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This comprehensive and up-to-date handbook on this highly topical field, covering everything from new process concepts to commercial applications. Describing novel developments as well as established methods, the authors start with the evaluation of different oxygen carriers and subsequently illuminate various technological concepts for the energy conversion process. They then go on to discuss the potential for commercial applications in gaseous, coal, and fuel combustion processes in industry. The result is an invaluable source for every scientist in the field, from inorganic chemists in academia to chemical engineers in industry.
Calcium and Chemical Looping Technology for Power Generation and Carbon Dioxide (CO2) Capture reviews the fundamental principles, systems, oxygen carriers, and carbon dioxide carriers relevant to chemical looping and combustion. Chapters review the market development, economics, and deployment of these systems, also providing detailed information on the variety of materials and processes that will help to shape the future of CO2 capture ready power plants. - Reviews the fundamental principles, systems, oxygen carriers, and carbon dioxide carriers relevant to calcium and chemical looping - Provides a lucid explanation of advanced concepts and developments in calcium and chemical looping, high pressure systems, and alternative CO2 carriers - Presents information on the market development, economics, and deployment of these systems
This is the first comprehensive guide to the principles and techniques of chemical looping partial oxidation. With authoritative explanations from a pioneer of the chemical looping process, you will: • Gain a holistic overview of metal oxide reaction engineering, with coverage of ionic diffusion, nanostructure formation, morphological evolution, phase equilibrium, and recyclability properties of metal oxides during redox reactions • Learn about the gasification of solid fuels, the reforming of natural gas, and the catalytic conversion of methane to olefins • Understand the importance of reactor design and process integration in enabling metal oxide oxygen carriers to produce desired products • Discover other applications of catalytic metal oxides, including the production of maleic anhydride and solar energy conversions Aspen Plus® simulation software and results accompany the book online. This is an invaluable reference for researchers and industry professionals in the fields of chemical, energy and environmental engineering, and students studying process design and optimization.
In this Ph.D. thesis a system of coupled fluidized bed reactors is modelled and simulated dynamically. Chemical Looping Combustion was used as an exemplary process in both the numerical and the experimental part of this work. For the simulation purpose a novel flowsheeting software was used and models for the needed process units developed and integrated into this software. The needed unit models were three interconnected fluidized bed reactors in circulating and bubbling operation conditions, a cyclone for gas-solid separation and loop seals, which ensured solids transport and gas separation between the reactors. Additionally, lab scale experiments on the reactivity of the used solids, oxygen carrier and solid fuels, were conducted and kinetic parameters extracted. All unit models were connected to a process flowsheet and simulated dynamically. The simulation results were compared to experimental data from a 25 kWth pilot plant operated at the university by the author. It could be shown that a detailed and dynamic simulation of the whole process can be carried out over a time period of more than 45 minutes and the experimental results from start-up, steady state operation and shutdown of the plant were predicted accurately.
Oxy-fuel combustion is currently considered to be one of the major technologies for carbon dioxide (CO2) capture in power plants. The advantages of using oxygen (O2) instead of air for combustion include a CO2-enriched flue gas that is ready for sequestration following purification and low NOx emissions. This simple and elegant technology has attracted considerable attention since the late 1990s, rapidly developing from pilot-scale testing to industrial demonstration. Challenges remain, as O2 supply and CO2 capture create significant energy penalties that must be reduced through overall system optimisation and the development of new processes.Oxy-fuel combustion for power generation and carbon dioxide (CO2) capture comprehensively reviews the fundamental principles and development of oxy-fuel combustion in fossil-fuel fired utility boilers. Following a foreword by Professor János M. Beér, the book opens with an overview of oxy-fuel combustion technology and its role in a carbon-constrained environment. Part one introduces oxy-fuel combustion further, with a chapter comparing the economics of oxy-fuel vs. post-/pre-combustion CO2 capture, followed by chapters on plant operation, industrial scale demonstrations, and circulating fluidized bed combustion. Part two critically reviews oxy-fuel combustion fundamentals, such as ignition and flame stability, burner design, emissions and heat transfer characteristics, concluding with chapters on O2 production and CO2 compression and purification technologies. Finally, part three explores advanced concepts and developments, such as near-zero flue gas recycle and high-pressure systems, as well as chemical looping combustion and utilisation of gaseous fuel.With its distinguished editor and internationally renowned contributors, Oxy-fuel combustion for power generation and carbon dioxide (CO2) capture provides a rich resource for power plant designers, operators, and engineers, as well as academics and researchers in the field. - Comprehensively reviews the fundamental principles and development of oxy-fuel combustion in fossil-fuel fired utility boilers - Provides an overview of oxy-fuel combustion technology and its role in a carbon-constrained environment - Introduces oxy-fuel combustion comparing the economics of oxy-fuel vs. post-/pre-combustion CO2 capture
Fluidization Engineering, Second Edition, expands on its original scope to encompass these new areas and introduces reactor models specifically for these contacting regimes. Completely revised and updated, it is essentially a new book. Its aim is to distill from the thousands of studies those particular developments that are pertinent for the engineer concerned with predictive methods, for the designer, and for the user and potential user of fluidized beds. - Covers the recent advances in the field of fluidization. - Presents the studies of developments necessary to the engineers, designers, and users of fluidized beds.
This book presents the recent research on the separation, purification and downstream utilization of CO2 and other flue gases. Chapters include a detailed discussion on the purification and further conversion of CO2 to commodity chemicals and fuels. With contributions from renowned researchers in the field, the book focuses on the current challenges of catalytic high-pressure chemical conversion and biochemical conversion into high-value products. This book is of interest to researchers, professionals, and students working on carbon capture and sequestration, and is a valuable resource for policy makers and government agents working on guidelines and frameworks for carbon capture and reuse.
Many important industrial chemical processes rely heavily on catalysis and so researchers are always on the lookout for alternative catalytic materials that may improve existing processes or lead to new ones. Families of alternative catalytic materials currently being investigated include the carbides, nitrides and phosphides as well as amorphous boron catalysts. The addition of carbon, nitrogen or phosphorous to transition metals and the creation of boron-transition metal alloys leads to catalytic materials that have interesting properties, with applications in a range of different reactions, including electrocatalysis. This book provides a comprehensive account of the preparation, characterisation and application of these catalytic materials. It is an important reference for researchers and industrialists working in heterogeneous catalysis and materials chemistry.
This book provides the latest global perspective on the role and value of CCS in delivering temperature targets and reducing the impact of global warming.
Carbon dioxide (CO2) capture and conversion to value added products, such as chemicals, polymers, and carbon-based fuels represents a promising approach to transform a potential threat to the environment into a value-added product for long term sustainability. Emerging Carbon Capture Technologies: Towards a Sustainable Future provides a multidisciplinary view of the research that is being carried out in this field, covering materials and processes for CO2 capture and utilization and including a broad discussion of the impact of novel technologies in carbon capture on the energy landscape, society and climate. Of interest to students, researchers and professionals in industries related to greenhouse gas mitigation, post-combustion CO2 capture processes, coal-fired power plants, environmental sustainability, green solvents, green technologies, and the utilization of clean energy for environmental protection, this book covers both the experimental and theoretical aspects of novel materials and process development providing a holistic approach toward a sustainable energy future. - Includes a wide range of processes and their applications - Covers the experimental and theoretical aspects of novel materials and process development - Includes techno-economics analysis, regulation, policies and future prospects