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Methane plays many important roles in the earth's environment. It is a potent "greenhouse gas" that warms the earth; controls the oxidizing capacity of the atmosphere (OH) indirectly affecting the cycles and abundances of many atmospheric trace gases; provides water vapor to the stratosphere; scavenges chlorine atoms from the stratosphere, terminating the catalytic ozone destruction by chlorine atoms, including the chlorine released from the man-made chlorofluorocarbons; produces ozone, CO, and CO2 in the troposphere; and it is an index of life on earth and so is present in greater quantities during warm interglacial epochs and dwindles to low levels during the cold of ice ages. By all measures, methane is the second only to CO2 in causing future global warming. The book presents a comprehensive account of the current understanding of atmospheric methane, and it is an end point for summarizing more than a decade of intensive research on the global sources, sinks, concentrations, and environmental role of methane.
The analysis of polar ice cores has proven to be very instructive about past environmental conditions on the time scale of several climatic cycles, and recent drilling operations have provided information of great value for global change issues. The book presents the most recent data extracted from Greenland ice cores and surface experiments and compares them with former Antarctic results. It contains background articles, original contributions and group reports of interest to scientists, climatologists, atmospheric chemists, and glaciologists involved in global change research.
Polar ice cores have provided tremendous advances in our knowledge of past climate change. They also contain an archive of geochemical data, which can certainly delineate some of the forcing factors that govern climate change. However, our ability to interpret these data is severely curtailed by lack of knowledge of the processes governing the transfer of chemical species from the air to the snow. This book outlines the potential and problems of ice core chemistry and discusses the processes involved in air-snow transfer. It gives the state of current knowledge and an agenda for future research.
One of the major findings in the 1992 IPCC report and the 1994 World Meteorological Organization's Ozone Assessment report was the identification of possible climatic effects over the last few decades resulting from anthropogenic ally-induced changes in atmospheric ozone. The initial quantitative estimates of their direct climatic effects indicate significant impacts, though large uncertainties exist and studies using general circulation models are needed. A point that needs to be addressed in particular is that atmospheric ozone differs from greenhouse gases in that it is formed and destroyed by chemical processes in the atmosphere due to interaction involving a large number of source gases (e. g. H0, NO ' CO, 2 x NMHC, N0, CH and the CFCs). Therefore, the indirect effect of climate-chemistry 2 4 interaction involving atmospheric ozone is an important aspect for consideration in general circulation models. During the last few years, there have been several international workshops related to atmospheric ozone. In 1987, a NATO workshop on atmospheric ozone was held in Lillehammer, Norway. More recently, two workshops were organized to discuss the topic "General Circulation Model Study of Climate-Chemistry Interaction. " The first was held August 19-21, 1992, in Oslo, Norway, and the second held May 26-27,1993, in Albany, New York, USA. The two workshops were IAMAP activities under the Trace Constituent Working Group.
The Arctic troposphere (0 to ca. 8 km) plays an important role in environmental concerns for global change. It is a unique chemical reactor influenced by human activity and the Arctic ocean. It is surrounded by industrialized continents that in winter contribute gaseous and particulate pollution (Arctic haze). It is underlain by the flat Arctic ocean from which it is separated by a crack-ridden ice membrane 3 to 4 m thick. Ocean to atmosphere exchange of heat, water vapor and marine biogenic gases influence the composition of the reactor. From September 21 to December 21 to March 21, the region north of the Arctic circle goes from a completely sunlit situation to a completely dark one and then back to light. At the same time the lower troposphere is stably stratified. This hinders vertical mixing. During this light period, surface temperature reaches as low as -40°C. In this environment, chemical reactions involving sunlight are generally much slower than further south. Thus, the abundance of photochemically reactive compounds in the atmosphere can be high prior to polar sunrise. Between complete dark in February and complete light in April, a number of chemical changes in the lower troposphere take place.
Presented here are authoritative and up-to-date assessments of the homogenous and heterogenous chemical and physical processes occuring in the troposphere and stratosphere, especially during the "ozone hole" event. The book begins with an overview of atmospheric chemistry, followed by reviews of relevant homogenous reactions in the gas phase and the microphysics and physical chemistry of heterogenous processes that occur on, or in aerosols, rain and ice. Low temperature laboratory studies are compared with related fieldwork measurements, particularly in relation to the formation and composition of polar stratospheric clouds. Also discussed are measurements in glacial ice. Finally chemical modelling of the troposphere and stratosphere, including heterogenous processes, is reviewed.
Antarctica is no longer a 'pole apart'. From a scientific perspective, the Antarctic ice sheet, ocean and climate systems are intimately linked with the global climate and are now seen to be of international significance for understanding climate change. From an economic perspective, the Antarctic is perceived to have great potential as a source of marine resources although the extent of speculated mineral and hydrocarbon resources is unknown. From a conservation perspective, the continent of Antarctica represents the ideal image of unspoiled wilderness. Antarctic Environments and Resources is an accessible and timely new geography of the Antarctic which examines the differing and sometimes conflicting interests in the great southern continent, the Southern Ocean and the subantarctic islands against a background of the physical and natural systems of the region and their interactions. It charts the development of human involvement in the area, focusing on the exploitation of resources from early sealing to modern fisheries, tourism and science, and it assesses the consequent impacts on the natural environment. The text also reviews the emerging framework for future environmental management developed under the Antarctic Treaty System. This is an ideal text for undergraduates studying glacial geomorphology, environmental management, polar regions and the Antarctic.
Praise for Guy P. Brasseur's Atmospheric Chemistry in a Changing World American Meteorological Society "This volume summarizes and integrates more than a decade of atmospheric chemistry research. During the period under consideration, great progress has been made in computing, modeling, and observational techniques, and methods have also improved. Here, suggestions for the highest priority research for the next decade are made, and important information is related regarding impacts on the environment."
This book considers the effects of life on the Earth's chemistry on a global level.