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Proceedings of the NATO Advanced Study Institute, Durham, New Hampshire, U.S.A., July 19-30, 1982
The oceans and atmosphere interact through various processes, including the transfer of momentum, heat, gases and particles. In this book leading international experts come together to provide a state-of-the-art account of these exchanges and their role in the Earth-system, with particular focus on gases and particles. Chapters in the book cover: i) the ocean-atmosphere exchange of short-lived trace gases; ii) mechanisms and models of interfacial exchange (including transfer velocity parameterisations); iii) ocean-atmosphere exchange of the greenhouse gases carbon dioxide, methane and nitrous oxide; iv) ocean atmosphere exchange of particles and v) current and future data collection and synthesis efforts. The scope of the book extends to the biogeochemical responses to emitted / deposited material and interactions and feedbacks in the wider Earth-system context. This work constitutes a highly detailed synthesis and reference; of interest to higher-level university students (Masters, PhD) and researchers in ocean-atmosphere interactions and related fields (Earth-system science, marine / atmospheric biogeochemistry / climate). Production of this book was supported and funded by the EU COST Action 735 and coordinated by the International SOLAS (Surface Ocean- Lower Atmosphere Study) project office.
This book arises from a NATO-sponsored Advanced Study Institute on 'The Role of Air-Sea Exchange in Geochemical Cycling' held at Bombann@§. near Bordeaux, France. from 16 to 27 September 1985. The chapters of the book are the written versions of the lectures given at the Institute. The aim of the book is to give a comprehensive up-to-date coverage of the subject. presented in a teaching mode. The chapters contain much recent research material and attempt to give the reader an understanding of how the role of air-sea exchange in geochemical cycling can be quantitatively assessed. In the last decade, major advances in the fields of marine and atmospheric chemistry have underlined the role of physical, chemical and biological processes at and near the air-sea interface in a number of geochemical cycles (C. S, N, metals etc ... ). Further, there is strong concern over the anthropogenic perturbation of these cycles on both regional and global scales. The first part of the book (Chapters 1 to 8) provides a review of topics fundamental to such studies. These topics include concepts in geochemical modelling, assessment of atmospheric transport from sources to the oceans. description of mixing and transport processes within the ocean for both dissolved and particulate materials, quantification of air-sea fluxes for both gases and particles, photochemical transformations in the atmospheric and oceanic boundary layers.
The transfer across the surface of environmental waters is of interest as an important phase in the geophysical and natural biochemical cycles of numer ous substances; indeed it governs the transition, one way or the other, be tween the dissolved state in the water and the gaseous state in the atmo sphere. Especially with increasing population and industrialization, gas transfer at water surfaces has become a critical factor in the understanding of the various pathways of wastes in the environment and of their engineering management. This interfacial mass transfer is, by its very nature, highly complex. The air and the water are usually in turbulent motion, and the interface be tween them is irregular, and disturbed by waves, sometimes accompanied by breaking, spray and bubble formation. Thus the transfer involves a wide variety of physical phenomena occurring over a wide range of scales. As a consequence, scientists and engineers from diverse disciplines and problem areas, have approached the problem, often with greatly differing analytical and experimental techniques and methodologies.
This revised and updated study is about the atmosphere and humanity's influence on it. Following an analysis of the natural environment, it re-examines the sources of air pollution and its effects, including decline in health, damage to plants and animals, indoor pollution, and acid rain.
During the 1980's a wealth of information was reported from field and laboratory experiments in order to validate andlor modify various aspects of the surface layer Monin-Obukhov (M-O) similarity theory for use over the sea, and to introduce and test new concepts related to high resolution flux magnitudes and variabilities. For example, data from various field experiments conducted on the North Sea, Lake Ontario, and the Atlantic experiments, among others, yielded information on the dependence of the flux coefficients on wave state. In all field projects, the usual criteria for satisfying M-O similarity were applied. The assumptions of stationarity and homogeneity was assumed to be relevant over both small and large scales. In addition, the properties of the outer layer were assumed to be "correlated" with properties of the surface layer. These assumptions generally required that data were averaged for spatial footprints representing scales greater than 25 km (or typically 30 minutes or longer for typical windspeeds). While more and more data became available over the years, and the technology applied was more reliable, robust, and durable, the flux coefficients and other turbulent parameters still exhibited significant unexplained scatter. Since the scatter did not show sufficient reduction over the years to meet customer needs, in spite of improved technology and heavy financial investments, one could only conclude that perhaps the use of similarity theory contained too many simplifications when applied to environments which were more complicated than previously thought.
Chemical Dynamics in Freshwater Ecosystems reviews the processes that control the distribution and impacts of chemical substances discharged into freshwater aquatic environments. The book focuses on the relationships between chemical emissions and the resulting ambient concentration in water, sediments, fish, benthos, plants, and other components of real aquatic ecosystems. Hydrodynamics, sediment dynamics, chemical fate processes, bioaccumulation, and food-chain transfer are major topics discussed in the book. Case studies and models are used to illustrate how quantitative predictions of chemical dynamics and behavior in the aquatic environment can be made. Chemical Dynamics in Freshwater Ecosystems is an excellent reference for aquatic toxicologists, wildlife toxicologists, wildlife biologists, environmental chemists, governmental regulators, environmental modelers, consultants, and students studying the effects of chemicals on aquatic environments.
Our world is changing at an accelerating rate. The global human population has grown from 6.1 billion to 7.1 billion in the last 15 years and is projected to reach 11.2 billion by the end of the century. The distribution of humans across the globe has also shifted, with more than 50 percent of the global population now living in urban areas, compared to 29 percent in 1950. Along with these trends, increasing energy demands, expanding industrial activities, and intensification of agricultural activities worldwide have in turn led to changes in emissions that have altered the composition of the atmosphere. These changes have led to major challenges for society, including deleterious impacts on climate, human and ecosystem health. Climate change is one of the greatest environmental challenges facing society today. Air pollution is a major threat to human health, as one out of eight deaths globally is caused by air pollution. And, future food production and global food security are vulnerable to both global change and air pollution. Atmospheric chemistry research is a key part of understanding and responding to these challenges. The Future of Atmospheric Chemistry Research: Remembering Yesterday, Understanding Today, Anticipating Tomorrow summarizes the rationale and need for supporting a comprehensive U.S. research program in atmospheric chemistry; comments on the broad trends in laboratory, field, satellite, and modeling studies of atmospheric chemistry; determines the priority areas of research for advancing the basic science of atmospheric chemistry; and identifies the highest priority needs for improvements in the research infrastructure to address those priority research topics. This report describes the scientific advances over the past decade in six core areas of atmospheric chemistry: emissions, chemical transformation, oxidants, atmospheric dynamics and circulation, aerosol particles and clouds, and biogeochemical cycles and deposition. This material was developed for the NSF's Atmospheric Chemistry Program; however, the findings will be of interest to other agencies and programs that support atmospheric chemistry research.
This book presents an up-to-date analysis of ocean-atmosphere interaction. Well known experts examine diverse subjects such as ocean surface waves, air-sea exchange processes, ocean surface mixed layer, water-mass formation, as well as general circulation of the oceans, El Nino and Southern Oscillation (ENSO), and the deep-ocean circulation. Other areas described are basic dynamics, data analysis techniques, numerical modelling, and remote sensing. This book is primarily aimed at graduate and senior undergraduate courses in the area of ocean-atmosphere research.
The past two or three decades have seen many important advances in our knowledge of the chemistry, physics, geology and biology of the oceans. It has also become apparent that in order to understand the manner in which the oceans work as a 'chemical system', it is necessary to use a framework which takes account of these interdisciplinary advances. Marine geochemistry has been written in response to the need for a single state-of-the-art text that addresses the subject of treating the sea water, sediment and rock reservoirs as a unified system. In taking this approach, a process-orientated framework has been adopted in which the emphasis is placed on identifying key processes operating within the 'unified ocean'. In doing this, particular attention has been paid to making the text accessible to students from all disciplines in such a way that future advances can readily be understood. I would like to express my thanks to those people who have helped with the writing of this volume. In particular, I wish to put on record my sincere appreciation of extremely helpful suggestions made by Professor John Edmond, FRS. In addition, I thank Dr S. Rowlatt for his comments on the sections covering the geochemistry of oceanic sediments, and Dr G. Wolff for his invaluable advice on the organic geochemistry of biota, water and sediments. It is a great pleasure to acknowledge the help of Dr K. J. T.