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This book describes advances in both experimental and theoretical treatments in the field of energy transfer processes that are relevant to various fields, such as spectroscopy, laser technology, phosphors, artificial solar energy conversion, and photobiology. It presents the principles and available techniques through specific examples. In addition, it examines current and possible applications, including the most recent developments, and projects future advances and research possibilities in the field. Contents: Fundamental Interactions Leading to Energy Transfer (B Di Bartolo); Energy Transfer Processes in Atoms and Molecules (W DemtrAder et al.); Advances in the Techniques for the Study of Energy Transfer (D Hulin); Upconversion Phenomena with Laser Applications (X Chen); New Applications of Ultrafast Spectroscopy (J M Hvam); Efficient Solid State Lasers (N P Barnes); Emission Efficiency and Energy Transfer in Color Centers at High Concentrations (G Baldacchini); Four-Wave Mixing Studies of Energy Transfer Processes (G Boulon); Upconventional Light Emissions in Rare-Earth Doped Solids (F Auzel); Photonic Molecular and Supramolecular Devices (J M Lehn); Reflections on the Theory of Everything (G Costa); Earthquakes, Measurements, and Mitigation of Seismic Risk (R Console); Site Selectivity of Defects in IIIOCoV Compounds by Local Mode Spectroscopy and Model Calculations (D N Talwar); The General Non-Radiative Energy Transfer Master Equations for Crystalline Materials, the Exact Solution and Current Modeling (L A D az-Torres et al.); and other papers. Readership: Researchers and graduate students in the fields of lasers and optics."
Applying a unified quantum approach, contributors offer fresh insights into the theoretical developments in the excitation energy transfer processes in condensed matter. This comprehensive volume examines Frenkel and Wannier excitonic processes; rates of excitonic processes; theory of laser sputter and polymer ablation; and polarons, excitonic polarons and self-trapping.
This book presents an account of the NATO Advanced Study Institute on "Energy Transfer Processes in Condensed Matter", held in Erice, Italy, from June 16 to June 30, 1983. This meeting was organized by the International School of Atomic and Molecular Spectroscopy of the "Ettore Majorana" Centre for Scientific Culture. The objective of the Institute was to present a comprehensive treatment of the basic mechanisms by which electronic excitation energy, initially localized in a particular constituent or region of a condensed material, transfers itself to the other parts of the system. Energy transfer processes are important to such varied .fields as spectroscopy, lasers, phosphor technology, artificial solar energy conversion, and photobiology. This meeting was the first encounter of this sort entirely dedicated to this important topic. A total of 65 participants came from 47 laboratories and 16 nations (Belgium, Czechoslovakia, F.R. of Germany, France, Greece, India, Ireland, Israel, Italy, The Netherlands, Poland, Portugal, Switzerland, Turkey, United Kingdom, and the United States of A America). The secretaries of the course were: Ms. Aliki Karipidou for the scientific aspects and Mr. Massimo Minella for the admini strative aspects of the meeting.
An accessible yet rigorous introduction to nanophotonics, covering basic principles, technology, and applications in lighting, lasers, and photovoltaics. Providing a wealth of information on materials and devices, and over 150 color figures, it is the 'go-to' guide for students in electrical engineering taking courses in nanophotonics.
We have made substantial progress in experimental and theoretical studies in two areas: Photoinduced donor to acceptor electron transfer followed by back transfer in random solutions; and electronic excitation transport in systems with complex inhomogeneous spatial geometries and inhomogeneous energy distributions. Through the development of accurate statistical mechanical theories, we have been able to relate dynamics in complex systems to experimental observables. We have then used the experimental observables, time resolved fluorescence depolarization and transient grating experiments, to examine well defined molecular systems. The agreement between theory and experiment is excellent. 11 refs.
This program involves the experimental and theoretical study of optically induced electron transfer and electronic excitation transport in systems with complex structures. The focus is to obtain an understanding of the intimate interplay among intermolecular interactions, structure, and dynamics. A combination of picosecond transient grating experiments, time resolved fluorescence depolarization experiments, conventional optical spectroscopy, and statistical mechanical theory is being employed to elucidated fundamental aspects of processes which are important in the conversion of solar energy to usable forms of energy. We are continuing to address the very important problem of electron back transfer following optically induced donor to acceptor electron transfer. In a system in which there are donors (low concentration) and acceptors (high concentration) randomly distributed in solution, optical excitation of a donor can be followed by transfer of an electron to an acceptor. One electron transfer has occurred. there exists a ground state radical cation (D) near a ground state radical anion (A−). Since the thermodynamically stable state is neutral ground state D and A, back transfer will occur. The electron will back transfer from A− to D to regenerate the neutral species. In liquid solution, back transfer competes with separation by diffusion. Separated ions are extremely reactive and can go on to do useful chemistry. 10 refs.
The program involves the investigation of excitation transport and electron transfer in complex systems. In the area of electron transfer, we have been studying electron back transfer following donor-acceptor photoinduced electron transfer. We are addressing this problem both theoretically and experimentally. In the area of excitation transport, we have been examining transport in solid solutions, liquid solutions, and in clustered excitation transport systems. Again, we are pursuing both experimental and theoretical approaches. The problem of electron back transfer between photogenerated ions is of central importance in both artificial and biological solar energy conversion. Once an electron has been transferred from an optically excited donor to an acceptor, back transfer competes with the ability of the radical ions to go on to do useful chemistry. We are studying the back transfer process using picosecond transient grating experiments in conjunction with time resolved and steady state fluorescence quenching measurements. The transient grating experiments makes the back transfer process a direct experimental observable, while the fluorescence experiments allow the forward transfer to be examined. By combining the experiments, a complete picture emerges. 10 refs.
Charge and Energy Transfer Dynamics in Molecular Systems Comprehensive resource offering knowledge on charge and energy transfer dynamics in molecular systems and nanostructures Charge and Energy Transfer Dynamics in Molecular Systems provides a unified description of different charge and energy transfer phenomena in molecular systems with emphasis on the theory, bridging the regimes of coherent and dissipative dynamics and thus presenting classic rate theories as well as modern treatments of ultrafast phenomena. Starting from microscopic models, the common features of the different transfer processes are highlighted, along with applications ranging from vibrational energy flow in large polyatomic molecules, the motion of protons in solution, up to the concerted dynamics of electronic and nuclear degrees of freedom in molecules and molecular aggregates. The newly revised and updated Fourth Edition contains a more detailed coverage of recent developments in density matrix theory, mixed quantum-classical methods for dynamics simulations, and a substantially expanded treatment of time-resolved spectroscopy. The book is written in an easy-to-follow style, including detailed mathematical derivations, thus making even complex concepts understandable and applicable. Charge and Energy Transfer Dynamics in Molecular Systems includes information on: Electronic and vibrational molecular states, covering molecular Schrödinger equation, Born—Oppenheimer separation and approximation, Hartree-Fock equations and other electronic structure methods Dynamics of isolated and open quantum systems, covering multidimensional wave packet dynamics, and different variants of density operator equations Interaction of molecular systems with radiation fields, covering linear and nonlinear optical response using the correlation function approach Intramolecular electronic transitions, covering optical transition and internal conversion processes Transfer processes of electrons, protons, and electronic excitation energy Providing in-depth coverage of the subject, Charge and Energy Transfer Dynamics in Molecular Systems is an essential resource for anyone working on timely problems of energy and charge transfer in physics, chemistry and biophysics as well as for all engaged in nanoscience and organic electronics.
Modulating the spectroscopic overlap between the emission bands of donors and the absorption spectra of acceptors by various simulations, it is possible to systematically investigate the emission behaviors of lanthanide complexes under different conditions. To establish the relationships between emission behaviors and various external simulations, it is necessary to study the energy transfer rate and efficiency between the donor and acceptor under different conditions to clarify the luminescent mechanism of the complexes, providing a theoretical basis for high-performance smart materials. This review focuses on the recent progress of luminescence performance of lanthanide complexes, including energy transfer mechanisms, emission color modulation, the strategies for optimizing lanthanide luminescence, and finally, various applications based on luminescence performance of lanthanide complexes and lanthanide metal-organic frameworks.