great efforts of Tito Arecchi as the director of the school, and the assistance of Mrs. Maria Bonaria Petrone and Mrs. Giovanna Ravini in the or ganization of the conference. On behalf of all participants we thank Miss Iva Arecchi for the friendly care she has taken and for her profound guidance through its history and the arts of the Toscana during the excursions. We are in particular indebted to Giacinto Scoles who organ ized this meeting together with Karl L. Kompa. Unfortunately, due to health reasons, Giacinto Scoles had to give up the idea of edit ing the proceedings of this meeting. Naturally, the change in the editorial staff caused a delay in the preparation of this volume. The subject of laser application to chemistry has not been review ed comprehensively in recent years. Many of the lectures andsem inars presented in San Miniato had the character of review arti cles. Therefore we feel that the material contained in this vol ume has not lost any of its actuality.