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Neutrinos can arguably be labeled as the most fascinating elementary particles known as their small but non-zero rest mass points to new mass generating mechanisms beyond the Standard Model, and also assigns primordial neutrinos from the Big Bang a distinct role in shaping the evolution of large-scale structures in the universe. The open question of the absolute neutrino mass scale will be addressed by the Karlsruhe Tritium Neutrino (KATRIN) experiment, currently under construction. This thesis reports major contributions to developing and implementing new laser-spectroscopic precision tools to continuously monitor the isotope content of the windowless gaseous tritium source of KATRIN. The method of choice, Raman spectroscopy, is ideally suited for in-situ monitoring of all six hydrogen isotopologues. In a series of beautiful experiments the author obtained two independent novel calibration methods, first based on a comparison of experimental Raman depolarization ratios with corresponding quantum-chemical calculations, and second on a gas sampling technique. Both methods yield consistent cross-calibration results and, as well as yielding improvements in precision, will be of major importance in reducing systematic effects in long-term neutrino mass measurements. The methods developed in this thesis also have great potential to further broaden the applications of Raman spectroscopy to study extended sources such as in atmospheric physics.
This book presents the latest technological advances in Raman spectroscopy that are presently redrawing the landscape of many fields of biomedical and pharmaceutical R&D. Numerous examples are given to illustrate the application of the new methods.
The increasing concern about CO2 emissions and energy prices has led to new CO2 emission and fuel economy legislation being introduced in world regions served by the automotive industry. In response, automotive manufacturers and Tier-1 suppliers are developing a new generation of internal combustion (IC) engines with ultra-low emissions and high fuel efficiency. To further this development, a better understanding is needed of the combustion and pollutant formation processes in IC engines. As efficiency and emission abatement processes have reached points of diminishing returns, there is more of a need to make measurements inside the combustion chamber, where the combustion and pollutant formation processes take place. However, there is currently no good overview of how to make these measurements. Based on the author’s previous SAE book, Engine Combustion Instrumentation and Diagnostics, this book focuses on laser-based optical techniques for combustion flows and in-cylinder measurements. Included are new chapters on optical engines and optical equipment, case studies, and an updated description of each technique. The purpose of this book is to provide, in one publication, an introduction to experimental techniques that are best suited for in-cylinder engine combustion measurements. It provides sufficient details for readers to set up and apply these techniques to IC engines and combustion flows.
This work covers principles of Raman theory, analysis, instrumentation, and measurement, specifying up-to-the-minute benefits of Raman spectroscopy in a variety of industrial and academic fields, and how to cultivate growth in new disciplines. It contains case studies that illustrate current techniques in data extraction and analysis, as well as over 500 drawings and photographs that clarify and reinforce critical text material. The authors discuss Raman spectra of gases; Raman spectroscopy applied to crystals, applications to gemology, in vivo Raman spectroscopy, applications in forensic science, and collectivity of vibrational modes, among many other topics.
This book explains physical principles, unique benefits, broad categories, implementation aspects, and performance criteria of distributed optical fiber sensors (DOFS). For each kind of sensor, the book highlights industrial applications, which range from oil and gas production to power line monitoring, plant and process engineering, environmental monitoring, industrial fire and leakage detection, and so on. The text also includes a discussion of such key areas as backscattering, launched power limitations, and receiver sensitivity, as well as a concise historical account of the field’s development.