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This thesis presents the first successful realization of a compact, low-noise, and few-cycle light source in the mid-infrared wavelength region. By developing the technology of pumping femtosecond chromium-doped II-VI laser oscillators directly with the emission of broad-stripe single-emitter laser diodes, coherent light was generated with exceptionally low amplitude noise — crucial for numerous applications including spectroscopy at high sensitivities. Other key parameters of the oscillator's output, such as pulse duration and output power, matched and even surpassed previous state-of-the-art systems. As a demonstration of its unique capabilities, the oscillator's powerful output was used to drive — without further amplification — the nonlinear generation of coherent mid-infrared light spanning multiple octaves. The resulting table-top system uniquely combines high brilliance and ultrabroad spectral bandwidth in the important mid-infrared spectral range. The rapid development of this technology is comprehensively and lucidly documented in this PhD thesis. Together with a thorough review of literature and applications, and an extensive analysis of the theoretical foundations behind ultrafast laser oscillators, the thesis will serve as a valuable reference for the construction of a new generation of mid-infrared light sources.
"The presence of vibrational and rotational transition lines in the mid-infrared (MIR) (2-10 æm) spectral range has stimulated numerous applications in the fields of spectroscopy, sensing and medicine. These emerging applications have intensified the research effort for the growth and development of novel optical light sources. Nonlinear effects in glass fibers are being extensively studied to generate ultrafast pulses at this wavelength range. Highly nonlinear silica fiber has shown record performance in the telecommunication wavelength band, however the strong material absorption of silica glass at wavelengths>2 æm limits its applicability in MIR. Recently, due to the extended MIR transmission (>12 æm wavelength) and ultra-high nonlinear gain, chalcogenide (ChG) fibers have attracted a great deal of attention and being widely investigated as an efficient solution towards this end. ChG microwires, in addition, enable engineerable chromatic dispersion, thereby allowing easy access to different nonlinear processes for pulse generation. This dissertation explores the potential of ChG microwires for generation of ultrafast pulses at MIR wavelengths. Several different all-fiber optical sources are developed as a result of the nonlinear processes implemented to reach these wavelengths. This includes the design and development of parametric oscillators and mode-locked lasers, four-wave mixing wavelength converters, Raman soliton generation systems and supercontinuum lasers. The demonstrated sources generate pulses of wide range of temporal duration and power level, while covering a wavelength range of 1.9 æm to 3.0 æm with broadband and/or selective wavelength tunability. The numerical investigation of the underlying nonlinear process are also performed to confirm and predict the experimental behavior. Owing to their compactness, hand-portability, low power consumption and broad operation window, these novel optical sources are expected find wide range of applications in MIR spectroscopy and sensing"--
This thesis presents first successful experiments to carrier-envelope-phase stabilize a high-power mode-locked thin-disk oscillator and to compress the pulses emitted from this laser to durations of only a few-optical cycles. Moreover, the monograph introduces several methods to achieve power-scalability of compression and stabilization techniques. All experimental approaches are compared in detail and may serve as a guideline for developing high-power waveform controlled, few-cycle light sources which offer tremendous potential to exploit extreme nonlinear optical effects at unprecedentedly high repetition rates and to establish table-top infrared light sources with a unique combination of brilliance and bandwidth. As an example, the realization of a multi-Watt, multi-octave spanning, mid-infrared femtosecond source is described. The thesis starts with a basic introduction to the field of ultrafast laser oscillators. It subsequently presents additional details of previously published research results and establishes a connection between them. It therefore addresses both newcomers to, and experts in the field of high-power ultrafast laser development.
A description of procedures for probing bond activation, H-bonded systems, molecular dynamical mechanisms, vibrational dephasing, simple liquids, and proteins and energy flow effects using ultrafast vibrational spectroscopy experiments. It discusses experimental and theoretical methods of ultrafast infrared and Raman measurements.
The book describes the most advanced techniques for generating coherent light in the mid-infrared region of the spectrum. These techniques represent diverse areas of photonics and include heterojunction semiconductor lasers, quantum cascade lasers, tunable crystalline lasers, fiber lasers, Raman lasers, and optical parametric laser sources. Offering authoritative reviews by internationally recognized experts, the book provides a wealth of information on the essential principles and methods of the generation of coherent mid-infrared light and on some of its applications. The instructive nature of the book makes it an excellent text for physicists and practicing engineers who want to use mid-infrared laser sources in spectroscopy, medicine, remote sensing and other fields, and for researchers in various disciplines requiring a broad introduction to the subject.
This book covers the physics, technology and applications of short pulse laser sources that generate pulses with durations of only a few optical cycles. The basic design considerations for the different systems such as lasers, parametric amplifiers and external compression techniques which have emerged over the last decade are discussed to give researchers and graduate students a thorough introduction to this field. The existence of these sources has opened many new fields of research that were not possible before. These are UV and EUV generation from table-top systems using high-harmonic generation, frequency metrology enabling optical frequency counting, high-resolution optical coherence tomography, strong-field ultrafast solid-state processes and ultrafast spectroscopy, to mention only a few. Many new applications will follow. The book attempts to give a comprehensive, while not excessive, introduction to this exciting new field that serves both experienced researchers and graduate students entering the field. The first half of the book covers the current physical principles, processes and design guidelines to generate pulses in the optical range comprising only a few cycles of light. Such as the generation of relatively low energy pulses at high repetition rates directly from the laser, parametric generation of medium energy pulses and high-energy pulses at low repetition rates using external compression in hollow fibers. The applications cover the revolution in frequency metrology and high-resolution laser spectroscopy to electric field synthesis in the optical range as well as the emerging field of high-harmonic generation and attosecond science, high-resolution optical imaging and novel ultrafast dynamics in semiconductors. These fields benefit from the strong electric fields accompanying these pulses in solids and gases during events comprising only a few cycles of light.
Broadly tunable lasers continue to have a tremendous impact in many and diverse fields of science and technology. From a renaissance in laser spectroscopy to Bose-Einstein condensation, the one nexus is the tunable laser. Tunable Laser Applications describes the physics and architectures of widely applied tunable laser sources. Fully updated and ex
An important guide to the major techniques for generating coherent light in the mid-infrared region of the spectrum Laser-based Mid-infrared Sources and Applications gives a comprehensive overview of the existing methods for generating coherent light in the important yet difficult-to-reach mid-infrared region of the spectrum (2–20 μm) and their applications. The book describes major approaches for mid-infrared light generation including ion-doped solid-state lasers, fiber lasers, semiconductor lasers, and laser sources based on nonlinear optical frequency conversion, and reviews a range of applications: spectral recognition of molecules and trace gas sensing, biomedical and military applications, high-field physics and attoscience, and others. Every chapter starts with the fundamentals for a given technique that enables self-directed study, while extensive references help conduct deeper research. Laser-based Mid-infrared Sources and Applications provides up-to-date information on the state-of the art mid-infrared sources, discusses in detail the advancements made over the last two decades such as microresonators and interband cascade lasers, and explores novel approaches that are currently subjects of intense research such as supercontinuum and frequency combs generation. This important book: • Explains the fundamental principles and major techniques for coherent mid-infrared light generation • Discusses recent advancements and current cutting-edge research in the field • Highlights important biomedical, environmental, and military applications Written for researchers, academics, students, and engineers from different disciplines, the book helps navigate the rapidly expanding field of mid-infrared laser-based technologies.
Ultrashort laser pulses with durations in the femtosecond range up to a few picoseconds provide a unique method for precise materials processing or medical applications. Paired with the recent developments in ultrashort pulse lasers, this technology is finding its way into various application fields. The book gives a comprehensive overview of the principles and applications of ultrashort pulse lasers, especially applied to medicine and production technology. Recent advances in laser technology are discussed in detail. This covers the development of reliable and cheap low power laser sources as well as high average power ultrashort pulse lasers for large scale manufacturing. The fundamentals of laser-matter-interaction as well as processing strategies and the required system technology are discussed for these laser sources with respect to precise materials processing. Finally, different applications within medicine, measurement technology or materials processing are highlighted.
Covering fundamental principles and the state of the art, this is a collection of reviews from experts in mid-infrared (mid-IR) coherent sources. Among the sources covered are optical parametric oscillators, difference frequency generators, and the most recent broadband crystalline, quantum cascade, and fiber lasers. The authors show how advances in mid-IR science and technology make these sources indispensable for a variety of applications.