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Understanding charge dynamics and the origin of superconductivity in iron-based materials is one of the most important topics in condensed matter physics. Among different structures of iron-based materials, 122-type iron arsenides are of considerable interest due to their diverse phase diagrams, relatively high superconducting transition temperatures, and the availability of high quality single crystals. In this dissertation, we study temperature and frequency dependence of charge dynamics of the electron-doped 122-type iron arsenides in the metallic and superconducting states using broadband infrared spectroscopy at cryogenic temperatures. We have investigated the charge dynamics and the nature of many-body interactions in metallic La- and Pr- doped CaFe2As2. From the infrared part of the optical conductivity, we discover that the scattering rate of mobile carriers above 200 K exhibits saturation at the Mott-Ioffe-Regel limit of metallic transport. However, the dc resistivity continues to increase with temperature above 200 K due to the loss of Drude spectral weight. The loss of Drude spectral weight with increasing temperature is seen in a wide temperature range in the uncollapsed tetragonal phase, and this spectral weight is recovered at energy scales about one order of magnitude larger than the Fermi energy scale in these semimetals. The phenomena noted above have been observed previously in other correlated metals in which the dominant interactions are electronic in origin. Further evidence of significant electron-electron interactions is obtained from the presence of quadratic temperature and frequency-dependence scattering rate at low temperatures and frequencies in the uncollapsed tetragonal structures of La- and Pr-doped CaFe2As2. We also observe weakening of electronic correlations and a decrease of Drude spectral weight upon the transition to the collapsed tetragonal phase in Pr-doped CaFe2As2. We have measured infrared reflectance spectra of BaFe1.9Pt0.1As2 in the normal and superconducting states. We find that this superconductor has fully gapped Fermi surfaces. Importantly, we observe strong-coupling electron-boson interaction features in the infrared absorption spectra. By using two modeling methods which include strong-coupling effects via the Eliashberg function, we obtain a good quantitative description of the energy gaps and the temperature dependent strong-coupling features. Our experimental data and analysis provide compelling evidence that superconductivity in BaFe1.9Pt0.1As2 is induced by the coupling of electrons to a low energy bosonic mode.
This thesis combines highly accurate optical spectroscopy data on the recently discovered iron-based high-temperature superconductors with an incisive theoretical analysis. Three outstanding results are reported: (1) The superconductivity-induced modification of the far-infrared conductivity of an iron arsenide with minimal chemical disorder is quantitatively described by means of a strong-coupling theory for spin fluctuation mediated Cooper pairing. The formalism developed in this thesis also describes prior spectroscopic data on more disordered compounds. (2) The same materials exhibit a sharp superconductivity-induced anomaly for photon energies around 2.5 eV, two orders of magnitude larger than the superconducting energy gap. The author provides a qualitative interpretation of this unprecedented observation, which is based on the multiband nature of the superconducting state. (3) The thesis also develops a comprehensive description of a superconducting, yet optically transparent iron chalcogenide compound. The author shows that this highly unusual behavior can be explained as a result of the nanoscopic coexistence of insulating and superconducting phases, and he uses a combination of two complementary experimental methods - scanning near-field optical microscopy and low-energy muon spin rotation - to directly image the phase coexistence and quantitatively determine the phase composition. These data have important implications for the interpretation of data from other experimental probes.
This thesis presents analytical theoretical studies on the interplay between charge density waves (CDW) and superconductivity (SC) in the actively studied transition-metal dichalcogenide 1T-TiSe2. It begins by reapproaching a years-long debate over the nature of the phase transition to the commensurate CDW (CCDW) state and the role played by the intrinsic tendency towards excitonic condensation in this system. A Ginzburg-Landau phenomenological theory was subsequently developed to understand the experimentally observed transition from commensurate to incommensurate CDW (ICDW) order with doping or pressure, and the emergence of a superconducting dome that coexists with ICDW. Finally, to characterize microscopically the effects of the interplay between CDW and SC, the spectrum of CDW fluctuations beyond mean-field was studied in detail. In the aggregate, the work reported here provides an encompassing understanding of what are possibly key microscopic underpinnings of the CDW and SC physics in TiSe2.
The parent phases of the Fe-arsenide superconductors harbor an antiferromagnetic ground state. Significantly, the Neel transition is either preceded or accompanied by a structural transition that breaks the four fold symmetry of the high-temperature lattice. Borrowing language from the field of soft condensed matter physics, this broken discrete rotational symmetry is widely referred to as an Ising nematic phase transition. Understanding the origin of this effect is a key component of a complete theoretical description of the occurrence of superconductivity in this family of compounds, motivating both theoretical and experimental investigation of the nematic transition and the associated in-plane anisotropy. Here we review recent experimental progress in determining the intrinsic in-plane electronic anisotropy as revealed by resistivity, reflectivity and ARPES measurements of detwinned single crystals of underdoped Fe arsenide superconductors in the '122' family of compounds.
The authors of this book present a thorough discussion of the optical properties of solids, with a focus on electron states and their response to electrodynamic fields. A review of the fundamental aspects of the propagation of electromagnetic fields, and their interaction with condensed matter, is given. This is followed by a discussion of the optical properties of metals, semiconductors, and collective states of solids such as superconductors. Theoretical concepts, measurement techniques and experimental results are covered in three interrelated sections. Well-established, mature fields are discussed (for example, classical metals and semiconductors) together with modern topics at the focus of current interest. The substantial reference list included will also prove to be a valuable resource for those interested in the electronic properties of solids. The book is intended for use by advanced undergraduate and graduate students, and researchers active in the fields of condensed matter physics, materials science and optical engineering.
Since the discovery of superconductivity, a great number of theoretical and experimental efforts have been made to describe this new phase of matter that emerged in many body systems. In this regard, theoretical models have been presented; the most famous of which was the BCS theory that can only describe conventional superconductors. With the discovery of new class superconductors, the superconducting mechanism became a new challenge in the field of condensed matter physics. This unexpected discovery opened a new area in the history of superconductivity, and experimental researchers started trying to find new compounds in this class of superconductors. These superconductors are often characterized by the anisotropic character in the superconducting gap function with nodes along a certain direction in the momentum space. Since the pairing interaction has an important role in the superconducting gap structure, its determination is very important to explain the basic pairing mechanism.In this regard, this book includes valuable theoretical and experimental discussions about the properties of superconductors. Here you will find valuable research describing the properties of unconventional superconductors.